Abstract
Source characterization of heavy metals is prerequisite to assessing their potential contamination pathways and environmental risks, based on which pollution control and environmental remediation measures can be properly targeted. In the present study, recent progress in methodologies of source identification of heavy metals in solid waste are summarized. The key scientific concerns related to these methodologies based on the total contents, chemical speciation, isotopic composition, and single-particle signature are also discussed. Finally, prospective research with regard to source identification of heavy metals in solid waste is discussed according to current research conditions and progress.
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References
Merdy P, Huclier S, Koopal L K. Modeling metal-particle interactions with an emphasis on natural organic matter. Environ Sci Technol, 2006, 40: 7459–7466
Weiss D J, Rehkämper M, Schoenberg R, et al. Application of nontraditional stable-isotope systems to the study of sources and fate of metals in the environment. Environ Sci Technol, 2008, 42: 655–664
Zhang H. Source and Fate of Heavy Metals in Municipal Solid Waste Incineration Residues (in Chinese). Dissertation for the Doctoral Degree. Shanghai: Tongji University, 2006. 29–50
Chang S H, Wang K S, Chang H F, et al. Comparison of source identification of metals in road-dust and soil. Soil Sediment Contam, 2009, 18: 669–683
Kartal S, Aydin Z, Tokalioğlu S. Fractionation of metals in street sediment samples by using the BCR sequential extraction procedure and multivariate statistical elucidation of the data. J Hazard Mater, 2006, 132: 80–89
Davis H T, Aelion C M, McDermott S, et al. Identifying natural and anthropogenic sources of metals in urban and rural soils using GIS-based data, PCA, and spatial interpolation. Environ Pollut, 2009, 157: 2378–2385
Tang W, Shan B, Zhang H, et al. Heavy metal sources and associated risk in response to agricultural intensification in the estuarine sediments of Chaohu Lake Valley, East China. J Hazard Mater, 2010, 176: 945–951
Shikazono N, Tatewaki K, Mohiuddin K M, et al. Sources, spatial variation, and speciation of heavy metals in sediments of the Tamagawa River in Central Japan. Environ Geochem Health, 2012, 34: 13–26
Jacobson A R, Dousset S, Andreux F, et al. Electron microprobe and synchrotron X-ray fluorescence mapping of the heterogeneous distribution of copper in high-copper vineyard soils. Environ Sci Technol, 2007, 41: 6343–6349
Carignan J, Libourel G, Cloquet C, et al. Lead isotopic composition of fly ash and flue gas residues from municipal solid waste combustors in France: Implications for atmospheric lead source tracing. Environ Sci Technol, 2005, 39: 2018–2024
Cheng H, Hu Y. Lead (Pb) isotopic fingerprinting and its applications in lead pollution studies in China: A review. Environ Pollut, 2010, 158: 1134–1146
Hass A, Fine P. Sequential selective extraction procedures for the study of heavy metals in soils, sediment, and waste materials-a critical review. Crit Rev Environ Sci Technol, 2010, 40: 365–399
Linge K L. Methods for investigating trace element binding in sediments. Crit Rev Environ Sci Technol, 2008, 38: 165–196
Scheinost A C, Kretzschmar R, Pfister S. Combining selective sequential extractions, X-ray absorption spectroscopy, and principal component analysis for quantitative zinc speciation in soil. Environ Sci Technol, 2002, 35: 5021–5028
Zhang H, He P J, Lü F, et al. A review on the methods for investigating heavy metal speciation in environmental chemistry (in Chinese). Environ Chem, 2011, 30: 130–137
Terzano R, Spagnuolo M, Vekemans B, et al. Assessing the origin and fate of Cr, Ni, Cu, Zn, Pb, and V in industrial polluted soil by combined microspectroscopic techniques and bulk extraction methods. Environ Sci Technol, 2007, 41: 6762–6769
Arai T, Ikemoto T, Hokura A, et al. Chemical forms of mercury and cadmium accumulated in marine mammals and seabirds as determined by XAFS analysis. Environ Sci Technol, 2004, 38: 6468–6474
Sheng G, Yang S, Sheng J, et al. Macroscopic and microscopic investigation of Ni(II) sequestration on diatomite by batch, XPS, and EXAFS techniques. Environ Sci Technol, 2011, 45: 7718–7726
Tian S, Yu M, Wang W, et al. Investigating the speciation of copper in secondary fly ash by X-ray absorption spectroscopy. Environ Sci Technol, 2009, 43: 9084–9088
Wu F, Zheng J, Liao H, et al. Anomalous plutonium isotopic ratios in sediments of Lake Qinghai from the Qinghai-Tibetan Plateau, China. Environ Sci Technol, 2011, 45: 9188–9194
Cloquet C, Carignan J, Libourel G, et al. Tracing source pollution in soils using cadmium and lead isotopes. Environ Sci Technol, 2006, 40: 2525–2530
Guelke M, Blanckenburg F V. Fractionation of stable iron isotopes in higher plants. Environ Sci Technol, 2007, 41: 1896–1901
Scaife B. Lead isotope ratios for ores from Italy. http://www.brettscaife.net/lead/data/meditaly.html
Fernandez C, Monna F, Labanowski J, et al. Anthropogenic lead distribution in soils under arable land and permanent grassland estimated by Pb isotopic compositions. Environ Pollut, 2008, 156: 1083–1091
Geage M L, Stille P, Millet M, et al. REE characteristics and Pb, Sr and Nd isotopic compositions of steel plant emissions. Sci Total Environ, 2007, 373: 404–419
Cloquet C, Carignan J, Libourel G. Atmospheric pollutant dispersion around an urban area using trace metal concentrations and Pb isotopic compositions in epiphytic lichens. Atmos Environ, 2006, 40: 574–587
Cloquet C, Carignan J, Libourel G. Isotopic composition of Zn and Pb atmospheric depositions in an urban/periurban area of northeastern France. Environ Sci Technol, 2006, 40: 6594–6600
Dolgopolova A, Weiss D J, Seltmann R, et al. Use of isotope ratios to assess sources of Pb and Zn dispersed in the environment during mining and ore processing within the Orlovka-Spokoinoe mining site (Russia). Appl Geochem, 2006, 21: 563–579
Luo X S, Yu S, Li X D. Distribution, availability, and sources of trace metals in different particle size fractions of urban soils in Hong Kong: Implications for assessing the risk to human health. Environ Pollut, 2011, 159: 1317–1326
Jouvin D, Louvat P, Juillot F, et al. Zinc isotopic fractionation: Why organic matters. Environ Sci Technol, 2009, 43: 5747–5754
Vitòria L, Otero N, Soler A, et al. Fertilizer characterization: isotopic data (N, S, O, C, and Sr). Environ Sci Technol, 2004, 38: 3254–3262
Wei Y M, Li Y, Guo B L. Research of Analytical Approaches to Trace Pollution Origin of Plant-derived Foods (in Chinese). Beijing: Science Press, 2010. 10–12
Sun G X, Wang X J, Hu Q H. Using stable lead isotopes to trace heavy metal contamination sources in sediments of Xiangjiang and Lishui Rivers in China. Environ Pollut, 2011, 159: 3406–3410
Ettler V, Mihaljevič M, Šebek O, et al. Geochemical and Pb isotopic evidence for sources and dispersal of metal contamination in stream sediments from the mining and smelting district of Příbram, Czech Republic. Environ Pollut, 2006, 142: 409–417
Geagea M L, Stille P, Gauthier-Lafaye F, et al. Tracing of industrial aerosol sources in an urban environment using Pb, Sr, and Nd isotopes. Environ Sci Technol, 2008, 42: 692–698
Estrade N, Carignan J, Donard O F X. Isotope tracing of atmospheric mercury sources in an urban area of northeastern France. Environ Sci Technol, 2010, 44: 6062–6067
Donner E, Howard D L, de Jonge M D, et al. X-ray absorption and micro X-ray fluorescence spectroscopy investigation of copper and zinc speciation in biosolids. Environ Sci Technol, 2011, 45: 7249–7257
Thieme J, McNulty I, Vogt S, et al. X-ray spectromicroscopy—A tool for environmental sciences. Environ Sci Technol, 2007, 41: 6885–6889
Maclean L C W, Beauchemin S, Rasmussen P E. Lead speciation in house dust from Canadian urban homes using EXAFS, micro-XRF, and micro-XRD. Environ Sci Technol, 2011, 45: 5491–5497
Bernaus A, Gaona X, Esbrí J M, et al. Microprobe techniques for speciation analysis and geochemical characterization of mine environment: The mercury district of Almadén in Span. Environ Sci Technol, 2006, 40: 4090–4095
Punshon T, Bertsch P M, Lanzirotti A, et al. Geochemical signature of contaminated sediment remobilization revealed by spatially resolved X-ray microanalysis of annual rings of Salix nigra. Environ Sci Technol, 2003, 37: 1766–1774
Camerani M C, Somogyi A, Vekemans B, et al. Determination of the Cd-bearing phases in municipal solid waste and biomass single fly ash particles using SR-μXRF Spectroscopy. Anal Chem, 2007, 79: 6496–6506
Pinzani M C C, Somogyi A, Simionovici A S, et al. Direct determination of cadmium speciation in municipal solid waste fly ashes by synchrotron radiation induced μ-X-ray fluorescence andμ-X-ray absorption spectroscopy. Environ Sci Technol, 2002, 36: 3165–3169
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Zhang, H., Yao, Q., Zhu, Y. et al. Review of source identification methodologies for heavy metals in solid waste. Chin. Sci. Bull. 58, 162–168 (2013). https://doi.org/10.1007/s11434-012-5531-2
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DOI: https://doi.org/10.1007/s11434-012-5531-2