Abstract
Three different catalytic materials for NH3–SCR applications have been tested and compared in terms of activity and selectivity towards undesired products, such as N2O and NH4NO3. The selected materials were characterized by the same Cu loading and consisted of a large pore Cu–BETA catalyst and two small pore structures, a Cu–CHA and a Cu–SAPO material. The aim was to investigate the possible effect of the microporous structure of the catalyst on the SCR performances.
Similar content being viewed by others
References
Nova I, Tronconi E (2014) Urea-SCR technology for deNOx after treatment of diesel exhausts. Springer, New York
Gao F, Kwak JH, Szanyi J, Peden CH (2013) Top Catal 56:1441–1459
Kwak JH, Tonkyn RG, Kim DH, Szanyi J, Peden CH (2010) J Catal 275:187–190
H.-Y. Chen (2015) N2O Formation in the selective catalytic reduction of NOx with NH3 on zeolite supported Cu catalysts. In: 24th North American catalysis society meeting, Nam
Leistner K, Mihai O, Wijayanti K, Kumar A, Kamasamudram K, Currier NW, Yezerets A, Olsson L (2015) Catal Today 174:212–224
Wang D, Gao F, Peden CH, Li J, Kamasamudram K, Epling WS (2014) ChemCatChem 6:1579–1583
Wang J, Peng Z, Qiao H, Han L, Bao W, Chang L, Feng G, Liu W (2014) RSC Adv 4:42403–42411
Ma L, Cheng Y, Cavataio G, McCabe RW, Fu L, Li J (2013) Chem Eng J 225:323–330
Kwak JH, Tran D, Szanyi J, Peden CH, Lee JH (2012) Catal Lett 142:295–301
Wang D, Zhang L, Li J, Kamasamudram K, Epling WS (2014) Catal Today 231:64–74
Kwak JH, Varga T, Peden CH, Gao F, Hanson JC, Szanyi J (2014) J Catal 314:83–93
Kwak JH, Zhu H, Lee JH, Peden CH, Szanyi J (2012) Chem Commun 48:4758–4760
H.-Y. Chen (2014) Cu/zeolite SCR catalysts for automotive diesel NOx emission control. In: Nova I, Tronconi E (eds) Urea-SCR technology for deNOx after treatment of diesel exhausts. Springer, New York, pp 123–147
Tronconi E, Nova I, Ciardelli C, Chatterjee D, Bandl-Konrad B, Burkhardt T (2005) Catal Today 105:529–536
Nova I, Ciardelli C, Tronconi E, Chatterjee D, Bandl-Konrad B (2006) AIChE J 52:3222–3233
Colombo M, Nova I, Tronconi E (2010) Catal Today 151:223–230
Lezcano-Gonzalez I, Deka U, Arstad B, Van Yperen-De Deyne A, Hemelsoet K, Waroquier M, Van Speybroeck V, Weckhuysen BM, Beale AM (2014) Phys Chem Chem Phys 16:1639–1650
Wang D, Zhang L, Kamasamudram K, Epling WS (2013) ACS Catal 3:871–881
Colombo M, Nova I, Tronconi E (2012) Appl Catal B 111:433–444
Gao F, Walter ED, Kollar M, Wang Y, Szanyi J, Peden CH (2014) J Catal 319:1–14
Wang L, Gaudet JR, Li W, Weng D (2013) J Catal 306:68–77
VennestrØm PNR, Katernopolou A, Tiruvalam RR, Kustov A, Moses PG, Concepcion P, Corma A (2013) ACS Catal 3:2158–2161
Petitto C, Delahay G (2015) Chem Eng J 264:404–410
Grossale A, Nova I, Tronconi E, Chatterjee D, Weibel M (2009) Top Catal 52:1837–1841
Ciardelli C, Nova I, Tronconi E, Chatterjee D, Konrad B (2004) Chem Commun 23:2718–2719
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Ruggeri, M.P., Nova, I., Tronconi, E. et al. Structure–Activity Relationship of Different Cu–Zeolite Catalysts for NH3–SCR. Top Catal 59, 875–881 (2016). https://doi.org/10.1007/s11244-016-0562-6
Published:
Issue Date:
DOI: https://doi.org/10.1007/s11244-016-0562-6