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Methane Oxidation over Alumina and Ceria Supported Platinum

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Abstract

Oxidation of methane over Pt/Al2O3 and Pt/CeO2 catalysts was studied by transient gas-flow reactor and in situ FTIR spectroscopy experiments. The Pt/CeO2 catalyst is generally more active, indicating more efficient CH4 dissociation, especially during oxygen pulsing, which likely is connected to the higher oxygen storage capacity/mobility of ceria.

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Acknowledgements

This work was performed within Swedish Research Council project 621-2005-3592 and the Competence Centre for Catalysis, which is financially supported by Chalmers University of Technology, the Swedish Energy Agency and the member companies: AB Volvo, Volvo Car Corporation, Scania CV AB, GM Powertrain Sweden AB, Haldor Topsøe A/S and The Swedish Space Corporation.

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Authors and Affiliations

  1. Competence Centre for Catalysis and Department of Chemical and Biological Engineering, Chalmers University of Technology, 412 96, Göteborg, Sweden

    Elin Becker, Per-Anders Carlsson & Magnus Skoglundh

Authors
  1. Elin Becker
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  2. Per-Anders Carlsson
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  3. Magnus Skoglundh
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Correspondence to Elin Becker.

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Becker, E., Carlsson, PA. & Skoglundh, M. Methane Oxidation over Alumina and Ceria Supported Platinum. Top Catal 52, 1957 (2009). https://doi.org/10.1007/s11244-009-9379-x

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  • DOI: https://doi.org/10.1007/s11244-009-9379-x

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