Skip to main content

Advertisement

Log in

Assessment of the Impacts of Climate Change on European Ozone Levels

  • Published:
Water, Air, & Soil Pollution Aims and scope Submit manuscript

Abstract

The objective of this study is to investigate the potential impact of future climate change on ozone air quality in Europe. To provide a full assessment, simulations with the global chemical transport model GEOS-CHEM driven by the NASA Goddard Institute for Space Studies general circulation model (NASA/GISS GCM) are conducted. To isolate the effects from changes in climate and anthropogenic emissions four types of simulations are performed: (1) present-day climate and emissions (2) future climate following the IPCC Special Report on Emission Scenarios (SRES) A1B scenario and present-day anthropogenic emissions of ozone precursors (3) present-day climate and future emissions and (4) future climate and future emissions. Results indicate that climate change impact on its own leads to an increase of less than 3 ppb in western and central Europe whereas decreases are evident for the rest of the areas with the highest (about 2.5 ppb) in southeastern Europe (Italy, Greece). Increases are attributed to the increases of isoprene biogenic emissions due to increasing temperatures whereas decreases are associated with the increase of water vapor over sea which tends to decrease the lifetime of ozone as well as the increased wind speeds in the 2050 climate. When future emissions are implemented in the future climate simulations, the greatest increases are seen in the southwest and southeast Mediterranean (about 16 ppb) due to the increased isoprene biogenic emissions under higher levels of NO x in the model. Decreases up to 2 ppb of ozone are shown for France, Switzerland, Northern Italy and northern Europe.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6
Fig. 7

Similar content being viewed by others

References

  • Andersson, C., & Engardt, M. (2010). European ozone in a future climate: importance of changes in dry deposition and isoprene emissions. Journal of Geophysical Research, 115, D02303. doi:10.1029/2008JD011690.

    Article  Google Scholar 

  • Auvray, M., Bey, I. (2005). Long-range transport to Europe: seasonal variations and implications for the European ozone budget. Journal of Geophysical Research: Atmospheres 110:n/a–n/a. doi: 10.1029/2004JD005503

  • Beekmann, M., & Vautard, R. (2010). A modelling study of photochemical regimes over Europe: robustness and variability. Atmospheric Chemistry and Physics, 10, 10067–10084. doi:10.5194/acp-10-10067-2010.

    Article  CAS  Google Scholar 

  • Bell, M. L., Goldberg, R., Hogrefe, C., Kinney, P. L., Knowlton, K., Lynn, B., Rosenthal, J., Rosenzweig, C., & Patz, J. A. (2007). Climate change, ambient ozone, and health in 50 US cities. Climatic Change, 82(61–76), 2007.

    Google Scholar 

  • DiCiccio, T. J., & Efron, B. (1996). Bootstrap confidence intervals. Statistical Science, 11, 189–228. doi:10.1214/ss/1032280214.

    Article  Google Scholar 

  • Directive 2008/50/EC of the European Parliament and of the Council of 21 May 2008 on ambient air quality and cleaner air for Europe (http://www.eea.europa.eu/policy-documents/directive-2008-50-ec-o).

  • Duncan, B.N., Bey, I., (2004). A modeling study of the export pathways of pollution from Europe: seasonal and interannual variations (1987–1997). Journal of Geophysical Research: Atmospheres 109:n/a–n/a. doi:10.1029/2003JD004079

  • Efron, B. (1987). Better bootstrap confidence intervals. Journal of the American Statistical Association, 82, 171. doi:10.2307/2289144.

    Article  Google Scholar 

  • Fiore, A. M., Horowitz, L. W., Purves, D. W., et al. (2005). Evaluating the contribution of changes in isoprene emissions to surface ozone trends over the eastern United States. Journal of Geophysical Research, 110, D12303. doi:10.1029/2004JD005485.

    Article  Google Scholar 

  • Forkel, R., & Knoche, R. (2006). Regional climate change and its impact on photooxidant concentrations in southern Germany: simulations with a coupled regional climate-chemistry model. Journal of Geophysical Research, 111(D12), D12302. doi:10.1029/2005JD006748.

    Article  Google Scholar 

  • Forkel, R., & Knoche, R. (2007). Nested regional climate–chemistry simulations for central Europe. Comptes Rendus Geoscience, 339(11–12), 734–746. doi:10.1016/j.crte.2007.09.018.

    Article  CAS  Google Scholar 

  • Giorgi, F., & Meleux, F. (2007). Modelling the regional effects of climate change on air quality. Comptes Rendus Geoscience, 339(11–12), 721–733. doi:10.1016/j.crte.2007.08.006.

    Article  CAS  Google Scholar 

  • Guerova, G., & Jones, N. (2007). A global model study of ozone enhancement during the August 2003 heat wave in Europe. Environmental Chemistry, 4, 285–292.

    CAS  Google Scholar 

  • Haylock, M.R., Hofstra, N., Klein Tank, A.M.G., et al. (2008). A European daily high-resolution gridded data set of surface temperature and precipitation for 1950–2006. Journal of Geophysical Research: Atmospheres 113:(D20), D20119 doi:10.1029/2008JD010201

  • Hedegaard, G. B., Brandt, J., Christensen, J. H., et al. (2008). Impacts of climate change on air pollution levels in the Northern Hemisphere with special focus on Europe and the Arctic. Atmospheric Chemistry and Physics, 8, 3337–3367. doi:10.5194/acp-8-3337-2008.

    Article  CAS  Google Scholar 

  • Hofstra N., Haylock, M., New, M., Jones, P.D., (2009). Testing E-OBS European high-resolution gridded data set of daily precipitation and surface temperature. Journal of Geophysical Research: Atmospheres 114:(D21), D21101 doi:10.1029/2009JD011799

  • Jacob, D. J., & Winner, D. A. (2009). Effect of climate change on air quality. Atmospheric Environment, 43, 51–63. doi:10.1016/j.atmosenv.2008.09.051.

    Article  CAS  Google Scholar 

  • Jacob, D. J., Logan, J. A., Gardner, G. M., et al. (1993). Factors regulating ozone over the United States and its export to the global atmosphere. Journal of Geophysical Research-Atmospheres, 98, 14817–14826. doi:10.1029/98JD01224.

    Article  Google Scholar 

  • Johnson, C. E., Collins, W. J., Stevenson, D. S., & Derwent, R. G. (1999). Relative roles of climate and emissions changes on future tropospheric oxidant concentrations. Journal of Geophysical Research, 104, 18631–18,645. doi:10.1029/1999JD900204.

    Article  CAS  Google Scholar 

  • Jonson, J. E., Simpson, D., Fagerli, H., & Solberg, S. (2006). Can we explain the trends in European ozone levels? Atmospheric Chemistry and Physics, 6, 51–66. doi:10.5194/acp-6-51-2006.

    Article  CAS  Google Scholar 

  • Katragkou, E., Zanis, P., Kioutsioukis, I., et al. (2011). Future climate change impacts on summer surface ozone from regional climate-air quality simulations over Europe. Journal of Geophysical Research, 116, D22307. doi:10.1029/2011JD015899.

    Article  Google Scholar 

  • Kostopoulou, E., Giannakopoulos, C., Hatzaki, M., & Tziotziou, K. (2012). Climate extremes in the NE Mediterranean: assessing the E-OBS dataset and regional climate simulations. Climate Research, 54, 249–270. doi:10.3354/cr01110.

    Article  Google Scholar 

  • Kyselý, J., & Plavcová, E. (2010). A critical remark on the applicability of E-OBS European gridded temperature data set for validating control climate simulations. Journal of Geophysical Research. doi:10.1029/2010JD014123.

    Google Scholar 

  • Langner, J., Bergström, R., & Foltescu, V. (2005). Impact of climate change on surface ozone and deposition of sulphur and nitrogen in Europe. Atmospheric Environment, 39, 1129–1141. doi:10.1016/j.atmosenv.2004.09.082.

    Article  CAS  Google Scholar 

  • Langner, J., Engardt, M., Baklanov, A., et al. (2012). A multi-model study of impacts of climate change on surface ozone in Europe. Atmospheric Chemistry and Physics Discussions, 12, 4901–4939. doi:10.5194/acpd-12-4901-2012.

    Article  Google Scholar 

  • Leung, L.R., Gustafson, W.I., (2005). Potential regional climate change and implications to U.S. air quality. Geophysical Research Letters 32:n/a–n/a. doi:10.1029/2005GL022911

  • Meleux, F., Solmon, F., & Giorgi, F. (2007). Increase in summer European ozone amounts due to climate change. Atmospheric Environment, 41, 7577–7587. doi:10.1016/j.atmosenv.2007.05.048.

    Article  CAS  Google Scholar 

  • Mickley, L.J., Jacob, D.J., Field, B.D., Rind, D., (2004). Effects of future climate change on regional air pollution episodes in the United States. Geophysical Research Letters 31:n/a–n/a. doi:10.1029/2004GL021216

  • Nakicenovic, N., and Swart, R., (2000). Special Report on Emissions Scenarios. A Special Report of Working Group III of the Intergovernmental Panel on Climate Change. Cambridge University Press, Cambridge, UK, 570 pp

  • Protonotariou, A. P., Tombrou, M., Giannakopoulos, C., et al. (2010). Study of CO surface pollution in Europe based on observations and nested-grid applications of GEOS-CHEM global chemical transport model. Tellus B, 62, 209–227. doi:10.1111/j.1600-0889.2010.00462.x.

    Article  Google Scholar 

  • Rasmussen, D. J., Fiore, A. M., Naik, V., et al. (2012). Surface ozone–temperature relationships in the eastern US: a monthly climatology for evaluating chemistry-climate models. Atmospheric Environment, 47, 142–153. doi:10.1016/j.atmosenv.2011.11.021.

    Article  CAS  Google Scholar 

  • Rind, D., Lerner, J., & McLinden, C. (2001). Changes of tracer distributions in the doubled CO2 climate. Journal of Geophysical Research, 106, 28061. doi:10.1029/2001JD000439.

    Article  CAS  Google Scholar 

  • Selin, N. E., Wu, S., Nam, K. M., Reilly, J. M., Paltsev, S., Prinn, R. G., & Webster, M. D. (2009). Global health and economic impacts of future ozone pollution. Environmental Research Letters, 4(4), 044014. doi:10.1088/1748-9326/4/4/044014

  • Sillman, S., & Samson, P. J. (1995). Impact of temperature on oxidant photochemistry in urban, polluted rural and remote environments. Journal of Geophysical Research-Atmospheres, 100, 11497–11508. doi:10.1029/94JD02146.

    Article  CAS  Google Scholar 

  • Smith, R. J. (2009). Use and misuse of the reduced major axis for line-fitting. American Journal of Physical Anthropology, 140(3), 476–486. doi:10.1002/ajpa.21090.

    Article  Google Scholar 

  • Streets, D.G., Bond, T.C., Lee, T., Jang, C., (2004). On the future of carbonaceous aerosol emissions. Journal of Geophysical Research: Atmospheres 109:(D24), D24212 doi:10.1029/2004JD004902

  • Varotsos, K. V., Tombrou, M., & Giannakopoulos, C., (2013). Statistical estimations of the number of future ozone exceedances due to climate change in Europe, J. Geophys. Res. Atmos., 118, doi:10.1002/jgrd.50451.

  • Vautard, R., Schaap, M., Bergström, R., et al. (2009). Skill and uncertainty of a regional air quality model ensemble. Atmospheric Environment, 43, 4822–4832. doi:10.1016/j.atmosenv.2008.09.083.

    Article  CAS  Google Scholar 

  • Wu, S., Mickley, L. J., Jacob, D. J., Logan, J. A., Yantosca, R. M., & Rind, D. (2007). Why are there large differences between models in global budgets of tropospheric ozone? Journal of Geophysical Research: Atmospheres, 112(D5), D05302. doi:10.1029/2006JD007801

  • Wu, S., Mickley, L. J., Leibensperger, E. M., Jacob, D. J., Rind, D., & Streets, D. G. (2008). Effects of 2000–2050 global change on ozone air quality in the United States. Journal of Geophysical Research: Atmospheres, 113(D6), D06302. doi:10.1029/2007JD008917

Download references

Acknowledgments

This research has been co-financed by the European Union (European Social Fund [ESF]) and Greek national funds through the Operational Program "Education and Lifelong Learning" of the National Strategic Reference Framework (NSRF) — Research Funding Program: Heracleitus II. Investing in knowledge society through the European Social Fund.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to C. Giannakopoulos.

Rights and permissions

Reprints and permissions

About this article

Cite this article

Varotsos, K.V., Giannakopoulos, C. & Tombrou, M. Assessment of the Impacts of Climate Change on European Ozone Levels. Water Air Soil Pollut 224, 1596 (2013). https://doi.org/10.1007/s11270-013-1596-z

Download citation

  • Received:

  • Accepted:

  • Published:

  • DOI: https://doi.org/10.1007/s11270-013-1596-z

Keywords

Navigation