Abstract
Optical quantum memory is a key component of emerging quantum technologies and applications. One of the most promising protocols, far-off-resonant Raman memory, is still beset by its efficiency. Until now, the only effective method for enhancing its efficiency in experiments has been the intensity modulation method on the control field, while the experimental demonstrations still fail to meet the theoretical expectation. In this study, we experimentally demonstrate how to optimize the Raman quantum memory process using a new method called phase modulation; 52.7% total memory efficiency is realized by applying a phase modulation on the control field with a near-square intensity waveform of the control field, thereby resulting in an increase in efficiency of 13.3% compared to the best case of no phase modulation. Additionally, a hybrid method, combining the phase and intensity modulations, is demonstrated with 87.3% memory efficiency. Such high-efficiency results in 99.0% unconditional fidelity even at near single photon level. The unconditional fidelity is always higher than that of the intensity method as the input photon number of the signal increases and can still beat the nonclone limit, even at 128.1 photons/pulse. Our phase modulation method has great potential applications in quantum information processing due to the advantages of low experimental requirements but an additional degree of freedom and high performance, especially for the high speed and high photon number state manipulation.
Similar content being viewed by others
References
Ferguson K R, Beavan S E, Longdell J J, et al. Generation of light with multimode time-delayed entanglement using storage in a solid-state spin-wave quantum memory. Phys Rev Lett, 2016, 117: 020501
Bhaskar M K, Riedinger R, Machielse B, et al. Experimental demonstration of memory-enhanced quantum communication. Nature, 2020, 580: 60–64
Heshami K, England D G, Humphreys P C, et al. Quantum memories: emerging applications and recent advances. J Modern Opt, 2016, 63: 2005–2028
Reim K F, Michelberger P, Lee K C, et al. Single-photon-level quantum memory at room temperature. Phys Rev Lett, 2011, 107: 053603
Guo J, Feng X, Yang P, et al. High-performance Raman quantum memory with optimal control in room temperature atoms. Nat Commun, 2019, 10: 148
Hosseini M, Campbell G, Sparkes B M, et al. Unconditional room-temperature quantum memory. Nat Phys, 2011, 7: 794–798
Sparkes B M, Hosseini M, Cairns C, et al. Precision spectral manipulation: a demonstration using a coherent optical memory. Phys Rev X, 2012, 2: 021011
Phillips D F, Fleischhauer A, Mair A, et al. Storage of light in atomic vapor. Phys Rev Lett, 2001, 86: 783–786
Longdell J J, Fraval E, Sellars M J, et al. Stopped light with storage times greater than one second using electromagnetically induced transparency in a solid. Phys Rev Lett, 2005, 95: 063601
Honda K, Akamatsu D, Arikawa M, et al. Storage and retrieval of a squeezed vacuum. Phys Rev Lett, 2008, 100: 093601
de Riedmatten H, Afzelius M, Staudt M U, et al. A solid-state light-matter interface at the single-photon level. Nature, 2008, 456: 773–777
Afzelius M, Simon C, de Riedmatten H, et al. Multimode quantum memory based on atomic frequency combs. Phys Rev A, 2009, 79: 052329
Michelberger P S, Champion T F M, Sprague M R, et al. Interfacing GHz-bandwidth heralded single photons with a warm vapour Raman memory. New J Phys, 2015, 17: 043006
Hsiao Y F, Tsai P J, Chen H S, et al. Highly efficient coherent optical memory based on electromagnetically induced transparency. Phys Rev Lett, 2018, 120: 183602
Ma Y, Ma Y Z, Zhou Z Q, et al. One-hour coherent optical storage in an atomic frequency comb memory. Nat Commun, 2021, 12: 2381
Ding D S, Zhang W, Zhou Z Y, et al. Raman quantum memory of photonic polarized entanglement. Nat Photon, 2015, 9: 332–338
Nunn J, Reim K, Lee K C, et al. Multimode memories in atomic ensembles. Phys Rev Lett, 2008, 101: 260502
England D G, Fisher K A G, MacLean J P W, et al. Storage and retrieval of THz-bandwidth single photons using a room- temperature diamond quantum memory. Phys Rev Lett, 2015, 114: 053602
Gorshkov A V, Andre A, Lukin M D, et al. Photon storage in λ-type optically dense atomic media. II. Free-space model. Phys Rev A, 2007, 76: 033805
Zhang X, Kalachev A, Kocharovskaya O. All-optical quantum storage based on spatial chirp of the control field. Phys Rev A, 2014, 90: 052322
Minar J, Sangouard N, Afzelius M, et al. Spin-wave storage using chirped control fields in atomic frequency comb-based quantum memory. Phys Rev A, 2010, 82: 042309
Zhang X, Kalachev A, Kocharovskaya O. Quantum storage based on control-field angular scanning. Phys Rev A, 2013, 87: 013811
Kalachev A, Kocharovskaya O. Multimode cavity-assisted quantum storage via continuous phase-matching control. Phys Rev A, 2013, 88: 033846
Dabrowski M, Chrapkiewicz R, Wasilewski W. Hamiltonian design in readout from room-temperature Raman atomic memory. Opt Express, 2014, 22: 26076–26091
Kalachev A, Kocharovskaya O. Quantum storage via refractive-index control. Phys Rev A, 2011, 83: 053849
Clark J, Heshami K, Simon C. Photonic quantum memory in two-level ensembles based on modulating the refractive index in time: equivalence to gradient echo memory. Phys Rev A, 2012, 86: 013833
Gorshkov A V, Andre A, Lukin M D, et al. Photon storage in λ-type optically dense atomic media. I. Cavity model. Phys Rev A, 2007, 76: 033804
Shinbrough K, Hunt B D, Lorenz V O. Optimization of broadband λ-type quantum memory using Gaussian pulses. Phys Rev A, 2021, 103: 062418
Appel J, MacRae A, Lvovsky A I. A versatile digital GHz phase lock for external cavity diode lasers. Meas Sci Technol, 2009, 20: 055302
Zahedinejad E, Schirmer S, Sanders B C. Evolutionary algorithms for hard quantum control. Phys Rev A, 2014, 90: 032310
Yang X, Li J, Peng X. An improved differential evolution algorithm for learning high-fidelity quantum controls. Sci Bull, 2019, 64: 1402–1408
Zhang K, Guo J, Chen L Q, et al. Suppression of the four-wave-mixing background noise in a quantum memory retrieval process by channel blocking. Phys Rev A, 2014, 90: 033823
Nunn J, Munns J H D, Thomas S, et al. Theory of noise suppression in λ-type quantum memories by means of a cavity. Phys Rev A, 2017, 96: 012338
Bustard P J, England D G, Heshami K, et al. Reducing noise in a Raman quantum memory. Opt Lett, 2016, 41: 5055–5058
Thomas S E, Hird T M, Munns J H D, et al. Raman quantum memory with built-in suppression of four-wave-mixing noise. Phys Rev A, 2019, 100: 033801
Acknowledgements
This work was supported by Innovation Program for Quantum Science and Technology (Grant No. 2021ZD-0303200), Innovation Program of Shanghai Municipal Education Commission (Grant No. 202101070008E00099), National Key Research and Development Program of China (Grant No. 2016YFA0302001), National Natural Science Foundation of China (Grant Nos. 11904227, 12104161, 11654005, 11874152, 12274132, 12204303), Fellowship of China Postdoctoral Science Foundation (Grant Nos. 2020TQ0193,2021M702146), and Shanghai Municipal Science and Technology Major Project (Grant No. 2019SHZDZX01). Weiping ZHANG also acknowledges additional support from the Shanghai Talent Program.
Author information
Authors and Affiliations
Corresponding authors
Rights and permissions
About this article
Cite this article
Ming, S., Guo, J., Wu, Y. et al. Optimizing Raman quantum memory with dynamic phase. Sci. China Inf. Sci. 66, 180505 (2023). https://doi.org/10.1007/s11432-022-3614-7
Received:
Revised:
Accepted:
Published:
DOI: https://doi.org/10.1007/s11432-022-3614-7