Abstract
The presence of underlying uranium deposits may contaminate the upper soil of a region. We have carried out a detailed investigation of radionuclides (Ra, Th, and K) present in the soil around the reported uranium deposit site in the Sikar district of Rajasthan, India. Measurements are carried out using the state-of-the-art gamma-ray spectroscopy (HPGe detector) technique. The specific activity of 226Ra, 232Th, and 40K are found in the range of 9.5 ± 0.5–50.6 ± 1.0 Bq kg−1, 11.0 ± 0.4–83.2 ± 1.5 Bq kg−1, and 177 ± 13–753 ± 47 Bq kg−1 with the mean values of 17.8 ± 7.5 Bq kg−1, 22.6 ± 13.4 Bq kg−1, and 393 ± 76 Bq kg−1 respectively. The average value of Ra Eq. activity is 80.4 Bq kg−1, below the recommended limit of 370 Bq kg−1. For radiological implications in the study area, the indoor and outdoor absorbed dose rates and age-dependent annual effective dose are estimated, which are also found below their prescribed safe limit values. The mean value of other hazard indices (Hin and Hex) and level indices (Iα and Iγ) are less than unity. Our study shows that the underlying uranium deposits do not contaminate the soil of the studied area and the soil is safe to use for various purposes.
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References
Mathur AK, Gupta M, Varshney R, Sonkawade RG, Verma KD, Prasad R (2013) Radon exhalation and gamma radioactivity levels in soil and radiation hazard assessment in the surrounding area of National Thermal Power Corporation, Dadri (U.P.), India. Radiat Meas 50:130–135
Radhakrishna AP, Somasekarapa HM, Narayana Y, Siddappa K (1993) A new natural background radiation area on the southwest coast of India. Health Phys 65:390–395
Duggal V, Rani A, Mehra R, Ramola RC (2014) Assessment of natural radioactivity levels and associated dose rates in soil samples from Northern Rajasthan, India. Radiat Prot Dosim 158:235–240
UNSCEAR (2000) Sources and effects of ionizing radiation. United Nations Scientific Committee on the effects of atomic radiation report to the general assembly, with scientific annexes, v. I
Chikasawa K, Ishii T, Ugiyama H (2001) Terrestrial gamma radiation in Kochi prefecture, Japan. J Health Sci 47:361–372
Environmental Protection Agency, (EPA, 2007) (2007) United States. Ionizing radiation fact book. EPA. Office of radiation and indoor air. EPA-402-F-06e061
Srilatha MC, Rangaswamy DR, Sannappa J (2015) Measurement of natural radioactivity and radiation hazard assessment in the soil samples of Ramanagara and Tumkur districts, Karnataka, India. J Radioanal Nucl Chem 303:993–1003
Henshaw DL, Eatough JP, Richardson RB (1990) Radon as a causative factor in induction of myeloid leukaemia and other cancers. Lancet 335:1008–1012
Hassan NM, Mansour NA, Fayez-Hassan M (2017) Assessment of radiation hazards due to exposure to radionuclides in marble and ceramic commonly used as decorative building materials in Egypt. Indoor Built Environ 26(3):317–326
International Commission on Radiological Protection (ICRP) (1991) 1990 recommendation of the International Commission on radiological protection. Pergamon Press, Oxford. ICRP publication 60, Annal of the ICRP 21:1–3
Mehra R, Kaur S, Chand S, Charan C, Mehta M (2021) Dosimetric assessment of primordial radionuclides in soil and groundwater of Sikar district, Rajasthan. J Radioanal Nucl Chem 330:1605–1620
Mehra R, Singh S, Singh K, Sonkawade R (2007) 226Ra, 232Th and 40K analysis in soil samples from some areas of Malwa region, Punjab, India using gamma ray spectrometry. Environ Monit Assess 134:333–342
Ravisankar R, Chandrasekaran A, Vijayagopal P, Venkatraman B, Senthilkumar G, Eswaran P, Rajalakshmi A (2012) Natural radioactivity in soil samples of Yelagiri Hills, Tamil Nadu, India and the associated radiation hazards. Radiat Phys Chem 81(12):1789–1795
Dusane CB, Mishra S, Sahu SK, Pandit GG (2014) Distribution of 238U, 226Ra, 232Th and 40K in soil samples around Tarapur, India. J Radioanal Nucl Chem 302:1435–1440
Kumar M, Kumar P, Prajith R, Agrawal A, Sahoo BK (2022) Radon exhalation potential and natural radioactivity in soil collected from the surrounding area of a thermal power plant. J Radioanal Nucl Chem 331(6):2597–2607
Yadav M, Prasad M, Dutt S, Ramola RC (2022) Variation of natural radioactivity in soil and water samples of Garhwal Himalaya, India. J Radioanal Nucl Chem 331(4):1951–1958
Lotfalinezhad P, Kashian S, Kotahi MS, Fathivand AA (2017) Estimation of natural radioactivity and radiation exposure in environmental soil samples of Golestan, Iran. Iran J Med Phys 14(2):98–103
Degerlier M, Karahan G, Ozger G (2008) Radioactivity concentrations and dose assessment for soil samples around Adana, Turkey. J Environ Radioact 99:1018–1025
Joel ES, Maxwell O, Adewoyin OO, Olawole OC, Arijaje TE, Embong Z, Saeed MA (2019) Investigation of natural environmental radioactivity concentration in soil of coastaline area of Ado-Odo/Ota Nigeria and its radiological implications. Sci Rep 9(1):4219
Navas A, Gaspar L, López-Vicente M, Machín J (2011) Spatial distribution of natural and artificial radionuclides at the catchment scale (South Central Pyrenees). Radiat Meas 46(2):261–269
Abojassim AA, Rasheed LH (2021) Natural radioactivity of soil in the Baghdad governorate. Environ Earth Sci 80:1–13
Alasadi LA, Abojassim AA (2022) Mapping of natural radioactivity in soils of Kufa districts, Iraq using GIS technique. Environ Earth Sci 81(10):279
Ugbede FO, Osahon OD, Akpolile AF (2022) Natural radioactivity levels of 238U, 232Th and 40K and radiological risk assessment in paddy soil of Ezillo rice fields in Ebonyi State, Nigeria. Environ Forensics 23(1–2):32–46
Yang J, Sun Y (2022) Natural radioactivity and dose assessment in surface soil from Guangdong, a high background radiation province in China. J Radiat Res Appl Sci 15(1):145–151
Hamidalddin S (2022) Measurement of natural radiation, calculation of radiation doses of agricultural environmental samples in the western region-Kingdom of Saudi Arabia. J Radiat Res Appl Sci 15(1):69–74
Ion A, Cosac A, Ene VV (2022) Natural radioactivity in soil and radiological risk assessment in Lișava Uranium Mining Sector, Banat Mountains, Romania. Appl Sci 12(23):12363
Saleh MA, Ramli AT, Alajerami Y, Aliyu AS (2013) Assessment of natural radiation levels and associated dose rates from surface soils in Pontian district, Johor, Malaysia. J Ovonic Res 9(1):17–27
Rao N, Bhati SS, Rama Seshu P, Reddy AR (1996) Natural radioactivity in soil and radiation levels of Rajasthan. Radiat Prot Dosim 63(3):207–216
Uranium Corporation of India Limited (UCIL): 54th annual report, 2020–2021. https://ucil.gov.in/pdf/report/Final%20AR%20English.pdf
UCIL: Pre-feasibility report of Rohil Uranium Project of UCIL. https://environmentclearance.nic.in/writereaddata/Online/TOR/18_Nov_2017_185020967R3597Z9LPFR.pdf
Khyalia B, Kumar N, Beniwal R, Panghal A, Kataria N, Gautam P, Dalal R (2023) Assessment of age-dependent radiation dose and toxicological risk of uranium in ground water around uranium mines in Sikar, Rajasthan, India. J Pure Appl Phys 61:874–885
Groundwater Department Rajasthan: Hydrological atlas of Rajasthan Sikar District (2013). https://phedwater.rajasthan.gov.in/content/dam/doitassets/water/Ground%20Water/Pdf/PublicReports/Groundwater_Atlas/Districts/Districtwise%20Atlas%20-%20Sikar.pdf
Daulta R, Garg VK, Singh B (2019) Natural radioactivity in soil, associated radiation exposure and cancer risk to population of Eastern Haryana, India. J Geo Soc India 94:525–532
Ademola AK, Bello AK, Adejumobi AC (2014) Determination of natural radioactivity and hazard in soil samples in and around gold mining area in Itagunmodi, south-western, Nigeria. J Radiat Res Appl Sci 7(3):249–255
UNSCEAR (2008) Sources and effects of ionizing radiation, United Nations Scientific Committee on the effects of atomic radiation, annex B exposures of the public and workers from various sources of radiation. Exposure from natural sources of radiation, vol I. United Nations, New York
United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR) (1982) Ionizing radiation: sources and biological effects. Report of the general assembly, with annexes, United Nations, New York
Arafa W (2004) Specific activity and hazards of granite samples collected from the Eastern Desert of Egypt. J Environ Radioact 75:315–322
EC (1999) Radiological protection principles concerning the natural radioactivity of building materials. Radiation Protection 112, Directorate-General, Environment, Nuclear Safety and Civil Protection, European Commission, Luxembourg
Jain SC, Mehta SC, Kumar B (1995) Formulation of the reference Indian adult: anatomic and physiological data. Health Phys 68(4):509–522
Kumari P, Kumar G, Prasher S, Kumar M, Mehra R, Kaur S (2020) Determination of terrestrial radionuclides and related radiological risks in the soils from Pangi Valley of Chamba, Himachal Pradesh, India. In: Journal of Physics: Conference Series, vol 1531, no 1, p 012035. IOP Publishing
Brahmanandhan G, Selvasekarapandian S, Malathi J, Khanna D, Rajan M, Hegde A (2007) Natural radioactivity in the soil samples in and around Kudankulam nuclear power plant site. J Radioanal Nucl Chem 274(2):361–366
Karunakara N, Yashodhara I, Kumara KS, Tripathi RM, Menon SN, Kadam S, Chougaonkar MP (2014) Assessment of ambient gamma dose rate around a prospective uranium mining area of South India—a comparative study of dose by direct methods and soil radioactivity measurements. Results Phys 4:20–27
Levinson S, Lavi N, Nasar H, German U (2014) Radioactivity in soils and foodstuff samples in Israel
Taskin H, Karavus MELDA, Ay P, Topuzoglu AHMET, Hidiroglu SEYHAN, Karahan G (2009) Radionuclide concentrations in soil and lifetime cancer risk due to gamma radioactivity in Kirklareli, Turkey. J Environ Radioact 100(1):49–53
Hassan NM, Kim YJ, Jang J, Chang BU, Chae JS (2018) Comparative study of precise measurements of natural radionuclides and radiation dose using in-situ and laboratory γ-ray spectroscopy techniques. Sci Rep 8(1):14115
El-Gamal H, Farid MEA, Abdel Mageed AI, Hasabelnaby M, Hassanien HM (2013) Assessment of natural radioactivity levels in soil samples from some areas in Assiut, Egypt. Environ Sci Pollut Res 20:8700–8708
NEA-OECD (1979) Exposure to radiation from natural radioactivity in building materials. Report by NEA group of experts of the nuclear energy agency. OECD, Paris
Prasad M, Ranga V, Kumar GA, Ramola RC (2020) Radiological impact assessment of soil and groundwater of Himalayan regions in Uttarakhand, India. J Radioanal Nucl Chem 323:1269–1282
Kumar A, Sharma S, Mehra R, Mishra R, Taloor AK, Bhattacharya P (2022) Assessment of natural radioactivity levels in the Lesser Himalayas of the Jammu and Kashmir, India. J Radioanal Nucl Chem 331(4):1907–1921
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Bhupesh Khyalia's research work is supported by the research grant (Junior Research Fellowship) of the University Grant Commission (UGC) of India.
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Khyalia, B., Yadav, J., Kumar, N. et al. Estimation of radionuclides in the soil samples from the uranium mining zone of Sikar, Rajasthan, India. J Radioanal Nucl Chem (2024). https://doi.org/10.1007/s10967-024-09386-w
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DOI: https://doi.org/10.1007/s10967-024-09386-w