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Aerosol printing and photonic sintering of bioresorbable zinc nanoparticle ink for transient electronics manufacturing

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Abstract

Bioresorbable electronics technology can potentially lead to revolutionary applications in healthcare, consumer electronics, and data security. This technology has been demonstrated by various functional devices. However, majority of these devices are realized by CMOS fabrication approaches involving complex and time-consuming processes that are high in cost and low in yield. Printing electronics technology represents a series of printing and post processing techniques that hold promise to make high performance bioresorbable electronics devices. But investigation of printing approaches for bioresorbable electronics is very limited. Here we demonstrate fabrication of conductive bioresorbable patterns using aerosol printing and photonic sintering approaches. Experimental results and simulation reveals that ink compositions, photonic energy, film thickness, and ventilation conditions may influence the effect of photonic sintering. A maximum conductivity of 22321.3 S/m can be achieved using 1 flash with energy of 25.88 J/cm2 with duration of 2 ms. By combining two cascaded sintering procedures using flash light and laser further improve the conductivity to 34722.2 S/m. The results indicate that aerosol printing and photonic sintering can potentially yield mass fabrication of bioresorbable electronics, leading to prevalence of printable bioresorbable technology in consumer electronics and biomedical devices.

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References

  1. 1

    Huang X, Liu Y, Cheng H, et al. Biomedical sensors: materials and designs for wireless epidermal sensors of hydration and strain. Adv Funct Mater, 2014, 24: 3845–3845

  2. 2

    Huang X, Liu Y, Hwang S W, et al. Biodegradable materials for multilayer transient printed circuit boards. Adv Mater, 2014, 26: 7371–7377

  3. 3

    Hwang S W, Tao H, Kim D H, et al. A physically transient form of silicon electronics. Science, 2012, 337: 1640–1644

  4. 4

    Hwang S W, Huang X, Seo J H, et al. Materials for bioresorbable radio frequency electronics. Adv Mater, 2013, 25: 3526–3531

  5. 5

    Dagdeviren C, Hwang S W, Su Y, et al. Transient, biocompatible electronics and energy harvesters based on ZnO. Small, 2013, 9: 3398–3404

  6. 6

    Cavusoglu T, Yavuzer R, Basterzi Y, et al. Resorbable plate-screw systems: clinical applications. Ulus Travma Acil Cerrahi Derg, 2005, 11: 43–48

  7. 7

    Farra R, Sheppard N F, Mc Cabe L, et al. First-in-human testing of a wirelessly controlled drug delivery microchip. Sci Translational Med, 2012, 4: 122ra21

  8. 8

    Lee C H, Kang S K, Salvatore G A, et al. Wireless microfluidic systems for programmed, functional transformation of transient electronic devices. Adv Funct Mater, 2015, 25: 5100–5106

  9. 9

    Kim B H, Kim J H, Persano L, et al. Dry transient electronic systems by use of materials that sublime. Adv Funct Mater, 2017, 27: 1606008

  10. 10

    Sim K, Wang X, Li Y, et al. Destructive electronics from electrochemical-mechanically triggered chemical dissolution. J Micromech Microeng, 2017, 27: 065010

  11. 11

    Lee C H, Jeong J W, Liu Y, et al. Materials and wireless microfluidic systems for electronics capable of chemical dissolution on demand. Adv Funct Mater, 2015, 25: 1338–1343

  12. 12

    Pardo D A, Jabbour G E, Peyghambarian N. Application of screen printing in the fabrication of organic light-emitting devices. Adv Mater, 2000, 12: 1249–1252

  13. 13

    Tekin E, Smith P J, Schubert U S. Inkjet printing as a deposition and patterning tool for polymers and inorganic particles. Soft Matter, 2008, 4: 703–713

  14. 14

    Gu X, Zhou Y, Gu K, et al. Roll-to-roll printed large-area all-polymer solar cells with 5% efficiency based on a low crystallinity conjugated polymer blend. Adv Energy Mater, 2017, 7: 1–13

  15. 15

    Saleh E, Zhang F, He Y, et al. 3D inkjet printing of electronics using UV conversion. Adv Mater Technol, 2017, 2: 1700134

  16. 16

    Ko S H, Pan H, Grigoropoulos C P, et al. All-inkjet-printed flexible electronics fabrication on a polymer substrate by low-temperature high-resolution selective laser sintering of metal nanoparticles. Nanotechnology, 2007, 18: 345202

  17. 17

    Yu X, Mahajan B, Shuo W, et al. Materials, mechanics, and patterning techniques for elastomer-based stretchable conductors. Micromachine, 2017, 8: 7

  18. 18

    Jones C S, Lu X, Renn M, et al. Aerosol-jet-printed, high-speed, flexible thin-film transistor made using single-walled carbon nanotube solution. Microelectron Eng, 2010, 87: 434–437

  19. 19

    Sirringhaus H, Kawase T, Friend R H, et al. High-resolution inkjet printing of all-polymer transistor circuits. Science, 2000, 290: 2123–2126

  20. 20

    Kopola P, Zimmermann B, Filipovic A, et al. Aerosol jet printed grid for ITO-free inverted organic solar cells. Sol Energy Mater Sol Cells, 2012, 107: 252–258

  21. 21

    Chen H Y, Hou J, Zhang S, et al. Polymer solar cells with enhanced open-circuit voltage and efficiency. Nat Photon, 2009, 3: 649–653

  22. 22

    Xu B L, Zhao Y, Yu L K, et al. Aerosol jet printing on radio frequency identification tag applications. Key Eng Mater, 2013, 562–565: 1417–1421

  23. 23

    van Osch T H J, Perelaer J, de Laat A W M, et al. Inkjet printing of narrow conductive tracks on untreated polymeric substrates. Adv Mater, 2008, 2: 343–345

  24. 24

    Zhao D, Liu T, Zhang M, et al. Fabrication and characterization of aerosol-jet printed strain sensors for multifunctional composite structures. Smart Mater Struct, 2012, 21: 115008

  25. 25

    Lee H H, Chou K S, Huang K C. Inkjet printing of nanosized silver colloids. Nanotechnology, 2005, 16: 2436–2441

  26. 26

    Sekine C, Tsubata Y, Yamada T, et al. Recent progress of high performance polymer OLED and OPV materials for organic printed electronics. Sci Tech Adv Mater, 2014, 15: 034203

  27. 27

    Singh M, Haverinen H M, Dhagat P, et al. Inkjet printing-process and its applications. Adv Mater, 2010, 22: 673–685

  28. 28

    Shou W, Mahajan B K, Ludwig B, et al. Low-cost manufacturing of bioresorbable conductors by evaporationcondensation-mediated laser printing and sintering of zn nanoparticles. Adv Mater, 2017, 29: 1–7

  29. 29

    Hwang S W, Kim D H, Tao H, et al. Materials and fabrication processes for transient and bioresorbable highperformance electronics. Adv Funct Mater, 2013, 23: 4087–4093

  30. 30

    Taylor S L, Jakus A E, Shah R N, et al. Iron and nickel cellular structures by sintering of 3D-printed oxide or metallic particle inks?. Adv Eng Mater, 2017, 19: 1600365

  31. 31

    Jakus A E, Taylor S L, Geisendorfer N R, et al. Metallic architectures from 3D-printed powder-based liquid inks. Adv Funct Mater, 2015, 25: 6985–6995

  32. 32

    Mahajan B K, Yu X, Shou W, et al. Mechanically milled irregular zinc nanoparticles for printable bioresorbable electronics. Small, 2017, 13: 1700065

  33. 33

    Ludwig B, Zheng Z, Shou W, et al. Solvent-free manufacturing of electrodes for lithium-ion batteries. Sci Rep, 2016, 6: 23150

  34. 34

    Shukla A K, Neergat M, Bera P, et al. An XPS study on binary and ternary alloys of transition metals with platinized carbon and its bearing upon oxygen electroreduction in direct methanol fuel cells. J Electroanal Chem, 2001, 504: 111–119

  35. 35

    Li X. Influence of substrate temperature on the orientation and optical properties of sputtered ZnO films. Mater Lett, 2003, 57: 4655–4659

  36. 36

    Mukherjee S, Ramalingam B, Gangopadhyay S. Hydrogen spillover at sub-2 nm Pt nanoparticles by electrochemical hydrogen loading. J Mater Chem A, 2014, 2: 3954–3960

  37. 37

    Pal B N, Chakravorty D. Pattern formation of zinc nanoparticles in silica film by electrodeposition. J Phys Chem B, 2006, 110: 20917–20921

  38. 38

    Yatsimirskii K B, Nemoskalenko V V, Aleshin V G, et al. X-ray photoelectron spectra of mixed oxygenated cobalt(II)-amino acid-imidazole complexes. Chem Phys Lett, 1977, 52: 481–484

  39. 39

    Bang S, Lee S, Ko Y, et al. Photocurrent detection of chemically tuned hierarchical ZnO nanostructures grown on seed layers formed by atomic layer deposition. Nanoscale Res Lett, 2012, 7: 290

  40. 40

    Lee Y K, Kim J, Kim Y, et al. Room temperature electrochemical sintering of Zn microparticles and its use in printable conducting inks for bioresorbable electronics. Adv Mater, 2017, 29: 1702665

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Acknowledgements

This work was supported financially by Interdisciplinary Intercampus Funding Program (IDIC) of University of Missouri System, University of Missouri Research Board (UMRB), Intelligent System Center (ISC) and Material Research Center (MRC) at Missouri University of Science and Technology. This work was also partially supported by National Science Foundation of USA (Grant No. 1363313) and ORAU Ralph E. Powe Junior Faculty Enhancement Award. Xian HUANG acknowledges the support of the National 1000 Talent Program. This work was supported by National Natural Science Foundation of China (Grant No. 61604108) and Natural Science Foundation of Tianjin (Grant No. 16JCYBJC40600). The authors would like to thank Mr. Brian Porter for help with XPS measurements.

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Correspondence to Heng Pan or Xian Huang.

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Mahajan, B.K., Ludwig, B., Shou, W. et al. Aerosol printing and photonic sintering of bioresorbable zinc nanoparticle ink for transient electronics manufacturing. Sci. China Inf. Sci. 61, 060412 (2018). https://doi.org/10.1007/s11432-018-9366-5

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Keywords

  • bioresorbable electronics
  • photonic sintering
  • aerosol printing
  • transient electronics
  • printed electronics
  • zinc nanoparticles