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The Structure, Dielectric and Energy Storage Properties of Strontium Barium Niobate-Based Glass–Ceramics Doped with La2O3

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Abstract

In this work, the effect of La2O3 content on the phase evolution, microstructure, dielectric properties and energy storage properties of the strontium barium niobate (SBN)-based glass–ceramics were studied. The results show that the La3+ is easily incorporated into the tetragonal tungsten bronze structured phase, and La2O3 doped into the BSN-glass–ceramics, as a grain growth inhibitor, can have an evident effect on the grain size reduction and crystallization. The microstructure of the SBN-glass–ceramics becomes denser and more uniform with increasing La2O3 content. The remanent polarization of all samples is extremely low. The dielectric constant of the SBN-glass–ceramics obviously is decreased, while the breakdown strength is increased with the increment of La2O3 content. When La2O3 content in the SBN-glass–ceramics is 0.2 mol.%, the theoretical energy storage density is at the maximal level of 7.2 J/cm3. In addition, the energy discharging efficiency and discharging speed of the SBN-glass–ceramics with different La2O3 content were evaluated. With La2O3 content increasing, the energy discharging efficiency gradually increased.

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Authors and Affiliations

  1. Key Laboratory of Advanced Civil Engineering Materials of Ministry of Education, Functional Materials Research Laboratory, School of Materials Science and Engineering, Tongji University, 4800 Caoan Road, Shanghai, 201804, China

    Shaomei Xiu, Shi Xiao, Bo Shen & Jiwei Zhai

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  1. Shaomei Xiu
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  2. Shi Xiao
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  3. Bo Shen
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  4. Jiwei Zhai
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Correspondence to Bo Shen.

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Xiu, S., Xiao, S., Shen, B. et al. The Structure, Dielectric and Energy Storage Properties of Strontium Barium Niobate-Based Glass–Ceramics Doped with La2O3 . J. Electron. Mater. 46, 4557–4561 (2017). https://doi.org/10.1007/s11664-017-5422-z

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  • DOI: https://doi.org/10.1007/s11664-017-5422-z

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