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Petroleum sludge treatment and disposal techniques: a review

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Abstract

Petroleum sludge is a solid emulsified waste and contaminant commonly produced in the petroleum industry. In the recent past, there has been increased business growth in the oil sector, resulting in increased volumes of oily sludge characterized by high viscosity and toxicity. Therefore, sludge treatment before discarding is extremely necessary. This review seeks to highlight various conventional and evolving approaches in the treatment, recovery, and disposal of petroleum sludge and assess their suitability under various conditions.

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References

  • Aeslina A, Ali B (2017) Petroleum sludge treatment and reuse for cement production as setting retarder. IOP Conference Series: Mater Sci Eng

  • Aguelmous A, El Fels L, Souabi S, Zamama M, Hafidi M (2019) The fate of total petroleum hydrocarbons during oily sludge composting: a critical review. Rev Environ Sci Biotechnol 18(3):473–493

    Article  CAS  Google Scholar 

  • Aguelmous A, El Fels L, Souabi S, Zamama M, Yasri A, Lebrihi A, Hafidi M (2018) Petroleum sludge bioremediation and its toxicity removal by landfill in gunder semi-arid conditions. Ecotoxicol Environ Saf 166:482–487

    Article  CAS  Google Scholar 

  • Aguelmous A, Zegzouti Y, Khadra A, El Fels L, Souabi S, Hafidi M (2020) Landfilling and composting efficiency to reduce genotoxic effect of petroleum sludge. Environ Tech Innov 20:101047

  • Ahmaruzzaman M (2010) A review on the utilization of fly ash. Prog Energy Combust Sci 36(3):327–363

    Article  CAS  Google Scholar 

  • Akinyemi O (2020) Recent development on biological treatment of oil sludge from petroleum industry. Am J Sci Eng Res 3(3)

  • Al-Futaisi A, Jamrah A, Yaghi B, Taha R (2007) Assessment of alternative management techniques of tank bottom petroleum sludge in Oman. Journal of hazardous materials 141(3):557–564

    Article  CAS  Google Scholar 

  • Ali N, Dashti N, Khanafer M, Al-Awadhi H, Radwan S (2020) Bioremediation of soils saturated with spilled crude oil. Scientific reports 10(1):1–9

    CAS  Google Scholar 

  • Al-Khateeb HMM (2020) Effect of land-farming oily sludge on run-off water. Int J New Technol Res 6(8):41–46

    Google Scholar 

  • Asim, N., Badiei, M., Torkashvand, M., Mohammad, M., Alghoul, M. A., Gasaymeh, S. S., & Sopian, K. (2020). Wastes from the petroleum industries as sustainable resource materials in construction sectors: opportunities, limitations, and directions. Journal of Cleaner Production, 125459.

  • Azim A-AAA, Abdul-Raheim A-RM, Kamel RK, Abdel-Raouf ME (2011) Demulsifier systems applied to breakdown petroleum sludge. J Petrol Sci Eng 78(2):364–370

    Article  CAS  Google Scholar 

  • Bhattacharyya J, Shekdar A (2003) Treatment and disposal of refinery sludges: Indian scenario. Waste Manage Res 21(3):249–261

    Article  CAS  Google Scholar 

  • Canselier J, Delmas H, Wilhelm A, Abismail B (2002) Ultrasound emulsification—an overview. J Dispersion Sci Technol 23(1–3):333–349

    Article  CAS  Google Scholar 

  • Chen G, Li J, Li K, Lin F, Tian W, Che L, Yan B, Ma W, Song Y (2020) Nitrogen, sulfur, chlorine-containing pollutants releasing characteristics during pyrolysis and combustion of oily sludge. Fuel 273:117772

  • Chu Z, Gong Z, Wang Z, Zhang H, Liu L, Wu J, Wang J (2021) Experimental study on gasification of oil sludge with steam and its char characteristic. J Hazard Mater 416:125713

  • da Silva DC, dos Santos Lucas CR, de Moraes Juviniano HB, de Alencar Moura MCP, de Castro Dantas TN, Neto AAD (2019) Analysis of the use of microemulsion systems to treat petroleum sludge from a water flotation unit. J Environ Chem Eng 7(1):102934

  • da Silva LJ, Alves FC, de França FP (2012) A review of the technological solutions for the treatment of oily sludges from petroleum refineries. Waste Manage Res 30(10):1016–1030

    Article  CAS  Google Scholar 

  • Dando, D., & Martin, D. (2003). A guide for reduction and disposal of waste from oil refineries and marketing installations (Vol. 6). CONCAWE Brussels, Belgium.

  • Dantas TC, Oliveira K, Neto AD, Moura M (2009) The use of microemulsions to remove chromium from industrial sludge. Water Res 43(5):1464–1470

    Article  CAS  Google Scholar 

  • Das, S., Kuppanan, N., Channashettar, V. A., & Lal, B. (2018). Remediation of oily sludge-and oil-contaminated soil from petroleum industry: recent developments and future prospects. Advances in Soil Microbiology: Recent Trends and Future Prospects, 165–177.

  • Elektorowicz M, Habibi S, Chifrina R (2006) Effect of electrical potential on the electro-demulsification of oily sludge. J Colloid Interface Sci 295(2):535–541

    Article  CAS  Google Scholar 

  • Fenibo EO, Ijoma GN, Selvarajan R, Chikere CB (2019) Microbial surfactants: the next generation multifunctional biomolecules for applications in the petroleum industry and its associated environmental remediation. Microorganisms 7(11):581

  • Ferrarese E, Andreottola G, Oprea IA (2008) Remediation of PAH-contaminated sediments by chemical oxidation. J Hazard Mater 152(1):128–139

    Article  CAS  Google Scholar 

  • Gao N, Kamran K, Quan C, Williams PT (2020) Thermochemical conversion of sewage sludge: a critical review. Prog Energy Combust Sci 79:100843

  • Gong Z, Liu C, Wang M, Wang Z, Li X (2020) Experimental study on catalytic pyrolysis of oil sludge under mild temperature. Sci Total Environ 708:135039

  • Gorbaev A, Gorlenko N, Timofeeva S (2020) Use of oil sludge as a combustible additive for the production of bricks. IOP Conference Series: Mater Sci Eng 962(4):042031

  • Guerin TF (2021) Prototyping of co-composting as a cost-effective treatment option for full-scale on-site remediation at a decommissioned refinery. J Clean Prod 302:127012

  • Hahn, W., & Loehr, R. (1992). Biological treatment of petroleum oily sludges. Permian Basin Oil and Gas Recovery Conference,

  • He S, Tan X, Hu X, Gao Y (2019) Effect of ultrasound on oil recovery from crude oil containing sludge. Environ Technol 40(11):1401–1407

    Article  CAS  Google Scholar 

  • Hu G, Li J, Zeng G (2013) Recent development in the treatment of oily sludge from petroleum industry: a review. J Hazard Mater 261:470–490

    Article  CAS  Google Scholar 

  • Hu G, Li J, Hou H (2015) A combination of solvent extraction and freeze thaw for oil recovery from petroleum refinery wastewater treatment pond sludge. J Hazard Mater 283:832–840

    Article  CAS  Google Scholar 

  • Hu G, Li J, Huang S, Li Y (2016) Oil recovery from petroleum sludge through ultrasonic assisted solvent extraction. J Environ Sci Health A 51(11):921–929

    Article  CAS  Google Scholar 

  • Hu G, Li J, Zhang X, Li Y (2017) Investigation of waste biomass co-pyrolysis with petroleum sludge using a response surface methodology. J Environ Manage 192:234–242

    Article  CAS  Google Scholar 

  • Hu G, Feng H, He P, Li J, Hewage K, Sadiq R (2020a) Comparative life-cycle assessment of traditional and emerging oily sludge treatment approaches. J Clean Prod 251:119594

  • Hu Y, Cheng H, Ji J, Li Y-Y (2020b) A review of anaerobic membrane bioreactors for municipal wastewater treatment with a focus on multicomponent biogas and membrane fouling control. Environ Sci: Water Res Technol 6(10):2641–2663

  • Hua Q (2020) Experimental studies on viscosity reduction of heavy crude oil by ultrasonic irradiation. Acoust Phys 66(5):495–500

    Article  Google Scholar 

  • Huang Q, Wang J, Qiu K, Pan Z, Wang S, Chi Y, Yan J (2015) Catalytic pyrolysis of petroleum sludge for production of hydrogen-enriched syngas. Int J Hydrogen Energy 40(46):16077–16085

    Article  CAS  Google Scholar 

  • Hui, K., Tang, J., Lu, H., Xi, B., Qu, C., & Li, J. (2020). Status and prospect of oil recovery from oily sludge: a review. Arabian Journal of Chemistry.

  • Islam, M. (1995). New methods of petroleum sludge disposal and utilization. In Asphaltenes (pp. 219–235). Springer.

  • Islam B (2015) Petroleum sludge, its treatment and disposal: a review. Int J Chem Sci 13(4):1584–1602

    CAS  Google Scholar 

  • Jafarinejad, S. (2017). 7-solid-waste management in the petroleum industry, petroleum waste treatment and pollution control.

  • Jean D, Lee D (1999) Expression deliquoring of oily sludge from a petroleum refinery plant. Waste Manage 19(5):349–354

    Article  CAS  Google Scholar 

  • Jean D, Chu C, Lee D (2001) Freeze/thaw treatment of oily sludge from petroleum refinery plant. Sep Sci Technol 36(12):2733–2746

    Article  CAS  Google Scholar 

  • Johnson OA, Affam AC (2019) Petroleum sludge treatment and disposal: a review. Environ Eng Res 24(2):191–201

    Article  Google Scholar 

  • Johnson OA, Napiah M, Kamaruddin I (2014) Potential uses of waste sludge in construction industry: a review. Res J Appl Sci Eng Technol 8(4):565–570

    Article  Google Scholar 

  • Johnson OA, Madzlan N, Kamaruddin I (2015) Encapsulation of petroleum sludge in building blocks. Constr Build Mater 78:281–288

    Article  Google Scholar 

  • Kamil MNAF, Kadir AA, Bujang UH, Hassan HMI (2017) Treatment of petroleum sludge

  • Katsivela E, Moore E, Maroukli D, Strömpl C, Pieper D, Kalogerakis N (2005) Bacterial community dynamics during in-situ bioremediation of petroleum waste sludge in landfarming sites. Biodegradation 16(2):169–180

    Article  CAS  Google Scholar 

  • Khan FI, Husain T, Hejazi R (2004) An overview and analysis of site remediation technologies. J Environ Manage 71(2):95–122

    Article  Google Scholar 

  • Kirchmann H, Ewnetu W (1998) Biodegradation of petroleum-based oil wastes through composting. Biodegradation 9(2):151–156

    Article  CAS  Google Scholar 

  • Kokalj F, Arbiter B, Samec N (2017) Sewage sludge gasification as an alternative energy storage model. Energy Convers Manage 149:738–747

    Article  CAS  Google Scholar 

  • Koolivand A, Naddafi K, Nabizadeh R, Nasseri S, Jafari AJ, Yunesian M, Yaghmaeian K, Nazmara S (2013) Biodegradation of petroleum hydrocarbons of bottom sludge from crude oil storage tanks by in-vessel composting. Toxicol Environ Chem 95(1):101–109

    Article  CAS  Google Scholar 

  • Kriipsalu M, Marques M, Maastik A (2008) Characterization of oily sludge from a wastewater treatment plant flocculation-flotation unit in a petroleum refinery and its treatment implications. J Mater Cycles Waste Manage 10(1):79–86

    Article  CAS  Google Scholar 

  • Kuo C-H, Lee C-L (2010) Treatment of oil/water emulsions using seawater-assisted microwave irradiation. Separation and Purification Technology 74(3):288–293

    Article  CAS  Google Scholar 

  • Łamacz A, Krztoń A, Musi A, Da Costa P (2009) Reforming of model gasification tar compounds. Catal Lett 128(1):40–48

    Article  CAS  Google Scholar 

  • Lee CL, Tsai C-H, Jou C-JG (2020) Energy and resource utilization of refining industry oil sludge by microwave treatment. Sustainability 12(17):6862

    Article  CAS  Google Scholar 

  • Li J, Lin F, Li K, Zheng F, Yan B, Che L, Tian W, Chen G, Yoshikawa K (2020a) A critical review on energy recovery and non-hazardous disposal of oily sludge from petroleum industry by pyrolysis. J Hazard Mater 406(2021):124706

  • Li X, Zhang F, Guan B, Sun J, Liao G (2020b) Review on oily sludge treatment technology. IOP Conference Series: Earth Environ Sci 467(1):012173

  • Li Y, Jiang L (2021) Comparison of the crude oil removal effects of different surfactants in electrokinetic remediation of low-permeability soil. J Environ Chem Eng 9(4):105190

  • Liu C, Hu X, Xu Q, Zhang S, Zhang P, Guo H, You Y, Liu Z (2021a) Response surface methodology for the optimization of the ultrasonic-assisted rhamnolipid treatment of oily sludge. Arab J Chem 14(3):102971

  • Liu W-J, Shao Z-G, Xu Y (2021b) Emission characteristics of nitrogen and sulfur containing pollutants during the pyrolysis of oily sludge with and without catalysis. J Hazard Mater 401:123820

  • Lv X, Song Z, Yu J, Su Y, Zhao X, Sun J, Mao Y, Wang W (2020) Study on the demulsification of refinery oily sludge enhanced by microwave irradiation. Fuel 279:118417

  • Machín-Ramírez C, Okoh A, Morales D, Mayolo-Deloisa K, Quintero R, Trejo-Hernández M (2008) Slurry-phase biodegradation of weathered oily sludge waste. Chemosphere 70(4):737–744

    Article  CAS  Google Scholar 

  • Maga, S., Goetz, F., & Durlak, E. (2003). Operational test report (OTR): on-site degradation of oily sludge in a tenthousand gallon sequencing batch reactor at Navsta Pearl Harbor, HI.

  • Mahdi, A. M. E., Aziz, H. A., & Eqab, E. S. (2017). Review on innovative techniques in oil sludge bioremediation. AIP Conference Proceedings,

  • Marzuki I, Daris L, Yunus S, Riana AD (2020) Selection and characterization of potential bacteria for polycyclic aromatic biodegradation of hydrocarbons in sea sponges from Spermonde Islands. Indonesia. Aquac Aquar Conserv Legis 13(6):3493–3506

    Google Scholar 

  • McCauley, P., & Glaser, J. (1996). Slurry bioreactors for treatment of contaminated soils, sludges, and sediments.

  • Mishra H, Karmakar S, Kumar R, Singh J (2017) A framework for assessing uncertainty associated with human health risks from MSW landfill leachate contamination. Risk Anal 37(7):1237–1255

    Article  Google Scholar 

  • Obi L, Atagana H, Adeleke R, Maila M, Bamuza-Pemu E (2020) Potential microbial drivers of biodegradation of polycyclic aromatic hydrocarbons in crude oil sludge using a composting technique. J Chem Technol Biotechnol 95(5):1569–1579

    Article  CAS  Google Scholar 

  • Oladejo J, Shi K, Luo X, Yang G, Wu T (2019) A review of sludge-to-energy recovery methods. Energies 12(1):60

  • Ossai IC, Ahmed A, Hassan A, Hamid FS (2020) Remediation of soil and water contaminated with petroleum hydrocarbon: a review. Environ Technol Innov 17:100526

  • Pakpahan EN, Isa MH, Kutty SRM, Chantara S, Wiriya W (2013) Polycyclic aromatic hydrocarbon removal from petroleum sludge cake using thermal treatment with additives. Environ Technol 34(3):407–416

    Article  CAS  Google Scholar 

  • Peng L, Wang Y, Lei Z, Cheng G (2012) Co-gasification of wet sewage sludge and forestry waste in situ steam agent. Biores Technol 114:698–702

    Article  CAS  Google Scholar 

  • Pinheiro B, Holanda J (2009) Processing of red ceramics incorporated with encapsulated petroleum waste. J Mater Process Technol 209(15–16):5606–5610

    Article  CAS  Google Scholar 

  • Prashanth PF, Shravani B, Vinu R, Lavanya M, Prabu VR (2021) Production of diesel range hydrocarbons from crude oil sludge via microwave-assisted pyrolysis and catalytic upgradation. Process Saf Environ Prot 146:383–395

    Article  CAS  Google Scholar 

  • Raheem A, Sikarwar VS, He J, Dastyar W, Dionysiou DD, Wang W, Zhao M (2018) Opportunities and challenges in sustainable treatment and resource reuse of sewage sludge: a review. Chem Eng J 337:616–641

    Article  CAS  Google Scholar 

  • Ramirez D, Shaw LJ, Collins CD (2021) Oil sludge washing with surfactants and co-solvents: oil recovery from different types of oil sludges. Environ Sci Pollut Res 28(5):5867–5879

    Article  CAS  Google Scholar 

  • Roche E, de Andrés JM, Narros A, Rodríguez ME (2014) Air and air-steam gasification of sewage sludge. The influence of dolomite and throughput in tar production and composition. Fuel 115:54–61

    Article  CAS  Google Scholar 

  • Sampson, I. E., & Ujile, A. A. (2016). Bioreactor performance in anaerobic digestion of petroleum sludge based on hydrocarbon content of treated sludge.

  • Santiago YC, González AM, Venturini OJ, Maya DMY (2021) Assessment of the energy recovery potential of oil sludge through gasification aiming electricity generation. Energy 215:119210

  • Sayara T, Sánchez A (2020) Bioremediation of PAH-contaminated soils: process enhancement through composting/compost. Appl Sci 10(11):3684

  • Seo S, Mastiani M, Mosavati B, Peters DM, Mandin P, Kim M (2018) Performance evaluation of environmentally benign nonionic biosurfactant for enhanced oil recovery. Fuel 234:48–55

    Article  CAS  Google Scholar 

  • Shailubhai K (1986) Treatment of petroleum industry oil sludge in soil. Trends Biotechnol 4(8):202–206

    Article  CAS  Google Scholar 

  • Singh B, Kumar P (2020) Physicochemical characteristics of hazardous sludge from effluent treatment plant of petroleum refinery as feedstock for thermochemical processes. J Environ Chem Eng 8(4):103817

  • Smith, K. P., Arnish, J. J., Williams, G. P., & Blunt, D. L. (2003). Assessment of the disposal of radioactive petroleum industry waste in nonhazardous landfills using risk-based modeling. In: ACS Publications.

  • Swathi K, Muneeswari R, Ramani K, Sekaran G (2020) Biodegradation of petroleum refining industry oil sludge by microbial-assisted biocarrier matrix: process optimization using response surface methodology. Biodegradation 31(4):385–405

    Article  CAS  Google Scholar 

  • Taiwo E, Otolorin J (2009) Oil recovery from petroleum sludge by solvent extraction. Pet Sci Technol 27(8):836–844

    Article  CAS  Google Scholar 

  • Tang C, Guan J, Xie S (2020) Study on re-utilization of pyrolytic residues of oily sludge. Int J Anal Chem

  • Teng Q, Zhang D, Yang C (2020) A review of the application of different treatment processes for oily sludge. Environ Sci Pollut Res 28(1):121–132

    Article  CAS  Google Scholar 

  • Uwem UM, Sunday DM, Wosilat AF, Jonah UU (2019) Bioremediation of petroleum sludge impacted soils using agro-waste from Moringa seed. Sci J Anal Chem 7(1):1–12

    Article  CAS  Google Scholar 

  • Wang D, Zhao Z, Chenyu Q, Yang W, Yueying H, McKay P, Yang D, Liu Q, Zeng H (2020a) Techniques for treating slop oil in oil and gas industry: a short review. Fuel 279:118482

  • Wang X, Xu X, Dang W, Hu C, Tang Z, Wei B (2020b) Centrifugal reduction treatment process for high-water-content sludge in Oilfield. Nat Environ Pollut Technol 19(1):169–178

  • Ward O, Singh A, Van Hamme J (2003) Accelerated biodegradation of petroleum hydrocarbon waste. J Ind Microbiol Biotechnol 30(5):260–270

    Article  CAS  Google Scholar 

  • Werle S (2015) Gasification of a dried sewage sludge in a laboratory scale fixed bed reactor. Energies 8(8):8562–8572

    Article  CAS  Google Scholar 

  • Yang L, Nakhla G, Bassi A (2005) Electro-kinetic dewatering of oily sludges. J Hazard Mater 125(1–3):130–140

    Article  CAS  Google Scholar 

  • Yang Q, Zhang C, Li L, Xu W (2020) Anaerobic co-digestion of oil sludge with corn stover for efficient biogas production. Sustainability 12(5):1861

  • Yuan W, Zhang L, Chang Y, Ma H, Fu P, Wang H, Li J (2021) Treatment of biofuel production wastewater by a combined freezing method for resources recovery and waste reduction. Sci Total Environ 774:145173

  • Yuliarningsih R, Goembira F, Komala PS, Putra NP, Nasra M (2020) Oil sludge and biomass waste utilization as densified refuse-derived fuels for alternative fuels: case study of an indonesia cement plant. J Hazard Toxic Radioact Waste 24(4):05020001

  • Zain AM, Shaaban MG, Mahmud H (2010) Immobilization of petroleum sludge incorporating portland cement and rice husk ash. Int J Chem Eng Appl 1(3):234

    CAS  Google Scholar 

  • Zango ZU (2020) Review of petroleum sludge thermal treatment and utilization of ash as a construction material, a way to environmental sustainability. Int J Adv Appl Sci 7(12)

  • Zhang J, Li J, Thring RW, Hu X, Song X (2012) Oil recovery from refinery oily sludge via ultrasound and freeze/thaw. J Hazard Mater 203:195–203

    Article  CAS  Google Scholar 

  • Zhao J, Dai C, Ding Q, Du M, Feng H, Wei Z, Chen A, Zhao M (2015) The structure effect on the surface and interfacial properties of zwitterionic sulfobetaine surfactants for enhanced oil recovery. RSC Adv 5(18):13993–14001

    Article  CAS  Google Scholar 

  • Zheng X, Ying Z, Cui J, Wang B, Chen J, Zhang Q (2017) Simultaneous dewatering and recovering oil from high-viscosity oily sludge through the combination process of demulsification, viscosity reduction, and centrifugation. Energy Fuels 31(12):14401–14407

    Article  CAS  Google Scholar 

  • Zubaidy EA, Abouelnasr DM (2010) Fuel recovery from waste oily sludge using solvent extraction. Process Saf Environ Prot 88(5):318–326

    Article  CAS  Google Scholar 

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Acknowledgements

The authors would like to thank the Malaysia Ministry of Higher Education for funding this research through the Fundamental Research Grant Scheme, FRGS (Cost Center: 015MA0-082).

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Fundamental research grant scheme (FRGS) under Malaysia Ministry of Higher Education: FRGS (Cost Center: 015MA0-082).

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All authors contributed; where AAS to the study concept, design, supervision, and revision of the work and PIM to the literature search and drafting of the manuscript.

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Correspondence to Pearl Isabellah Murungi.

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Murungi, P.I., Sulaimon, A.A. Petroleum sludge treatment and disposal techniques: a review. Environ Sci Pollut Res 29, 40358–40372 (2022). https://doi.org/10.1007/s11356-022-19614-z

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