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Efficient and practical adsorption of mixed anionic dyes in aqueous solution by magnetic NiFe-layered double oxide

  • Environmental Engineering
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Abstract

The present research reports the adsorption capacity of magnetic NiFe-layered double oxide (NiFe-LDO) derived from the heat treatment of NiFe-layered double hydroxide (NiFe-LDH) on capturing of single anionic dye and mixed dyes in water. The formation and characteristics of NiFe-LDH and NiFe-LDO were verified by XRD, FT-IR, SEM, BET, VSM and UV-VIS. The obtained NiFe-LDO was mainly composed of NiFe2O4 and NiO phases, which showed strong magnetic property and made the adsorbents easily collected by external magnet. The amounts of the anionic dyes were captured on NiFe-LDO surface more than that on NiFe-LDH surface due to the larger surface area (68 m2/g for NiFe-LDO and 50 m2/g for NiFe-LDH). The maximum adsorption capacity of NiFe-LDO was in the range of 256–313 mg/g and 244–300 mg/g for eliminating the anionic dyes in single and multiple dye solution, respectively. The chemical adsorption affinity of the anionic dyes on the positive-charge surface of NiFe-LDO increased as follows: methyl orange<alizarin red S<orange II<Congo red. This work shows that NiFe-LDO is an efficient and cost-effective adsorbent for eliminating multiple anionic dyes and reusing for several times.

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References

  1. A. B. Pandit and J. K. Kumar, Annu. Rev. Chem. Biomol. Eng., 6, 217 (2015).

    Article  CAS  PubMed  Google Scholar 

  2. B. Petrie, R. Barden and B. Kasprzyk-Hordern, Water Res., 72, 3 (2015).

    Article  CAS  PubMed  Google Scholar 

  3. M. T. Yagub, T. K. Sen, S. Afroze and H. M. Ang, Adv. Colloid Interface Sci., 209, 172 (2014).

    Article  CAS  PubMed  Google Scholar 

  4. A. Tkaczyk, K. Mitrowska and A. Posyniak, Sci. Total Environ., 717, 137222 (2020).

    Article  CAS  PubMed  Google Scholar 

  5. V. Katheresan, J. Kansedo and S. Y. Lau, J. Environ. Chem. Eng., 6, 4676 (2018).

    Article  CAS  Google Scholar 

  6. S. Intachai, T. Nakato and N. Khaorapapong, Appl. Clay Sci., 201, 105927 (2021).

    Article  CAS  Google Scholar 

  7. N. Li, M. Zheng, X. Chang, G. Ji, H. Lu, L. Xue, L. Pan and J. Cao, J. Solid State Chem., 184, 953 (2011).

    Article  CAS  Google Scholar 

  8. K. A. Krishnan, K. Ajmal, A. K. Faisal and T. M. Liji, Sep. Sci. Technol., 50, 1147 (2015).

    Article  Google Scholar 

  9. V. V. Dev, G. Baburaj, S. Antony, V. Arun and K. A. Krishnan, J. Clean. Prod., 255, 120309 (2020).

    Article  CAS  Google Scholar 

  10. Q. Wang, L. Lei, F. Wang, C. Chen, X. Kang, C. Wang, J. Zhao, Q. Yang and Z. Chen, J. Solid State Chem., 292, 121656 (2020).

    Article  CAS  Google Scholar 

  11. C. Huang, B. Cai, L. Zhang, C. Zhang and H. Pan, J. Solid State Chem., 297, 122030 (2021).

    Article  CAS  Google Scholar 

  12. J.-Q. Jiang and S.M. Ashekuzzaman, Curr. Opin. Chem. Eng., 1, 191 (2012).

    Article  CAS  Google Scholar 

  13. S. G. Intasa-ard, K. J. Imwiset, S. Bureekaew and M. Ogawa, Dalton Trans., 47, 2896, (2018).

    Article  CAS  PubMed  Google Scholar 

  14. L. Mohapatra and K. Parida, J. Mater. Chem. A., 4, 10744 (2016).

    Article  CAS  Google Scholar 

  15. G. Rathee, A. Awasthi, D. Sood, R. Tomar, V. Tomar and R. Chandra, Sci. Rep., 9, 16225 (2019).

    Article  PubMed  PubMed Central  Google Scholar 

  16. H. Sun, Y.-J. Heo, J.-H. Park, K. Y. Rhee and S.-J. Park, Nanotechnol. Rev., 9, 1381 (2020).

    Article  CAS  Google Scholar 

  17. L. Gao, Q. Li, X. Hu, X. Wang, H. Song, L. Yan and H. Xiao, Appl. Clay Sci., 126, 299 (2016).

    Article  CAS  Google Scholar 

  18. G. Di, Z. Zhu, H. Zhang, J. Zhu, H. Lu, W. Zhang, Y. Qiu, L. Zhu and S. Küppers, Chem. Eng. J., 328, 141 (2017).

    Article  CAS  Google Scholar 

  19. R. Elmoubarki, F. Z. Mahjoubi, A. Elhalil, H. Tounsadi, M. Abdennouri, M. Sadiq, S. Qourzal, A. Zouhri and N. Barka, J. Mater. Res. Technol., 6, 271 (2017).

    Article  CAS  Google Scholar 

  20. M. Hu, X. Yan, X. Hu, R. Feng and M. Zhou, Colloids Surf. A: Physicochem. Eng. Asp., 540, 207 (2018).

    Article  CAS  Google Scholar 

  21. F. Khodam, H. R. Amani-Ghadim, S. Aber, A. R. Amani-Ghadim and I. Ahadzadeh, J. Ind. Eng. Chem., 68, 311 (2018).

    Article  CAS  Google Scholar 

  22. Z. Bai, C. Hu, H. Liu and J. Qu, J. Colloid Interface Sci., 539, 146 (2019).

    Article  CAS  PubMed  Google Scholar 

  23. C. Lei, M. Pi, P. Kuang, Y. Guo and F. Zhang, J. Colloid Interface Sci., 496, 158 (2017).

    Article  CAS  PubMed  Google Scholar 

  24. M. Zubair, N. Jarrah, S. A. Manzar, M. Al-Harthi, M. Daud, N. D. Mu’azu and S. A. Haladu, J. Mol. Liq., 230, 344 (2017).

    Article  CAS  Google Scholar 

  25. A. P. Teepakakorn, T. Yamaguchi and M. Ogawa, Chem. Lett., 48, 398 (2019).

    Article  CAS  Google Scholar 

  26. M. Zubair, M. Daud, G. McKay, F. Shehzad and M. A. Al-Harthi, Appl. Clay Sci., 143, 279 (2017).

    Article  CAS  Google Scholar 

  27. J. Tang, B. Mu, L. Zong and A. Wang, J. Clean. Prod., 172, 673 (2018).

    Article  CAS  Google Scholar 

  28. Y. Lu, B. Jiang, L. Fang, F. Ling, J. Gao, F. Wu and X. Zhang, Chemosphere, 152, 415 (2016).

    Article  CAS  PubMed  Google Scholar 

  29. D. B. Jiang, C. Jing, Y. Yuan, L. Feng, X. Liu, F. Dong, B. Dong and Y. Zhang, J. Colloid Interface Sci., 540, 398 (2019).

    Article  CAS  PubMed  Google Scholar 

  30. Y. M. Xia, Z. M. He, J. B. Su, B. Tang, K. J. Hu, Y. L. Lu, S. P. Sun and Z. P. Li, RSC Adv., 8, 4284 (2018).

    Article  CAS  Google Scholar 

  31. G. Zhao, C. Li, X. Wu, J. Yu, X. Jiang, W. Hu and F. Jiao, Appl. Surf. Sci., 434, 251 (2018).

    Article  CAS  Google Scholar 

  32. R. Vinayagam, S. Pai, G. Murugesan, T. Varadavenkatesan, S. Narayanasamy and R. Selvaraj, Chemosphere, 286, 131938 (2022).

    Article  CAS  PubMed  Google Scholar 

  33. S. Nayak and K. M. Parida, Sci. Rep., 9, 2458 (2019).

    Article  PubMed  PubMed Central  Google Scholar 

  34. C. Suppaso, N. Pongkan, S. Intachai, M. Ogawa and N. Khaorapapong, Appl. Clay Sci., 213, 106115 (2021).

    Article  CAS  Google Scholar 

  35. Y. Jia, L. Ding, P. Ren, M. Zhong, J. Ma and X. Fan, J. Chem. Eng. Data, 65, 725 (2020).

    Article  CAS  Google Scholar 

  36. R. Shabbir, A. Gu, J. Chen, M. M. Khan, P. Wang, Y. Jiao, Z. Zhang, Y. Liu and Y. Yang, Int. J. Environ. Anal. Chem., 9, 105197 (2021).

    Google Scholar 

  37. A. Khan, A. Naeem, T. Mahmood, B. Ahmad, Z. Ahmad, M. Farooq and T. Saeed, Int. J. Environ. Sci. Technol., 19, 2515 (2022).

    Article  CAS  Google Scholar 

  38. C. W. Chiu, Y. L. Liao and J. J. Lin, Ind. Eng. Chem. Res., 51, 581 (2012).

    Article  CAS  Google Scholar 

  39. V. Vimonses, S. Lei, B. Jin, C. W. K. Chow and C. Saint, Chem. Eng. J., 148, 354 (2009).

    Article  CAS  Google Scholar 

  40. R. Selvaraj, S. Pai, G. Murugesan, S. Pandey, R. Bhole, D. Gonsalves, T. Varadavenkatesan and R. Vinayagam, Appl. Nanosci., 11, 2227 (2021).

    Article  CAS  Google Scholar 

  41. T. Varadavenkatesan, S. Pai, R. Vinayagam and R. Selvaraj, Mater. Chem. Phys., 272, 125017 (2021).

    Article  CAS  Google Scholar 

  42. H. Palza, K. Delgado and J. Govan, Appl. Clay Sci., 183, 105350 (2019).

    Article  CAS  Google Scholar 

  43. B. Sarkar, Y. Xi, M. Megharaj and R. Naidu, Appl. Clay Sci., 51, 370 (2011).

    Article  CAS  Google Scholar 

  44. A. Tămaş, I. Cozma, L. Cocheci, L. Lupa and G. Rusu, Front. Chem., 8, 57353 (2020).

    Article  Google Scholar 

  45. X. Mi, G. Li, W. Zhu and L. Liu, J. Chem., 2016, 8457030 (2016).

    Article  Google Scholar 

  46. L. EL Mersly, E.M. El Mouchtari, E.M. Moujahid, C. Forano, M. E. Haddad, S. Briche, T. A. Alaoui and S. Rafqah, J. Sci.: Adv. Mater. Devices, 6, 118 (2021).

    CAS  Google Scholar 

  47. M. Roosta, M. Ghaedi and M. Mohammadi, Powder Technol., 267, 134 (2014).

    Article  CAS  Google Scholar 

  48. Z. Zhang, H. Chen, W. Wu, W. Pang and G. Yan, Bioresour. Technol., 293, 122100 (2019).

    Article  CAS  PubMed  Google Scholar 

  49. F. Fu, Z. Gao, L. Gao and D. Li, Ind. Eng. Chem. Res., 50, 9712 (2011).

    Article  CAS  Google Scholar 

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Funding

This project is funded by National Research Council of Thailand, Thailand. We sincerely acknowledge the scientific instrument support from Department of Chemistry, Faculty of Science, Thaksin University, and Department of Chemistry, Faculty of Science, Khon Kaen University, as well as Center for Innovation in Chemistry: Postgraduate Education and Research Program in Chemistry (PERCH-CIC), Commission on Higher Education, Ministry of Higher Education, Science, Research and Innovation.

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Authors and Affiliations

  1. Department of Chemistry, Faculty of Science, Thaksin University, Phatthalung, 93210, Thailand

    Sonchai Intachai, Pornnapa Tongchoo & Panita Sumanatrakul

  2. Materials Chemistry Research Center, Department of Chemistry and Center of Excellence for Innovation in Chemistry, Faculty of Science, Khon Kaen University, Khon Kaen, 40002, Thailand

    Prakaidao Pankam & Nithima Khaorapapong

Authors
  1. Sonchai Intachai
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  2. Pornnapa Tongchoo
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  3. Panita Sumanatrakul
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  4. Prakaidao Pankam
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  5. Nithima Khaorapapong
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Contributions

Sonchai Intachai supervised the research, analyzed and characterized the data, and took the lead in writing, editing the manuscript. Sonchai Intachai, Pornnapa Tongchoo and Prakaidao Pankam have carried out the experiments. Sonchai Intachai, Panita Sumanatrakul and Nithima Khaorapapong contributed to the interpretation of the results and revision of the manuscript.

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Correspondence to Sonchai Intachai.

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Intachai, S., Tongchoo, P., Sumanatrakul, P. et al. Efficient and practical adsorption of mixed anionic dyes in aqueous solution by magnetic NiFe-layered double oxide. Korean J. Chem. Eng. 39, 2675–2684 (2022). https://doi.org/10.1007/s11814-022-1099-y

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  • DOI: https://doi.org/10.1007/s11814-022-1099-y

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