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Assessment the Health Hazard from 222Rn in Old Metalliferous Mines in San Luis, Argentina

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Abstract

Radon levels in two old mines in San Luis, Argentina, are reported and analyzed. The radiation dose and environmental health risk of 222Rn concentrations to both guides and visitors were estimated. CR-39 nuclear track detectors were used for this purpose. The values for the 222Rn concentration at each monitoring site ranged from 0.43 ± 0.04 to 1.48 ± 0.12 kBq m−3 in the Los Cóndores wolfram mine and from 1.8 ± 0.1 to 6.0 ± 0.5 kBq·m−3 in the La Carolina gold mine, indicating that, in this mine, the radon levels exceed up to four times the action level of 1.5 kBq m−3 recommended by the International Commission on Radiological Protection. The patterns of the radon transport process revealed that the La Carolina gold mine can be interpreted as a gas confined into a single tube with constant cross-section and air velocity. Patterns of radon activity, taking into account the chimney-effect winds, were used to detect tributary currents of air from shafts or larger fissures along the main adit of the Los Cóndores mine, showing that radon can be used as an important tracer of tributary air currents stream out from fissures and smaller voids in the rock of the mine.

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References

  • Anjos, R. M., Veiga, R., Soares, T., Santos, A. M. A., Aguiar, J. G., Frascá, M. H. B. O., et al. (2005). Natural radionuclide distribution in Brazilian commercial granites. Radiation Measurements, 39, 245–253.

    Article  CAS  Google Scholar 

  • Anjos, R. M., Veiga, R., Macario, K., Carvalho, C., Sanches, N., Bastos, J., et al. (2006). Radiometric analysis of quaternary deposits from the southeastern Brazilian coast. Marine Geology, 229, 29–43.

    Article  Google Scholar 

  • Anjos, R. M., Veiga, R., Carvalho, C., Macario, K., & Gomes, P. R. S. (2007). Geological provenance of quaternary deposits from the southeastern Brazilian coast. Nuclear Physics A, 787, 642c–647c.

    Article  Google Scholar 

  • Anjos, R. M., Veiga, R., Carvalho, C., Sanches, N., Estellita, L., Zanuto, P., et al. (2008). Natural sources of radiation exposure and the teaching of radioecology. Physics Education, 43, 423–428.

    Article  Google Scholar 

  • Anjos, R. M., Macario, K. D., Lima, T. A., Veiga, R., Carvalho, C., Fernandes, P. J. F., et al. (2010). Correlations between radiometric analysis of quaternary deposits and the chronology of prehistoric settlements from the southeastern Brazilian coast. Journal of Environmental Radioactivity, 101, 75–81.

    Article  CAS  Google Scholar 

  • Atkinson, T. C., Smart, P. L., & Wigley, T. M. L. (1983). Climate and natural radon levels in Castleguard Cave, Columbia Icefields, Alberta, Canada. Arctic and Alpine, 15, 487–502.

    Article  Google Scholar 

  • Cigna, A. A. (2005). Radon in caves. International Journal of Speleology, 34, 1–18.

    Google Scholar 

  • Da Silva, A. A. R., & Yoshimura, E. M. (2005). Track analysis system for application in alpha particle detection with plastic detectors. Radiation Measurements, 39, 621–625.

    Article  Google Scholar 

  • Eappen, K. P., Mayya, Y. S., Patnaik, R. L., & Kushwaha, H. S. (2006). Estimation of radon progeny equilibrium factors and their uncertainty bounds using solid state nuclear track detectors. Radiation Measurements, 41, 342–348.

    Article  CAS  Google Scholar 

  • Estellita, L., Santos, A. M. A., Anjos, R. M., Yoshimura, E. M., Velasco, H., da Silva, A. A. R., et al. (2010). Analysis and risk estimates to workers of Brazilian granitic industries and sandblasters exposed to respirable crystalline silica and natural radionuclides. Radiation Measurements, 45, 196–203.

    Article  CAS  Google Scholar 

  • Gillmore, G. K., Phillips, P., Denman, A., Sperrin, M., & Pearce, G. (2001). Radon levels in abandoned metalliferous mines, Devon, Southwest England. Ecotoxicology and Environmental Safety, 49, 281–292.

    Article  CAS  Google Scholar 

  • Hakl, J. (1997). Application of radon-222, as a natural tracer in environmental studies. Ph.D. thesis. Lajos Kossuth University. http://ganymedes.lib.unideb.hu:8080/dea/bitstream/2437/80292/2/ertekezes.pdf

  • Hakl, J., Hunyadi, I., Csige, I., Géczy, G., Lénárt, L., & Törőcsik, I. (1992). Outline of natural radon occurences on karstic terrains of Hungary. Radiation Protection Dosimetry, 45, 183–186.

    CAS  Google Scholar 

  • Hakl, J., Csige, I., Hunyadi, I., Várhegyi, A., & Géczy, G. (1996). Radon transport in fractured porous media—Experimental study in caves. Environment International, 22, S433–S437.

    Article  CAS  Google Scholar 

  • Hakl, J., Hunyadi, I., Csige, I., Géczy, G., Lénárt, L., & Várhegyi, A. (1997). Radon transport phenomena studied in karst caves—International experiences on radon levels and exposures. Radiation Measurements, 28, 675–684.

    Article  CAS  Google Scholar 

  • Hoskold, H. D. (1904). Official Report upon the Mines, Mining, Metallurgy and Mining Laws of the Argentine Republic. Buenos Aires: Ministry of Agriculture, Commerce and Industries.

    Google Scholar 

  • Howarth, C. B., & Miles, J. C. H. (2003). NRPB Report W-44: Results of the 2002 NRPB Intercomparison of Passive Radon Detectors. Chilton: NRPB, National Radiological Protection Board.

    Google Scholar 

  • IAEA, (1987). Preparation and certification of IAEA gamma spectrometry reference materials, RGU-1, RGTh-1 and RGK-1. International Atomic Energy Agency. Report-IAEA/RL/148.

  • ICRP. (1993). International Commission on Radiological Protection, Protection Against Radon-222 at Home and at Work. ICRP Publication 65. Oxford: Pergamon.

    Google Scholar 

  • ICRP. (1994). International Commission on Radiological Protection. Human respiratory tract model for radiological protection. ICRP Publication 66. Oxford: Pergamon.

    Google Scholar 

  • ICRP, (2008). The 2007 recommendations of the international commission on radiological protection. In: ICRP Publication 103, vol. 37. Annals of the ICRP. 2–4.

  • ICRP, (2009). International Commission on Radiological Protection. International commission on radiological protection statement on radon. ICRP Ref 00/902/09. http://www.icrp.org/icrp_radon.asp.

  • Lario, J., Sánchez-Moral, S., Canaveras, J. C., Cuezva, S., & Soler, V. (2005). Radon continuous monitoring in Altamira Cave (northern Spain) to assess user’s annual effective dose. Journal of Environmental Radioactivity, 80, 161–174.

    Article  CAS  Google Scholar 

  • López de Luchi, M. G., Cerredo, M. E., Siegesmund, S., Steenken, A., & Wemmer, K. (2003). Provenance and tectonic setting of the protoliths of the Metamorphic Complexes of Sierra de San Luis. Revista de la Asociación Geológica Argentina, 58, 525–540.

    Google Scholar 

  • Miller, B. L., & Singewald, J. T. (1919). The Mineral Deposits of South America (p. 598). New York: McGraw-Hill Book Co.

    Google Scholar 

  • Nazaroff, W. W. (1992). Radon transport from soil to air. Reviews of Geophysics, 30, 137–160.

    Article  Google Scholar 

  • Orlando, C., Orlando, P., Patrizii, L., Tommasino, L., Tonnarini, S., Trevisi, R., et al. (2002). A passive radon dosemeter suitable for workplaces. Radiation Protection Dosimetry, 102, 163–168.

    CAS  Google Scholar 

  • Rastall, R. H., & Wilcockson, M. A. (1920). Tungsten ores: London, Imperial Institute Monograph on Mineral Resources with Special Reference to the British Empire, John Murray, 81 p.

  • Rogers, J. J. W., & Ragland, P. C. (1961). Variation of thorium and uranium in selected granitic rocks. Geochimica et Cosmochimica Acta, 25, 99–109.

    Article  CAS  Google Scholar 

  • Schlumberger. (1986). Log Interpretation Charts (p. 122). Houston: Schlumberger Well Services.

    Google Scholar 

  • Sharma, P. V. (1997). Environmental and Engineering Geophysics (p. 372). Cambridge: Cambridge University Press.

    Google Scholar 

  • Shweikani, R., & Durrani, S. A. (1995). Thoron contributions in radon measurements in the environments. Radiation Measurements, 25, 615–616.

    Article  CAS  Google Scholar 

  • UNSCEAR. (2000). Sources and Effects of Ionizing Radiation. United Nations: United Nations Scientific Committee on the Effects of Atomic Radiation.

    Google Scholar 

  • UNSCEAR. (2006). Effects of Ionizing Radiation—Annex E: Sources-to-Effects Assessment for Radon in Home and Workplaces. United Nations: United Nations Scientific Committee on the Effects of Atomic Radiation.

    Google Scholar 

  • Viñas, R., Eff-Darwich, A., Soler, V., Martín-Luis, M. C., Quesada, M. L., & Nuez, J. (2007). Processing of radon time series in underground environments: Implications for volcanic surveillance in the island of Tenerife, Canary Islands, Spain. Radiation Measurements, 42, 101–115.

    Article  Google Scholar 

  • Werner, A. B. T., Sinclair, W. D., & Amey, E. B. (1998). International strategic mineral issues summary report—Tungsten. US Geological Survey Circular 930-O.

  • Whitfield, J. M., Rogers, J. J. W., & Adams, J. A. S. (1959). The relationship between the petrology and the thorium and uranium contents of some granitic rocks. Geochimica et Cosmochimica Acta, 17, 248–271.

    Article  CAS  Google Scholar 

  • Wigley, T. M. L. (1967). Non-steady flow through porous medium and cave breathing. Journal of Geophysical Research, 72, 3199–3205.

    Article  Google Scholar 

Download references

Acknowledgments

The authors would like to thank the Brazilian (CNPq, PROSUL/CNPq, and FAPERJ) and Argentine (CONICET and UNSL) funding agencies for their financial support. We are grateful to workers of the La Carolina and Los Cóndores mines who assisted us with the radon measurements.

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Correspondence to R. M. Anjos.

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da Silva, A.A.R., Valladares, D.L., Anjos, R.M. et al. Assessment the Health Hazard from 222Rn in Old Metalliferous Mines in San Luis, Argentina. Water Air Soil Pollut 218, 371–386 (2011). https://doi.org/10.1007/s11270-010-0652-1

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  • DOI: https://doi.org/10.1007/s11270-010-0652-1

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