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Volumetric properties of supercritical carbon dioxide from volume-translated and modified Peng-Robinson equations of state

  • Separation Technology, Thermodynamics
  • Published:
Korean Journal of Chemical Engineering Aims and scope Submit manuscript

Abstract

Following three well-established approaches, different modifications have been proposed that significantly improve the Peng-Robinson EOS’s predictions of the volumetric properties of carbon dioxide in the supercritical region. By making use of 5301 experimental PVT data points of supercritical carbon dioxide (SC-CO2), three models have been developed based on the volume-translation concept, modification of the alpha function of the attractive term of the Peng-Robinson EOS and the addition of a third translation parameter to the EOS. The experimental data considered encompass a wide temperature and pressure range of 304.35-1,273.15 K and 7.38-800.00MPa, respectively. According to the results from several graphical and statistical analyses, the proposed models can reliably be employed for prediction and representation of the volumetric properties of SC-CO2 with AARDs below 1.3%. Comparisons have also been made with the modified Redlich-Kwong EOS as well as the standard reference multiparameter EOS developed by Span and Wagner, demonstrating the comparable accuracy of the proposed models, while offering notably simpler mathematical formulation.

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Authors and Affiliations

  1. Young Researchers and Elite Club, Shiraz Branch, Islamic Azad University, Shiraz, Iran

    Javad Hekayati

  2. Chemical Engineering, Oil and Gas Department, Shiraz University of Technology, Shiraz, Fars, Iran

    Aliakbar Roosta & Jafar Javanmardi

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  1. Javad Hekayati
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Correspondence to Aliakbar Roosta.

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Hekayati, J., Roosta, A. & Javanmardi, J. Volumetric properties of supercritical carbon dioxide from volume-translated and modified Peng-Robinson equations of state. Korean J. Chem. Eng. 33, 3231–3244 (2016). https://doi.org/10.1007/s11814-016-0176-5

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