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Saturated absorption and nonlinear refraction of silicate glasses doped with silver nanoparticles at 532 nm

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Abstract

The nonlinear optical characteristics of silicate glasses doped with silver nanoparticles are investigated by Z-scan technique using second harmonic radiation of picosecond Nd:YAG laser (λ=532 nm, τ=55 ps). The real and imaginary parts of third-order nonlinear susceptibility of silver-contained glasses were measured. It was found that the sign of Imχ (3)was negative due to saturated absorption and the sign of Reχ (3) was changed from negative (self-defocusing) to positive (self-focusing) with growth of laser radiation intensity. The mechanisms responsible for saturated absorption and nonlinear refraction are discussed.

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Ganeev, R., Ryasnyansky, A., Stepanov, A. et al. Saturated absorption and nonlinear refraction of silicate glasses doped with silver nanoparticles at 532 nm. Optical and Quantum Electronics 36, 949–960 (2004). https://doi.org/10.1007/s11082-004-3392-x

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