Skip to main content
Log in

Experimental investigation of temperature distribution and spontaneous combustion tendency of coal gangue stockpiles in storage

  • Published:
Environmental Science and Pollution Research Aims and scope Submit manuscript

Abstract

In this study, an experimental model about the coal gangue stockpiles in semi-open storage was developed. According to the model’s requirements, the corresponding coal gangues were piled up in the factory building, the heat source and collection points were arranged, and the four operating temperatures were selected from 70 to 350 °C for heating. A series of fire experiments concerning the temperature distributions of the coal gangue piles were conducted systematically. The spontaneous combustion tendency of coal gangue samples under kinds of the four heat sources was analyzed using scanning electron microscope (SEM), thermal gravity analysis, and differential thermal gravity (TG-DTG). Under the action of thermal damage, the surface of micropores in coal gangue becomes rough. Heat accumulation is, in nature, most likely to occur near 0.1~0.4 m away from the heat source of coal pile. Simultaneously, on each of the measured flat layers, the greater the horizontal distance from the heat source is, the lower the heated temperature of gangues is, and the lower the temperature change rate is, indicating that the horizontal heat conduction is also gradually weakened. The experimental model provides an empirical basis for studying the distribution of temperature field in the depth of gangue pile and kinetics reaction mechanism of spontaneous combustion.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6
Fig. 7
Fig. 8
Fig. 9
Fig. 10

Similar content being viewed by others

Data availability

The datasets used and/or analyzed during the current study are available from the corresponding author on reasonable request.

Abbreviations

C p :

Specific heat capacity, J/(kg·K)

t:

Record the instantaneous temperatures of time, h

T0 :

Initial temperature before heating, °C

T1 :

Temperature at a specific moment, °C

Δt :

Difference of time, h

v :

Temperature rise rate, °C/h

TG:

Thermal gravity

DTG:

Differential thermal gravity

SEM:

Scanning electron microscope

ρ :

The density of coal gangue, kg/m3

λ :

Thermal conductivity of coal gangue, W/(m·K)

ad:

Air-dried basis

daf:

Dry ash-free basis

X:

X direction

Y:

Y direction

Z:

Z direction

O:

Origin of a 3D axis

References

  • Arisoy A, Beamish B (2015) Reaction kinetics of coal oxidation at low temperatures. Fuel 159:412–417

  • Barkalov IM, Kiryukhin DP (1994) Kinetic calorimetry in the study of the mechanism of low-temperature chemical reactions. Int Rev Phys Chem 13:337–357

    Article  CAS  Google Scholar 

  • Bo C, Diao ZJ, Lu HYJF (2014) Using the ReaxFF reactive force field for molecular dynamics simulations of the spontaneous combustion of lignite with the Hatcher lignite model. Fuel 116:7–13

  • Deng J, Zhao J, Zhang Y, Huang A, Liu X, Zhai X, Wang C (2016) Thermal analysis of spontaneous combustion behavior of partially oxidized coal. Process Saf Environ Prot 104:218–224

    Article  CAS  Google Scholar 

  • Deng J, Li B, Xiao Y, Ma L, Shu C-M (2017) Spontaneous combustion characteristics and micro characterization of coal gangue based on thermogravimetry-Fourier transform infrared spectrometer. J Xi'an Univ Sci Technol 37:1–6

    Google Scholar 

  • Fan J, Liu P, Li J, Jiang D (2020) A coupled methane/air flow model for coal gas drainage: model development and finite-difference solution. Process Saf Environ Prot 141:288–304

    Article  CAS  Google Scholar 

  • Huang Y, Shi M, Zhu C (2020) What are the resource benefits of circulating fluidized bed power generation technology? Take some key thermal power units in China as an example. Int J Energy Res 44:4687–4702

    Article  Google Scholar 

  • Jiang L, Liang J, Yuan X, Li H, Li C, Xiao Z, Huang H, Wang H, Zeng G (2014) Co-pelletization of sewage sludge and biomass: the density and hardness of pellet. Bioresour Technol 166:435–443

    Article  CAS  Google Scholar 

  • Liang Y, Liang H, Zhu S (2016) Mercury emission from spontaneously ignited coal gangue hill in Wuda coalfield, Inner Mongolia, China. Fuel 182:525–530

    Article  CAS  Google Scholar 

  • Liu H, Liu Z (2010) Recycling utilization patterns of coal mining waste in China. Resour Conserv Recycl 54:1331–1340

    Article  Google Scholar 

  • Liu A, Liu P, Liu S (2020) Gas diffusion coefficient estimation of coal: a dimensionless numerical method and its experimental validation. Int J Heat Mass Transf 162:120336

    Article  CAS  Google Scholar 

  • Lu Y, Qin B (2015a) Experimental investigation of closed porosity of inorganic solidified foam designed to prevent coal fires. Adv Mater Sci Eng 1–9

  • Lu Y, Qin B (2015b) Mechanical properties of inorganic solidified foam for mining rock fracture filling. Mater Express 5:291–299

    Article  CAS  Google Scholar 

  • Misz-Kennan M, Fabiańska MJ (2011) Application of organic petrology and geochemistry to coal waste studies. Int J Coal Geol 88:1–23

    Article  CAS  Google Scholar 

  • Misz-Kennan M, Gardocki M, Tabor A (2015) Chapter 13 - fire prevention in coal waste dumps: exemplified by the Rymer Cones. Upper Silesian Coal Basin, Poland, pp 349–385

  • Moqbel S, Reinhart D, Chen RH (2010) Factors influencing spontaneous combustion of solid waste. Waste Manag 30:1600–1607

    Article  CAS  Google Scholar 

  • Nádudvari Á (2014) Thermal mapping of self-heating zones on coal waste dumps in Upper Silesia (Poland) — a case study. Int J Coal Geol 128–129:47–54

  • Querol X, Zhuang X, Font O, Izquierdo M, Alastuey A, Castro I, van Drooge BL, Moreno T, Grimalt JO, Elvira J, Cabañas M, Bartroli R, Hower JC, Ayora C, Plana F, López-Soler A (2011) Influence of soil cover on reducing the environmental impact of spontaneous coal combustion in coal waste gobs: a review and new experimental data. Int J Coal Geol 85:2–22

    Article  CAS  Google Scholar 

  • Ren W, Guo Q, Wang Z (2016) Application of foam–gel technology for suppressing coal spontaneous combustion in coal mines. Nat Hazards 84:1207–1218

    Article  Google Scholar 

  • Sawicki T (2004) Spontaneous combustion in stock piles as the cause of fire. Karbo 1:56–59

    Google Scholar 

  • Swaine DJ (2000) Why trace elements are important. Fuel Process Technol 65:21–33

    Article  Google Scholar 

  • Tang Y, Xue S (2015) Laboratory study on the spontaneous combustion propensity of lignite undergone heating treatment at low temperature in inert and low-oxygen environments. Energy Fuel 29:4683–4689

    Article  CAS  Google Scholar 

  • Taraba B, Peter R, Slovák V (2011) Calorimetric investigation of chemical additives affecting oxidation of coal at low temperatures. Fuel Energy Abstr 92:712–715

    CAS  Google Scholar 

  • Wang H, Dlugogorski BZ, Kennedy EM (2002) Thermal decomposition of solid oxygenated complexes formed by coal oxidation at low temperatures. Fuel 81:1913–1923

    Article  CAS  Google Scholar 

  • Wen H, Yu Z, Fan S, Zhai X, Liu W (2017) Prediction of spontaneous combustion potential of coal in the gob area using CO extreme concentration: a case study. Combust Sci Technol 189:1713–1727

    Article  CAS  Google Scholar 

  • Xia T, Zhou F, Wang X, Zhang Y, Li Y, Kang J, Liu J (2016) Controlling factors of symbiotic disaster between coal gas and spontaneous combustion in longwall mining gobs. Fuel 182:886–896

    Article  CAS  Google Scholar 

  • Yang Y, Li Z, Tang Y, Liu Z, Ji H (2014) Fine coal covering for preventing spontaneous combustion of coal pile. Nat Hazards 74:603–622

    Article  Google Scholar 

  • Yu Z, Gu Y, Yang S, Deng J (2020) Temperature characteristic of crushed coal under liquid coolant injection: a comparative investigation between CO2 and N2. J Therm Anal Calorim 1–10

  • Yuanyuan Z, Yanxia G, Fangqin C, Kezhou Y, Yan C (2015) Investigation of combustion characteristics and kinetics of coal gangue with different feedstock properties by thermogravimetric analysis. Thermochim Acta 614:137–148

    Article  Google Scholar 

  • Zhang J, Ren T, Liang Y, Wang Z (2016) A review on numerical solutions to self-heating of coal stockpile: mechanism, theoretical basis, and variable study. Fuel 182:80–109

    Article  CAS  Google Scholar 

  • Zhao J, Deng J, Chen L, Wang T, Song J, Zhang Y, Shu C-M, Zeng Q (2019a) Correlation analysis of the functional groups and exothermic characteristics of bituminous coal molecules during high-temperature oxidation. Energy 181:136–147

    Article  CAS  Google Scholar 

  • Zhao J, Deng J, Wang T, Song J, Zhang Y, Shu C-M, Zeng Q (2019b) Assessing the effectiveness of a high-temperature-programmed experimental system for simulating the spontaneous combustion properties of bituminous coal through thermokinetic analysis of four oxidation stages. Energy 169:587–596

    Article  CAS  Google Scholar 

Download references

Funding

The study is financially supported by major science and technology projects of Inner Mongolia Autonomous Region under Grant No. RZ190001148 and Grant No. NJZY21480. The authors appreciate the supports deeply.

Author information

Authors and Affiliations

Authors

Contributions

Ang Li: Conceptualization, Methodology, Data curation, Writing—original draft. Changkun Chen: Writing—review and editing; Supervision. Jie Chen: Writing—review and editing; Project administration. Peng Lei: Writing—review and editing. Yulun Zhang: Writing—review and editing.

Corresponding author

Correspondence to Changkun Chen.

Ethics declarations

Ethical approval

Not applicable.

Consent to participate

Not applicable.

Consent for publication

Not applicable.

Competing interest

The authors declare no competing interests.

Additional information

Responsible editor: Philippe Garrigues

Publisher’s note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Li, A., Chen, C., Chen, J. et al. Experimental investigation of temperature distribution and spontaneous combustion tendency of coal gangue stockpiles in storage. Environ Sci Pollut Res 28, 34489–34500 (2021). https://doi.org/10.1007/s11356-021-12964-0

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s11356-021-12964-0

Keywords

Navigation