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Enhanced Mechanical Properties and Corrosion Resistance by Minor Gd Alloying with a Hot-Extruded Mg Alloy

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Abstract

The microstructure, mechanical properties, and corrosion resistance to simulated body fluid solution behavior of as-extruded Mg-1.8Zn-0.5Zr alloys with different Gd additions are investigated. It is found that dynamic recrystallization occurs in the alloys during extrusion and the grain size gradually decreases with Gd alloying. The mechanical properties and corrosion resistance to simulated body fluid of the investigated alloys enhance firstly and then weaken with the increase in Gd content. The results reveal that the Mg-1.8Zn-0.5Zr with a 1.5 wt.% Gd addition has optimized mechanical properties and corrosion resistance. A three-stage corrosion mechanism, including sequential stages from hydroxidation, phosphatization and hydroxidation, to formation-dissolution dynamic equilibrium, is proposed through electrochemical measurements and corroded surface analyses. This study reveals the extruded Mg-1.8Zn-0.5Zr-1.5Gd alloy can be regarded as a potential candidate for using as biodegradable magnesium implants.

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Acknowledgments

This work was financially supported by the Education Department of Henan Province (20A430010), National Natural Science Foundation of China (U1804146, 52111530068), Foreign Experts and Introduction Project of Henan Province (HNGD2020009) and Academy of Finland Grant #311934. The Center for Material Analysis, University of Oulu, Finland, is acknowledged for XPS measurements.

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  1. School of Materials Science and Engineering, Henan University of Science and Technology, Luoyang, 471023, Henan, China

    Huai Yao, Yi Xiong & Marko Huttula

  2. Provincial and Ministerial Co-construction of Collaborative Innovation Center for Non-ferrous Metal New Materials and Advanced Processing Technology, Luoyang, 471023, Henan, China

    Huai Yao

  3. Nano and Molecular Systems Research Unit, Centre for Advanced Steels Research, University of Oulu, FI-90014, Oulu, Finland

    Shubo Wang, Harishchandra Singh, Marko Huttula & Wei Cao

  4. School of Physics and Electronic Engineering, Jiangsu Normal University, Xuzhou, 221116, Jiangsu, China

    Xinying Shi

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Yao, H., Wang, S., Xiong, Y. et al. Enhanced Mechanical Properties and Corrosion Resistance by Minor Gd Alloying with a Hot-Extruded Mg Alloy. J. of Materi Eng and Perform 31, 9997–10009 (2022). https://doi.org/10.1007/s11665-022-07024-8

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