Skip to main content
Log in

Removal of Acid Red G dye from aqueous solutions by adsorption to MCM-41-layered double hydroxides composite

  • Environmental Engineering
  • Published:
Korean Journal of Chemical Engineering Aims and scope Submit manuscript

Abstract

MCM-41 supported layered double hydroxides (LDH) composite materials (ML) were synthesized and studied for removal of Acid Red G (ARG), an anionic dye, with the adsorption method. ML was prepared using in situ synthesis procedure for the low supersaturation coprecipitation method, and ML10 and ML20 presented promising application towards ARG dye adsorption capacity in industrial wastewater. Powder samples were characterized by Xray diffraction, FTIR spectroscopy, scanning electron microscopy and energy dispersive spectrometry. The effects of different reaction time, initial solution pH and temperature on the dye adsorption capacity were investigated. Adsorption process was well described by pseudo-second-order kinetic model and Langmuir isotherm model. The fitting curves showed that ML10 and ML20 had higher adsorption rates and maintained a certain theoretical saturated adsorption capacity (92.19807mg/g and 96.41947mg/g, respectively) compared with LDH.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  1. B. Bi, L. Xu, B. Xu and X. Liu, Appl. Clay Sci., 54, 242 (2011).

    Article  CAS  Google Scholar 

  2. L. El Gaini, M. Lakraimi, E. Sebbar, A. Meghea and M. Bakasse, J. Hazard. Mater., 161, 627 (2009).

    Article  CAS  Google Scholar 

  3. A. K. Mittal and S. K. Gupta, Water Sci. Technol., 34, 81 (1996).

    CAS  Google Scholar 

  4. R.M.M. dos Santos, R.G.L. Gonçalves, V. R.L. Constantino, L.M. da Costa, L. H. M. da Silva, J. Tronto and F. G. Pinto, Appl. Clay Sci., 80, 189 (2013).

    Article  Google Scholar 

  5. D. Chebli, A. Bouguettoucha, A. Reffas, C. Tiar, M. Boutahala, H. Gulyas and A. Amrane, Desalination Water Treat., 57, 22061 (2016).

    Article  CAS  Google Scholar 

  6. V.M. Correia, T. Stephenson and S. J. Judd, Environ. Technol., 15, 917 (1994).

    Article  CAS  Google Scholar 

  7. R. Shan, L. Yan, Y. Yang, K. Yang, S. Yu, H. Yu, B. Zhu and B. Du, J. Ind. Eng. Chem., 21, 561 (2015).

    Article  CAS  Google Scholar 

  8. M.A. Kamboh, I.B. Solangi, S.T.H. Sherazi and S. Memon, J. Hazard. Mater., 186, 651 (2011).

    Article  CAS  Google Scholar 

  9. F. Bildik, G.T. Turan, G. Barim and B. F. Senkal, Sep. Sci. Technol., 49, 1700 (2014).

    Article  CAS  Google Scholar 

  10. N. Jovic-Jovicic, A. Milutinovic-Nikolic, I. Grzetic and D. Jovanovic, Chem. Eng. Technol., 31, 567 (2008).

    Article  CAS  Google Scholar 

  11. D. Bombos, R. Ganea, V. Matei, C. Marinescu, A. Bodnarev, S. Mihai, T. Natu and I. Tamas, Rev. Chim., 65, 976 (2014).

    CAS  Google Scholar 

  12. M. Qiu, C. Qian, J. Xu, J. Wu and G. Wang, Desalination, 243, 286 (2009).

    Article  CAS  Google Scholar 

  13. M. H. Beyki, H. Alijani and M. H. Ghasemi, Desalination Water Treat., 57, 20565 (2016).

    Article  CAS  Google Scholar 

  14. S.V. Mohan, N. C. Rao and J. Karthikeyan, J. Hazard. Mater., 90, 189 (2002).

    Article  Google Scholar 

  15. P. Janos, H. Buchtova and M. Ryznarova, Water Res., 37, 4938 (2003).

    Article  CAS  Google Scholar 

  16. R. Lafi, K. Charradi, M. A. Djebbi, A. Ben Haj Amara and A. Hafiane, Adv. Powder Technol., 27, 232 (2016).

    Article  CAS  Google Scholar 

  17. G. Bayramoglu, A. Akbulut, G. Liman and M.Y. Arica, Chem. Eng. Res. Des., 124, 85 (2017).

    Article  CAS  Google Scholar 

  18. K. Parida and J. Das, J. Mol. Catal. Chem., 151, 185 (2000).

    Article  CAS  Google Scholar 

  19. H. F.W. Taylor, Mineral. Mag., 39 (1973).

    Google Scholar 

  20. F. Jiao, J. Yu, H. Song, X. Jiang, H. Yang, S. Shi, X. Chen and W. Yang, Appl. Clay Sci., 101, 30 (2014).

    Article  CAS  Google Scholar 

  21. Z. Jia, S. Li, J. Liu, Q. Qin and R. Zhu, Bull. Mater. Sci., 38, 1757 (2015).

    Article  CAS  Google Scholar 

  22. M. Zhang, Q. Yao, C. Lu, Z. Li and W. Wang, ACS Appl. Mater. Interfaces, 6, 20225 (2014).

    Article  CAS  Google Scholar 

  23. C.T. Kresge, M. E. Leonowicz, W. J. Roth, J.C. Vartuli and J. S. Beck, Nature, 359, 710 (1992).

    Article  CAS  Google Scholar 

  24. G. Bayramoglu and M.Y. Arica, Micropor. Mesopor. Mater., 226, 117 (2016).

    Article  CAS  Google Scholar 

  25. T.A. Arica, E. Ayas and M.Y. Arica, Micropor. Mesopor. Mater., 243, 164 (2017).

    Article  CAS  Google Scholar 

  26. W. Lin, Q. Cai, W. Pang, Y. Yue and B. Zou, Micropor. Mesopor. Mater., 33, 187 (1999).

    Article  CAS  Google Scholar 

  27. L.K.G. Bhatta, S. Subramanyam, M.D. Chengala, U.M. Bhatta and K. Venkatesh, Ind. Eng. Chem. Res., 54, 10876 (2015).

    Article  CAS  Google Scholar 

  28. D. S. Tong, M. Liu, L. Li, C. X. Lin, W. H. Yu, Z. P. Xu and C.H. Zhou, Appl. Clay Sci., 70, 1 (2012).

    Article  CAS  Google Scholar 

  29. G. Darmograi, B. Prelot, G. Layrac, D. Tichit, G. Martin-Gassin, F. Salles and J. Zajac, J. Phys. Chem. C, 119, 23388 (2015).

    Article  CAS  Google Scholar 

  30. S. Wang, Z. Li and C. Lu, J. Colloid Interface Sci., 458, 315 (2015).

    Article  CAS  Google Scholar 

  31. A.K. Kushwaha, N. Gupta and M. C. Chattopadhyaya, Desalination Water Treat., 52, 4527 (2014).

    Article  CAS  Google Scholar 

  32. R. Extremera, I. Pavlovic, M.R. Pérez and C. Barriga, Chem. Eng., J. 213, 392 (2012).

    Article  CAS  Google Scholar 

  33. W.H. Zhang, X.D. Guo, J. He and Z.Y. Qian, J. Eur. Ceram. Soc., 28, 1623 (2008).

    Article  CAS  Google Scholar 

  34. J.M. Lee, Y. J. Min, K.B. Lee, S.G. Jeon, J.G. Na and H. J. Ryu, Langmuir, 26, 18788 (2010).

    Article  CAS  Google Scholar 

  35. Y.-S. Ho, J. Hazard. Mater., 136, 681 (2006).

    Article  CAS  Google Scholar 

  36. A. Özcan, E.M. Öncü and A. S. Özcan, Colloids Surf. Physicochem. Eng. Asp., 277, 90 (2006).

    Article  Google Scholar 

  37. N. Buvaneswari and C. Kannan, J. Hazard. Mater., 189, 294 (2011).

    Article  CAS  Google Scholar 

  38. T. Xue, Y. Gao, Z. Zhang, A. Umar, X. Yan, X. Zhang, Z. Guo and Q. Wang, J. Alloys Compd., 587, 99 (2014).

    Article  CAS  Google Scholar 

  39. I.M. Ahmed and M.S. Gasser, Appl. Surf. Sci., 259, 650 (2012).

    Article  CAS  Google Scholar 

  40. F. P. de Sá, B. N. Cunha and L. M. Nunes, Chem. Eng. J., 215, 122 (2013).

    Google Scholar 

  41. J. Liu, X. Li, J. Luo, C. Duan, H. Hu and G. Qian, Chem. Eng. J., 242, 187 (2014).

    Article  CAS  Google Scholar 

  42. H.M. F. Freundlich, Z. Phys. Chem. Leipz., 57A, 385 (1906).

    Google Scholar 

  43. I. Langmuir, J. Am. Chem. Soc., 38, 2221 (1916).

    Article  CAS  Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Tao Du.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Wang, Y., Du, T., Zhou, L. et al. Removal of Acid Red G dye from aqueous solutions by adsorption to MCM-41-layered double hydroxides composite. Korean J. Chem. Eng. 35, 709–716 (2018). https://doi.org/10.1007/s11814-017-0327-3

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s11814-017-0327-3

Keywords

Navigation