Abstract
This paper presents the study on co-capture of SO2 and NO x in O2/CO2 recycled coal combustion in a pilot scale facility with the heat input of 0.3 MW by using high-sulphur lean coal. Detailed comparison of SO2 and NO x emission indexes and desulphurization and denitration rates have been made among three working conditions of O2/CO2, O2/CO2 with limestone injection (O2/CO2+Ca) and O2/RFG (recycled flue gas) with limestone injection (O2/RFG+Ca). Combustion in air was performed as a base case. Results showed that in the O2/RFG with limestone injection, desulphurization and denitration rates could reach up to 96% and 89%, respectively. Limestone injection under the high-CO2 atmosphere caused a significant reduction on SO2 emission and NO x emission as well. This indicated O2/CO2 recycled coal combustion could reduce the investment on the flue gas purification. The techno-economic evaluation indicated that Oxy-combustion technique is not only feasible for CO2 emission control based on existing power plants but is also cost-effective.
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This work was supported by the National Basic Research Program of China (‘973’ Project) (Grant No. 2006CB705806) and the National Natural Science Foundation of China (Grant Nos. 50936001 and 50721005).
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Zou, C., Huang, Z., Xiong, J. et al. A pilot scale study on co-capture of SO2 and NO x in O2/CO2 recycled coal combustion and techno-economic evaluation. Sci. China Ser. E-Technol. Sci. 53, 155–159 (2010). https://doi.org/10.1007/s11431-009-0417-5
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DOI: https://doi.org/10.1007/s11431-009-0417-5