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Opportunities for ionic liquid-based electrolytes in rechargeable lithium batteries

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Abstract

Ionic liquids (ILs) have been deemed as promising electrolyte materials for building safer and highly-performing rechargeable lithium batteries, owing to their negligible volatility, low-flammability, and high thermal stability, etc. The profound structural designability of IL cations and anions allows relatively facile regulations of their key physical (e.g., viscosities, and ionic conductivities) and electrochemical (e.g., anodic, and cathodic stabilities) properties, and therefore fulfills the critical requirements stipulated by various battery configurations. In this review, a historical overview on the development of ILs for non-aqueous electrolytes is provided, and the correlations between chemical structures and the basic properties of ILs are discussed. Furthermore, the key achievements in the field of IL-based electrolytes are scrutinized, including liquid electrolytes, polymer electrolytes, and composite polymer electrolytes. Based on literature reports and our previous work in this field, possible strategies to improve the performance of IL-based electrolytes and their rechargeable batteries are discussed. The present work not only provides the status quo in the development of IL-based electrolytes but also inspires the structural design of ILs for other kinds of rechargeable batteries (e.g., sodium, potassium, zinc batteries).

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Acknowledgements

This work was supported from the Fundamental Research Funds for the Central Universities, HUST (2020kfyXJJS095), and the National Natural Science Foundation of China (52203223 and 22279037).

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  1. Key Laboratory of Material Chemistry for Energy Conversion and Storage (Ministry of Education), School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Wuhan, 430074, China

    Xingxing Wang, Letao Jin, Wenfang Feng, Zhibin Zhou & Heng Zhang

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Wang, X., Jin, L., Feng, W. et al. Opportunities for ionic liquid-based electrolytes in rechargeable lithium batteries. Sci. China Chem. 66, 3443–3466 (2023). https://doi.org/10.1007/s11426-023-1827-0

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