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Industry-compatible covalent organic frameworks for green chemical engineering

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Abstract

In order to move towards sustainable development, the discovery of energy-efficient and environmentally friendly materials has become increasingly imperative. Covalent organic frameworks (COFs) as emerging designable crystalline porous materials have captured increasing attention for a wide array of clean-energy and environmental applications, attributed to their attractive advantages of low density, high surface area, adjustable and periodic pores, and functional skeletons. This review attempts to highlight the key advancements made in the green synthesis of COFs, processing of COFs, energy and environment-related applications, including gas storage, water treatment, the separation of gas mixture and organic molecules, catalysis, supercapacitors, fuel cell, and rechargeable batteries. Finally, a perspective regarding the remaining challenges and future directions on the synthesis and promising application for green chemical engineering of COFs has also been presented based on current achievements.

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Acknowledgements

This work was supported by the National Natural Science Foundation of China (22001131), the Frontiers Science Center for New Organic Matter of Nankai University (63181206), 111 Projects (B12015), and the Postdoctoral Science Foundation of China (2019M660974).

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Authors and Affiliations

  1. State Key Laboratory of Medicinal Chemical Biology, College of Chemistry, Nankai University, Tianjin, 300071, China

    Zhifang Wang, Qianqian Zhu, Jiaxi Wang, Fazheng Jin, Penghui Zhang, Dong Yan, Peng Cheng, Yao Chen & Zhenjie Zhang

  2. Key Laboratory of Advanced Energy Materials Chemistry, Ministry of Education, Nankai University, Tianjin, 300071, China

    Zhifang Wang, Peng Cheng & Zhenjie Zhang

  3. College of Pharmacy, Nankai University, Tianjin, 300071, China

    Yao Chen

  4. Renewable Energy Conversion and Storage Center, Nankai University, Tianjin, 300071, China

    Peng Cheng & Zhenjie Zhang

  5. Frontiers Science Center for New Organic Matter, Nankai University, Tianjin, 300071, China

    Peng Cheng

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  1. Zhifang Wang
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  2. Qianqian Zhu
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  3. Jiaxi Wang
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  4. Fazheng Jin
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  5. Penghui Zhang
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  6. Dong Yan
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  7. Peng Cheng
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  8. Yao Chen
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  9. Zhenjie Zhang
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Correspondence to Yao Chen or Zhenjie Zhang.

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Wang, Z., Zhu, Q., Wang, J. et al. Industry-compatible covalent organic frameworks for green chemical engineering. Sci. China Chem. 65, 2144–2162 (2022). https://doi.org/10.1007/s11426-022-1391-0

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  • DOI: https://doi.org/10.1007/s11426-022-1391-0

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