Skip to main content

Advertisement

Log in

Determination of N2O Emissions Levels in the Selective Reduction of NOx by NH3 Over an On-Site-Used Commercial V2O5–WO3/TiO2 Catalyst Using a Modified Gas Cell

  • Original Paper
  • Published:
Topics in Catalysis Aims and scope Submit manuscript

Abstract

The formation of N2O in NH3–SCR deNOx reaction over an on-site-used commercial V2O5–WO3/TiO2 catalyst has been measured using an on-line IR system with a modified gas cell. The N2O could be formed by the SCR and NH3 oxidation reactions. These two reactions were particularly enhanced with the on-site-used sample.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6
Fig. 7
Fig. 8
Fig. 9
Fig. 10

Similar content being viewed by others

References

  1. Kroeze C (1994) Sci Total Environ 152:189

    Article  CAS  Google Scholar 

  2. Centi G, Perathoner S, Vazzana F (1999) Chemtech 29:48

    CAS  Google Scholar 

  3. Geraci CL Jr (1977) Anesthesia Analgesia 56:775

    Article  CAS  Google Scholar 

  4. Mattia MA (1983) Am J Nursing 1:73

    Google Scholar 

  5. Perez-Ramirez J, Kapteijn F, Bruckner A (2003) J Catal 218:234

    Article  CAS  Google Scholar 

  6. Doi K, Wu YY, Takeda R, Matsunami A, Arai N, Tagawa T, Goto S (2001) Appl Catal B 35:43

    Article  CAS  Google Scholar 

  7. Leckner B, Lyngfelt A (2002) Int J Energy Res 26:1191

    Article  CAS  Google Scholar 

  8. Becker KH, Lorzer JC, Kurtenbach R, Wiesen P, Jensen TE, Wallington TJ (1999) Environ Sci Technol 33:4134

    Article  CAS  Google Scholar 

  9. Lietti L, Nova I, Ramis G, Acqua LD, Busca G, Giamello E, Forzatti P, Bregani F (1999) J Catal 187:419

    Article  CAS  Google Scholar 

  10. Madia G, Elsener M, Koebel M, Raimondi F, Wokaun A (2002) Appl Catal B 39:181

    Article  CAS  Google Scholar 

  11. Martin JA, Yates M, Avila P, Suarez S, Blanco J (2007) Appl Catal B 70:330

    Article  CAS  Google Scholar 

  12. Yates M, Martin JA, Martin-Luengo MA, Suarez S, Blanco J (2005) Catal Today 107/108:120

    Article  Google Scholar 

  13. Suarez S, Martin JA, Yates M, Avila P, Blanco J (2005) J Catal 229:227

    Article  CAS  Google Scholar 

  14. Lietti L, Nova I, Forzatti P (2000) Top Catal 11/12:111

    Article  CAS  Google Scholar 

  15. Singoredjo L, Korver R, Kapteijn F, Moulijn J (1992) Appl Catal B 1:297

    Article  CAS  Google Scholar 

  16. Sjovall H, Olsson L, Fridell E, Blint RJ (2006) Appl Catal B 64:180

    Article  Google Scholar 

  17. Yang WH, Kim MH (2006) Korean J Chem Eng 23:908

    Article  CAS  Google Scholar 

  18. Choi JH, Kim MH, Nam IS (2005) Ind Eng Chem Res 44:707

    Article  CAS  Google Scholar 

  19. Ham SW, Nam IS (2002) In: Spivey JJ (ed) Catalysis—specialist periodical reports, vol 16. The Royal Society of Chemistry, Cambridge ch. 7

    Google Scholar 

  20. Inomata M, Miyamoto A, Murakami Y (1980) J Catal 62:140

    Article  CAS  Google Scholar 

  21. Janssen F, van der Kerkhof F, Bosch H, Ross JRH (1987) J Phys Chem 91:5921

    Article  CAS  Google Scholar 

  22. Nova I, Ciardelli C, Tronconi E, Chatterjee D, Weibel M (2007) Top Catal 42/43:43

    Article  CAS  Google Scholar 

  23. Kim MH (2007) Korean J Chem Eng 24:209

    Article  CAS  Google Scholar 

  24. Kim MH, Nam IS (2005) In: Spivey JJ (ed) Catalysis—specialist periodical reports, vol 18. The Royal Society of Chemistry, Cambridge ch. 4

    Google Scholar 

  25. Gutierrez MJF, Baxter D, Hunter C, Svoboda K (2005) Waste Manage Res 23:133

    Article  CAS  Google Scholar 

  26. Alemany LJ, Berti F, Busca G, Ramis G, Robba D, Toledo GP, Trombetta M (1996) Appl Catal B 10:299

    Article  CAS  Google Scholar 

  27. Djerad S, Crocoll M, Kureti S, Tifouti L, Weisweiler W (2006) Catal Today 113:208

    Article  CAS  Google Scholar 

  28. Kim MH, Ham SW (2009) Korean J Chem Eng (submitted)

  29. Kim KH, Lee YH, Kim MH, Ham SW, Lee SM, Lee JB (2008) In: Proceedings of 5th international conference on environmental catalysis, Belfast, Aug. 31–Sept. 3, 2008, paper # 450

  30. Lee YH, Kim MH, Ham SW (2009) In: Proceedings of 21st North American Catalysis Society meeting, San Francisco, CA, June 7–12, 2009, paper # P-M-143

  31. Feick G, Hainer RM (1954) J Am Chem Soc 76:5860

    Article  CAS  Google Scholar 

  32. Nova I, Ciardelli C, Tronconi E, Chatterjee D, Bandl-Konrad B (2006) AIChE J 52:3222

    Article  CAS  Google Scholar 

  33. Frischat GH, Czymai A (1997) Mikrochim Acta 125:79

    CAS  Google Scholar 

  34. Xia B, Li W, Zhang B, Xie Y (1999) J Mater Sci 34:3505

    Article  CAS  Google Scholar 

  35. Sussulini A, Lima AG, Figueiredo EC, Fernandes HL, Pinheiro SCL, Bueno MIMS, Pereira FMV (2009) X-ray Spectrom 38:254

    Article  CAS  Google Scholar 

  36. Busca G, Larrubia MA, Arrighi L, Ramis G (2005) Catal Today 107:139

    Article  Google Scholar 

Download references

Acknowledgement

This study was supported by a partial grant-in-aid via ETEP Grant # R-2007-1-002-0.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Moon Hyeon Kim.

Rights and permissions

Reprints and permissions

About this article

Cite this article

Kim, M.H., Ham, SW. Determination of N2O Emissions Levels in the Selective Reduction of NOx by NH3 Over an On-Site-Used Commercial V2O5–WO3/TiO2 Catalyst Using a Modified Gas Cell. Top Catal 53, 597–607 (2010). https://doi.org/10.1007/s11244-010-9493-9

Download citation

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s11244-010-9493-9

Keywords

Navigation