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Unusual supramolecular donor—acceptor complexes of bis(crown)stilbenes and bis(crown)azobenzene with viologen analogs

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Abstract

The results of the comprehensive study of novel supramolecular donor-acceptor complexes of bis(crown)stilbenes and bis(crown)azobenzene with viologen analogs are generalized. The original methodology for self-assembling of the organic donor-acceptor complexes possessing a very high thermodynamic stability is described. The hydrogen bonds between the peripheral fragments of the donor and acceptor play the key role in the self-assembling. The influence of different structural factors on the thermodynamic stability of the supramolecular donor-acceptor complexes and the efficiency of charge-transfer interactions between the donor and acceptor are discussed. The driving forces of the reaction leading to exotic trimolecular charge-transfer complexes are considered.

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Authors and Affiliations

  1. Photochemistry Center, Russian Academy of Sciences, 7A ul. Novatorov, 119421, Moscow, Russian Federation

    S. P. Gromov, A. I. Vedernikov, E. N. Ushakov & M. V. Alfimov

Authors
  1. S. P. Gromov
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  2. A. I. Vedernikov
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  3. E. N. Ushakov
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  4. M. V. Alfimov
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Correspondence to S. P. Gromov.

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Published in Russian in Izvestiya Akademii Nauk. Seriya Khimicheskaya, No. 4, pp. 779–787, April, 2008.

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Gromov, S.P., Vedernikov, A.I., Ushakov, E.N. et al. Unusual supramolecular donor—acceptor complexes of bis(crown)stilbenes and bis(crown)azobenzene with viologen analogs. Russ Chem Bull 57, 793–801 (2008). https://doi.org/10.1007/s11172-008-0118-4

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  • DOI: https://doi.org/10.1007/s11172-008-0118-4

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