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A study on zeolite-based adsorbents for \(\hbox {CO}_{2}\) capture

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Abstract

In this study, zeolite-based sorbents were prepared and examined for \(\hbox {CO}_{2}\) adsorption from a simulated flue gas mixture using a fixed-bed flow reactor. Various amines such as monoethanolamine, ethylenediamine, diethylenetriamine and triethylenetetramine (TETA) were impregnated on support materials to prepare the adsorbents. Also, the effects of various parameters on \(\hbox {CO}_{2}\) adsorption capacity have been examined in this work. Further, an effort has been made to characterize various physico-chemical properties like surface area, pore volume, chemical composition, etc. of the in-house developed sorbents. Observation showed that the \(\hbox {CO}_{2}\) adsorption capacity enhanced with amine loading up to a certain concentration. The maximum carbon capture capacity of the 30-TETA-ZSM-5 sorbent is around 53 g of \(\hbox {CO}_{2}/\hbox {kg}\) of adsorbent. The thermo-chemical stability of the adsorbents has been tested by reusing the same material for multiple adsorption–desorption cycles, and no significant change in \(\hbox {CO}_{2}\) adsorption capacities was observed.

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Acknowledgements

The authors express their gratitude to the Council of Scientific and Industrial Research (CSIR), India, for funding (CSIR No: 22(0694)/15/EMR-II) the present research work and also grateful to the BITS–Pilani Hyderabad Campus for extending the necessary support for the present study.

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Authors and Affiliations

  1. Department of Chemical Engineering, Birla Institute of Technology and Science, Pilani–Hyderabad Campus, Hyderabad, 500078, India

    Srikanta Dinda, Premanath Murge & Bipin Chakravarthy Paruchuri

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  1. Srikanta Dinda
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  2. Premanath Murge
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  3. Bipin Chakravarthy Paruchuri
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Correspondence to Srikanta Dinda.

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Dinda, S., Murge, P. & Chakravarthy Paruchuri, B. A study on zeolite-based adsorbents for \(\hbox {CO}_{2}\) capture. Bull Mater Sci 42, 240 (2019). https://doi.org/10.1007/s12034-019-1936-8

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  • DOI: https://doi.org/10.1007/s12034-019-1936-8

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