Abstract
This study focuses on fluxes of elements from, and changes in the soil properties of shallow organic material rich soil as a result of changes in precipitation acidity. Intact soil columns including natural vegetation from two areas (one exposed to acidic precipitation and one unpolluted) were used in a lysimeter experiment. The lysimeters were watered with simulated normal rain (pH 5.3) or simulated acidic rain (pH 4.3) for four years. Sulphuric acid and ammonium nitrate were used to regulate the quality of the simulated rain. Significantly more SO42− was leached from lysimeters receiving acid rain. Rain acidity had no significant effect on NO3− leaching. Significantly more Mg2+ was leached from lysimeters receiving acid rain, but this only applied for the soils from the unpolluted area. Four years of treatment did not cause any significant effect on the soil acidity and the amounts of base cations in the soil. The more acidic rain did, however, cause a significant lower cation exchange capacity. For the soils from the polluted area the acid precipitation did cause a lowering of the exchangeable K+ in the upper 5 cm of the soil. Different quality of the soil organic material indicated by different vegetation types appeared to cause significant differences in the amount of components leached from the soil, but did not cause any difference in response to the different rain qualities.
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References
Abrahamsen, G., Seip, H. M. and Semb, A.: 1989, ‘Long term acidic precipitation studies in Norway’, in D. C. Adriano and M. Havas (eds.), Acid Precipitation, Volume 1, Case Studies, pp. 137–179. Springer-Verlag, London.
Autry, A. R., Fitzgerald, J. W. and Cadwell, P. R.: 1990, ‘Sulfur fractions and retention mechanismes in forest soils’, Canadian Journal of Forest Research 20, 337–342.
Chang, F. H. and Alexander, M.: 1984, ‘Effects of simulated acid precipitation on decomposition and leaching of organic carbon in forest soils’, Soil Science 138, 226–234.
Christophersen, N., Stuanes, A. O. and Wright, R. F.: 1982, ‘Runoff chemisty at a mini-catchment watered with “unpolluted precipitation”’, Nordic Hydrology 13, 115–128.
David, M. B., Vance, G. F., Rissing, J. M. and Stevenson, F. J.: 1989, ‘Organic carbon fractions in extracts of O and B horizons from a New England Spodosol; effects of acid treatment’, Journal of Environmental Quality 18, 212–217.
de Graaf, M. C. C., Bobbink, R., Roelofs, J. G. M. and Verbeek, P. J. M.: 1998, ‘Differential effects of ammonium and nitrate on three heathland species’, Plant Ecology 135, 185–196.
FAO-Unesco: 1990, FAO/Unesco Soil Map of the World Revised Legend. 60, 1–140. ISRIC Wagningen. World Resources Reports.
Frogner, T.: 1990, ‘The effect of acid deposition on cation fluxes in artificially acidified catchments in Western Norway’, Geochimica et Cosmochimica Acta 54, 769–780.
Giesler, R., Hogberg, M. and Hogberg, P.: 1998, ‘Soil chemistry and plants in Fennoscandian boreal forest as exemplified by a local gradient’, Ecology 79, 119–137.
Giesler, R., Moldan, F., Lundstrom, U. and Hultberg, H.: 1996, ‘Reversing acidification in a forested catchment in southwestern Sweden: Effects on soil solution chemistry’, Journal of Environmental Quality 25, 110–119.
Godde, M., David, M. B., Christ, M. J., Kaupenjohann, M. and Vance, G. F.: 1996, ‘Carbon mobilization from the forest floor under red spruce in the northeastern U.S.A.’, Soil Biology and Biochemistry 28, 1181–1189.
Henriksen, A., Hindar, A., Hessen, D. O. and Kaste, ø.: 1997, ‘Contribution of nitrogen to acidity in the Bjerkreim river in Southwestern Norway’, Ambio 26, 304–311.
Hultberg, H., Dise, N. B., Wright, R. F., Andersson, I. and Nystrom, U.: 1994, ‘Nitrogen saturation induced during winter by experimental NH4 NO3 addition to a forested catchment’, Environmental Pollution 84, 145–147.
James, B. R. and Riha, S. J.: 1986, ‘pH buffering in forest soil organic horizons: Relevance to acid precipitation’, Journal of Environmental Quality 15, 229–234.
Johansson, E., Sanden, P. and Oberg, G.: 2003, ‘Spatial patterns of organic chlorine and chloride in Swedish forest soil’, Chemosphere 52, 391–397.
Kalbitz, K., Solinger, S., Park, J.-H., Michalzik, B. and Matzner, E.: 2000, ‘Controls on the dynamics of dissolved organic matter in soils: A review’, Soil Science 165, 277–304.
Kaste, O., Henriksen, A. and Hindar, A.: 1997, ‘Retention of atmospherically-derived nitrogen in subcatchments of the Bjerkreim river in southwestern Norway’, Ambio 26, 296–303.
Krug, E. C. and Isaacson, P. J.: 1984, ‘Comparison of water and dilute acid treatment on organic and inorganic chemistry of leachate from organic-rich horizons of an acid forest soil’, Soil Science 137, 370–378.
Mohren, G. M. J., Van den Burg, J. and Burger, F. W.: 1986, ‘Phosphorus deficiency induced by nitrogen input in Douglas Fir in the Netherlands’, Plant and Soil 95, 191–200.
Moldan, F., Skeffington, R. A., Morth, C. M., Torssander, P., Hultberg, H. and Munthe, J.: 2004, ‘Results from the Covered Catchment Experiment at Gardsjon, Sweden, after ten years of clean precipitation treatment’, Water Air and Soil Pollution 154, 371–384.
Moldan, F. and Wright, R. F.: 1998, ‘Episodic behaviour of nitrate in runoff during six years of nitrogen addition to the NITREX catchment at Gardsjon, Sweden’, Environmental Pollution 102, 439–444.
Nilsen, P. and Abrahamsen, G.: 2003, ‘Scots pine and Norway spruce stands responses to annual N, P, and Mg ferilization’, Forest Ecology and Management 174, 221–232.
Ogner, G., Haugen, A., Opem, M., Sjøtveit, G. and Sørlie, B.: 1984, ‘The chemical analysis program at the Norwegian Forest Research Institute’, Meddelelser fra Norsk Instiutt for Skogforskning 32, 209–232.
Rodstedth, M., Stahlberg, C., Sanden, P. and Oberg, G.: 2003, ‘Chloride imbalances in soil lysimeters’, Chemosphere 52, 381–389.
SFT The Norwegian State Pollution Control Authority.: 2001, Overvåkning av langtransportert luf og nedbør. Atmosfæriske tilførsler, 2000. (The Norwegian monitoring programme for long-range transported air pollutants. Results 2000). TA-1804/2001, 1–160.
Schecher, W. D. and Driscoll, C. T.: 1987, ‘An evaluation of uncertainties associated with aluminium equilibrium calculations’, Water Resources Research 23, 525–534.
Singh, B. R. and Johnson, D. W.: 1986, ‘Sulphate content and adsorption in soil of two forst watersheds in southern Norway’, Water Air and Soil Pollution 31, 847–856.
Singh, B. R., Abrahamsen, G. and Stuanes, A. O.: 1980, ‘Effects of simulated acid rain on sulfate movement in acid forest soils’, Soil Science Society of America Journal 44, 75–80.
Strand, L. T., Abrahamsen, G. and Stuanes, A. O.: 2002, ‘Leaching from organic matter-rich soils by rain of different qualities: I. Concentrations’, Journal of Environmental Quality 31, 547–556.
Strickland, T. C., Fitzgerald, J. W. and Swank, W. T.: 1986, ‘In situ measurements of sulfate incorporation into forest floor and soil organic matter’, Canadian Journal of Forest Research 16, 549–553.
Wesolowski, D. J. and Palmer, D. A.: 1994, ‘Alumium spesiation an equilibria and equilibria in aqueous solution: V. Gibbsite solubility at 50°C and at pH 3–9 in 0.1 molar NaCl solution (a general model of aluminum speciation; analytical methods)’, Geochimica et Cosmochimica Acta 58, 2947–2969.
Wright, R. F. and Hauhs, M.: 1990, ‘Reversibility of acidification: Soils and surface waters’, Proceedings of the Royal Society of Edinburgh Section B (Biological Sciences) 97, 191.
Wright, R. F., Gjessing, E., Christophersen, N., Lotse, E., Seip, H. M., Semb, A., Sletaune, B., Storhaug, R. and Wedum, K.: 1986, ‘Project rain: Changing acid deposition to whole catchments. The first year of treatment’, Water, Air, Soil Pollution 30, 47–63.
Wright, R. F., Lotse, E. and Semb, A.: 1988, ‘Reversibility of acidification shown by to whole-catchment experiments’, Nature (London) 334, 670–675.
Wright, R. F., Lotse, E. and Semb, A.: 1994, ‘Experimental acidification of alpine catchments at Sogndal, Norway: Results after 8 years’, Water, Air, & Soil Pollution 72, 297–315.
Wright, R. F. and Tietema, A.: 1995, ‘Ecosystem response to 9 years of nitrogen addition at Sogndal, Norway’, Forest Ecology and Management 71, 133–142.
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Strand, L.T., Abrahamsen, G. & Stuanes, A.O. Lysimeter Study on the Effects of Different Rain Qualities on Element Fluxes from Shallow Mountain Soils in Southern Norway. Water Air Soil Pollut 165, 379–402 (2005). https://doi.org/10.1007/s11270-005-7272-1
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DOI: https://doi.org/10.1007/s11270-005-7272-1