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GO-P25@SA gel beads with excellent separation performance for photocatalytic degradation of rhodamine B

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Abstract

Photocatalytic treatment of water pollutants has attracted extensive attention due to its low energy consumption, low cost and the avoidance of secondary environmental pollution. However, most photocatalysts are in powder form, which makes it difficult to separate from the water system after the reaction. Especially in practical applications, the recycling of the catalyst is an important part. Based on the characteristics that sodium alginate (SA) is easy to form gels under mild conditions, GO-P25@SA gel beads were prepared. The catalyst can be separated from the water system by simple filtration, which greatly saves the recycle cost. Besides, the light response of TiO2 (P25) and excellent conductivity of graphene oxide (GO) make GO-P25@SA have excellent photocatalytic degradation and cyclic stability for rhodamine B (RhB). In this work, the unique merits of GO and sodium alginate (SA) in developing functionalized photocatalyst were demonstrated, providing a low-cost and easy recycle treatment strategy for rhodamine B degradation.

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References

  1. A. Tkaczyk, K. Mitrowska, A. Posyniak, Sci. Total Environ. 717, 137222 (2020)

    Article  CAS  Google Scholar 

  2. E. Zuccato, S. Castiglioni, R. Fanelli, J. Hazard. Mater. 122, 205 (2005)

    Article  CAS  Google Scholar 

  3. D. Cao, Y. Wang, X. Zhao, Curr. Opin. Green Sust. 6, 78 (2017)

    Article  Google Scholar 

  4. S. Kanan, M.A. Moyet, R.B. Arthur, H.H. Patterson, Catal. Rev. 62, 1 (2020)

    Article  CAS  Google Scholar 

  5. W. Deng, H. Zhao, F. Pan, X. Feng, B. Jung, A. Abdel-Wahab, B. Batchelor, Y. Li, Environ. Sci. Technol. 51, 22 (2017)

    Google Scholar 

  6. S. Zhang, B. Li, X. Wang, G. Zhao, B. Hu, Z. Lu, T. Wen, J. Chen, X. Wang, Chem. Eng. J. 390, 124642 (2020)

    Article  CAS  Google Scholar 

  7. N. Wu, H. Wei, L. Zhang, Environ. Sci. Technol. 46, 1 (2012)

    Article  Google Scholar 

  8. Y.T. Wei, Y.M. Zheng, J.P. Chen, Water Res. 45, 2297 (2011)

    Article  CAS  Google Scholar 

  9. H. Demey, T. Vincent, M. Ruiz, M. Nogueras, A.M. Sastre, E. Guibal, Chem. Eng. J. 254, 463 (2014)

    Article  CAS  Google Scholar 

  10. Y. Zhen, Z. Ning, Z. Shaopeng, D. Yayi, Z. Xuntong, S. Jiachun, Y. Weiben, W. Yuping, C. Jianqiang, ACS Appl. Mater. Inter. 7, 24446 (2015)

    Article  CAS  Google Scholar 

  11. A. Ouyang, C. Wang, S. Wu, E. Shi, W. Zhao, A. Cao, D. Wu, ACS Appl. Mater. Inter. 7, 14439 (2015)

    Article  CAS  Google Scholar 

  12. W.W. Anku, S.O.B. Oppong, S.K. Shukla, E.S. Agorku, P.P. Govender, Res. Chem. Intermediat. 42, 7231 (2016)

    Article  CAS  Google Scholar 

  13. Q. Zhou, Y. Liu, G. Yu, F. He, K. Chen, D. Xiao, X. Zhao, Y. Feng, J. Li, Polym. Degrad. Stabil. 135, 111 (2017)

    Article  CAS  Google Scholar 

  14. Y. Wang, S. Fan, Y. Li, C. Niu, X. Li, Y. Guo, J. Zhang, J. Shi, X. Wang, Int. J. Biol. Macromol. 150, 1314 (2020)

    Article  CAS  Google Scholar 

  15. M. Hosseini, M. Sarafbidabad, A. Fakhri, Z. NoorMohammadi, S. Tahami, In. J. Biol. Macromol. 118, 1494 (2018)

    Article  CAS  Google Scholar 

  16. A. Cerciello, P. Del Gaudio, V. Granata, M. Sala, R.P. Aquino, P. Russo, In. J. Biol. Macromol. 101, 100 (2017)

    Article  CAS  Google Scholar 

  17. J. Zhang, J. Ke, Y. Zhu, J. Song, J. Yang, C. Wen, L. Zhang, Biomed. Mater. 15, 015003 (2019)

    Article  Google Scholar 

  18. N. Fatin-Rouge, A. Dupont, A. Vidonne, J. Dejeu, P. Fievet, A. Foissy, Water Res. 40, 1303 (2006)

    Article  CAS  Google Scholar 

  19. Y. Gu, S. Yang, G. Zhu, Y. Yuan, Q. Qu, Y. Wang, H. Zheng, Electrochim. Acta 269, 405 (2018)

    Article  CAS  Google Scholar 

  20. M. Hasanpour, M. Hatami, Adv. Colloid Interfac. 284, 102247 (2020)

    Article  CAS  Google Scholar 

  21. S.J. Wang, H. Bu, H.J. Chen, T. Hu, W.Z. Chen, J.H. Wu, H.J. Hu, M.Z. Lin, Y. Li, G.B. Jiang, Chem. Eng. J. 399, 125760 (2020)

    Article  CAS  Google Scholar 

  22. Q. Dong, J. Wang, X. Duan, X. Tan, S. Liu, S. Wang, Chem. Eng. J. 369, 1049 (2019)

    Article  CAS  Google Scholar 

  23. Y.G. Shul, H.J. Kim, S.J. Haam, H.S. Han, Res. Chem. Intermediat. 29, 849 (2003)

    Article  CAS  Google Scholar 

  24. I. Willner, Y. Eichen, B. Willner, Res. Chem. Intermediat. 20, 681 (1994)

    Article  CAS  Google Scholar 

  25. K. Singh, S. Harish, A.P. Kristy, V. Shivani, J. Archana, M. Navaneethan, M. Shimomura, Y. Hayakawa, Appl. Surf. Sci. 449, 755 (2018)

    Article  CAS  Google Scholar 

  26. C. Feng, L. Zhang, Z. Cheng, ChemistrySelect 5, 2142 (2020)

    Article  CAS  Google Scholar 

  27. P. Ren, M. Song, J. Lee, J. Zheng, Z. Lu, M. Engelhard, X. Yang, X. Li, D. Kisailus, D. Li, Adv. Mater. Interfaces 6, 1901121 (2019)

    Article  Google Scholar 

  28. F. Zou, J. Hu, W. Miao, Y. Shen, J. Ding, X. Jing, ACS Omega 5, 28510 (2020)

    Article  CAS  Google Scholar 

  29. S. Pu, R. Zhu, H. Ma, D. Deng, X. Pei, F. Qi, W. Chu, Appl. Catal. B-Environ. 218, 208 (2017)

    Article  CAS  Google Scholar 

  30. Y. Ide, N. Inami, H. Hattori, K. Saito, M. Sohmiya, N. Tsunoji, K. Komaguchi, T. Sano, Y. Bando, D. Go-lberg, Y. Sugahara, Angew. Chem. Int. Edit. 55, 3600 (2016)

    Article  CAS  Google Scholar 

  31. M. Sabbaghan, H. Charkhan, M. Ghalkhani, J. Beheshtian, Res. Chem. Intermediat. 45, 487 (2019)

    Article  CAS  Google Scholar 

  32. L.J. Luo, J. Li, J. Dai, L. Xia, C.J. Barrow, H. Wang, J. Jegatheesan, M. Yang, Process Saf. Environ. 112, 274 (2017)

    Article  CAS  Google Scholar 

  33. R.S. Das, S.K. Warkhade, A. Kumar, A.V. Wankhade, Res. Chem. Intermediat. 45, 1689 (2019)

    Article  CAS  Google Scholar 

  34. M. Fathizadeh, W.L. Xu, F. Zhou, Y. Yoon, M. Yu, Adv. Mater. Interfaces 4, 1600918 (2017)

    Article  Google Scholar 

  35. H. Yu, Y. He, G. Xiao, Y. Fan, J. Ma, Y. Gao, R. Hou, J. Chen, J. Mater. Sci. Technol. 39, 106 (2020)

    Article  Google Scholar 

  36. X. Ming, A. Guo, Q. Zhang, Z. Guo, F. Yu, B. Hou, Y. Wang, K.P. Homewood, X. Wang, Carbon 167, 285 (2020)

    Article  CAS  Google Scholar 

  37. W.L. Xu, C. Fang, F. Zhou, Z. Song, Q. Liu, R. Qiao, M. Yu, Nano Lett. 17, 5 (2017)

    Google Scholar 

  38. H. Ha, C.J. Ellison, Korean J. Chem. Eng. 35, 303 (2018)

    Article  CAS  Google Scholar 

  39. C. Yao, X. Wang, W. Zhao, T. Li, Y. He, X. Ran, L. Guo, J. Alloy Compd 846, 156335 (2020)

    Article  CAS  Google Scholar 

Download references

Acknowledgements

This work was supported by the National Natural Science Foundation of China (21673073, 21677048 and 5171101651), Shanghai Municipal Science and Technology Major Project (Grant No.2018SHZDZX03) and the Programme of Introducing Talents of Discipline to Universities (B16017), the Science and Technology Commission of Shanghai Municipality (16JC1401400, 17520711500) and the Fundamental Research Funds for the Central Universities (222201717003).

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Correspondence to Lingzhi Wang.

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Gong, J., He, C., Zhang, J. et al. GO-P25@SA gel beads with excellent separation performance for photocatalytic degradation of rhodamine B. Res Chem Intermed 47, 2331–2338 (2021). https://doi.org/10.1007/s11164-021-04403-z

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