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Critical Behavior of Ni-doped La0.7Sr0.3MnO3 Ceramics

  • 5th International Conference of Asian Union of Magnetics Societies
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Abstract

The effect of Ni substitution on the magnetic properties and the critical behavior of La0.7Sr0.3Mn1−xNixO3 compounds, which were prepared by the solid-state reaction method has been investigated. Based on our investigations of the temperature and the magnetic field dependences of magnetization M(T, H) data, it is shown that the Curie temperature (\( T_{\rm{C}}\)) of La0.7Sr0.3Mn1−xNixO3 compounds will be shifted toward room temperature with increasing Ni concentration (x), \(T_{\rm{C}}\) = 359–307 K for x = 0.0–0.1. By using the modified Arrott plots and the Kouvel–Fisher methods together with \(M(H,T)\) data in the vicinity of the ferromagnetic (FM)–paramagnetic phase transition, the critical exponents (β, γ, and δ) have been determined. Our results show the existence of a short-range FM order in the undoped sample (x = 0). The values of β, γ, and δ will be shifted gradually toward those of the mean-field theory when x increases, suggesting that the long-range FM order is favored in Ni-doped samples. The results calculated on the effective exponents of \(\beta_{\rm{eff}} (\varepsilon )\) and \(\gamma_{\rm{eff}} (\varepsilon )\) in the asymptotic region indicate the existence of a magnetic disorder in all the samples.

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Acknowledgments

This research was supported by the Institute of Materials Science, VAST, Vietnam under Grant No. CSCL01.18, the Vietnam Academy of Science and Technology under the Program of development in the field of physics by 2020 (Grant No. VAST.CTVL.01/17-20), and by Vietnam National Foundation for Science and Technology Development (NAFOSTED) under Grant No. 103.02-2017.57.

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Authors and Affiliations

  1. Department of Physics, Chungbuk National University, Cheongju, 28644, South Korea

    Tran Dang Thanh, Pham Duc Huyen Yen, Kieu Xuan Hau & Seong Cho Yu

  2. Institute of Materials Science, Vietnam Academy of Science and Technology, 18-Hoang Quoc Viet, Hanoi, Vietnam

    Tran Dang Thanh & Nguyen Thi Dung

  3. Graduate University of Science and Technology, Vietnam Academy of Science and Technology, 18-Hoang Quoc Viet, Hanoi, Viet Nam

    Tran Dang Thanh & Nguyen Thi Dung

  4. Department of Engineering and Technology, Hong Duc University, Thanh Hoa, Vietnam

    Le Vi Nhan, Le Thi Huong & Le Viet Bau

  5. Department of Physics, Hanoi University of Science, Vietnam National University, Hanoi, Vietnam

    Le Thi Anh Thu & Bach Thanh Cong

  6. Institute of Physics, Vietnam Academy of Science and Technology, 18-Hoang Quoc Viet, Hanoi, Viet Nam

    Nguyen Xuan Nghia & Le Hong Khiem

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  1. Tran Dang Thanh
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  2. Pham Duc Huyen Yen
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Correspondence to Tran Dang Thanh or Seong Cho Yu.

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Thanh, T.D., Yen, P.D.H., Hau, K.X. et al. Critical Behavior of Ni-doped La0.7Sr0.3MnO3 Ceramics. J. Electron. Mater. 48, 1353–1362 (2019). https://doi.org/10.1007/s11664-018-06909-6

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  • DOI: https://doi.org/10.1007/s11664-018-06909-6

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