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Electrolyte chemistry for lithium metal batteries

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Abstract

Li metal batteries (LMBs) are considered as the next-generation energy storage systems because of their high energy density. However, due to the high reactivity of Li metal with the electrolyte, the unwanted safety concerns inhibit the practical application of LMBs. To overcome these drawbacks, exploring suitable electrolytes is considered to be urgent. Great effort has been made to modify electrolytes to achieve the stability of LMBs. In this review, different kinds of LMBs are firstly introduced. Then, the regulation of electrode—electrolyte interphase is discussed. Next, recent advances on the functional electrolytes for LMBs are overviewed, including fireproof electrolytes, extreme-temperature electrolytes and high-voltage electrolytes. Finally, the perspective on the development of future electrolytes is provided.

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Acknowledgements

This work was supported by the National Natural Science Foundation of China (51971090 and U21A20311).

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Authors and Affiliations

  1. School of Materials and Energy, University of Electronic Science and Technology of China, Chengdu, 610054, China

    Junda Huang, Mingguang Wu, Huaping Wang, Shihan Qi, Gaoxue Jiang, Xiu Li & Jianmin Ma

  2. School of Physics and Electronics, Hunan University, Changsha, 410082, China

    Junda Huang, Fang Li, Mingguang Wu, Huaping Wang & Gaoxue Jiang

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  1. Junda Huang
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Huang, J., Li, F., Wu, M. et al. Electrolyte chemistry for lithium metal batteries. Sci. China Chem. 65, 840–857 (2022). https://doi.org/10.1007/s11426-021-1235-2

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