Abstract
Using self-flux method, we have successfully grown the parent phase of the single crystals of CaFeAsF1−x . The X-ray diffraction indicates good crystallinity. In-plane resistivity shows a bad metallic behavior with a sharp drop of resistivity at about T SDW =119 K. This anomaly is associated with the possible spin density wave (SDW) order. Interestingly near T SDW, the resistivity exhibits a cusp-like feature, which may be understood as the strong coupling effect between the electrons and the antiferromagnetic (AF) spin fluctuations. A reduction of fluorine or application of a high pressure will suppress the SDW feature and induce superconductivity. Hall effect measurements reveal a positive Hall coefficient below T SDW indicating a dominant role of the hole-like charge carriers in the parent phase. Strong magnetoresistance has been observed below T SDW suggesting multiple conduction channels of the charge carriers.
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Tao, J., Li, S., Zhu, X. et al. Growth and transport properties of CaFeAsF1−x single crystals. Sci. China Phys. Mech. Astron. 57, 632–636 (2014). https://doi.org/10.1007/s11433-014-5422-4
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DOI: https://doi.org/10.1007/s11433-014-5422-4