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The chemistry and physics of organic—inorganic hybrid perovskite quantum wells

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Abstract

Organic—inorganic hybrid two dimensional (2D) lead halide perovskites (LHPs) are tunable quantum wells that exhibit a set of intriguing structural and physical properties including soft and dynamic lattices, organic—inorganic epitaxial heterointerfaces, quantum and dielectric confinements, strong light—matter interactions, and large spin—orbit coupling, which enable promising perspectives for optoelectronics, ferroelectrics, and spintronics. While the properties of 2D LHPs bear some resemblance of the 3D LHPs, they are often drastically altered due to the reduced dimensionality and the complex interactions between organic and inorganic components. In this review, we discuss the influences of the reduced dimensionality and the organic—inorganic interplays on the structural stability and distortion of the inorganic lattices, inversion symmetry of the crystal structure, electronic band structures, excitonic physics, and carrier—phonon interactions in 2D LHPs. An emphasis is placed on the relationships between the crystal structures and photophysical properties. Future perspectives on the opportunities of hybrid quantum wells are provided.

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Acknowledgements

This work is supported by the National Natural Science Foundation of China (22271006). Y. F. thanks Peking University and Beijing National Laboratory for Molecular Sciences for startup funding.

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  1. Beijing National Laboratory for Molecular Science, State Key Laboratory of Rare Earth Materials Chemistry and Applications, College of Chemistry and Molecular Engineering, Peking University, Beijing, 100871, China

    Yongping Fu

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Fu, Y. The chemistry and physics of organic—inorganic hybrid perovskite quantum wells. Sci. China Chem. 65, 2058–2076 (2022). https://doi.org/10.1007/s11426-022-1389-6

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