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Assessment of tritium monitoring for radiation environment around the typical nuclear power plants in China

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Abstract

During the conventional operation, nuclear power plants discharge waste water containing amount of radioactivity, one of main ingredient is the artificial radionuclide tritium. In this paper, the chemical characteristics and the level of tritium in the environment are studied. The monitoring medium and results of tritium in eight typical nuclear power plants are described. According to the monitoring data, the emission of tritium in heavy water reactor is relatively high, while that in pressurized water reactor is basically at the background level. Tips on topics related to strengthen the monitoring of radiation environment around the nuclear power plants have noted.

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References

  1. Liang J, Cheng W-y (2022) Annual variation of different forms of tritium in the soil around Qinshan Nuclear Power Plant. J Environ Radioact 251–252:106957. https://doi.org/10.1016/j.jenvrad.2022.106957

    Article  CAS  PubMed  Google Scholar 

  2. Guo F (2020) Distribution of tritium concentration in the 0–25 cm surface soil of cultivated and uncultivated soil around the Qinshan nuclear power plant in China. Appl Radiat Isot 164:109311. https://doi.org/10.1016/j.apradiso.2020.109311

    Article  CAS  PubMed  Google Scholar 

  3. Köllő Z, Palcsu L, Major Z, Papp L, Molnár M, Ranga T, Dombóvári P, Manga LL (2011) Experimental investigation and modelling of tritium washout by precipitation in the area of the nuclear power plant of Paks, Hungary. J Environ Radioact 102:53–59. https://doi.org/10.1016/j.jenvrad.2010.09.002

    Article  CAS  PubMed  Google Scholar 

  4. Hirao S, Kakiuchi H (2021) Investigation of atmospheric tritiated water vapor level around the Fukushima Daiichi nuclear power plant. Fusion Eng Des 171:112556. https://doi.org/10.1016/j.fusengdes.2021.112556

    Article  CAS  Google Scholar 

  5. Zhao C (2021) Transport and dispersion of tritium from the radioactive water of the Fukushima Daiichi nuclear plant. Mar Pollut Bull 169:112515. https://doi.org/10.1016/j.marpolbul.2021.112515

    Article  CAS  PubMed  Google Scholar 

  6. de Carvalho Gomes F (2014) Tritium (3H) as a tracer for monitoring the dispersion of conservative radionuclides discharged by the Angra dos Reis nuclear power plants in the Piraquara de Fora Bay. J Environ Radioact 136:169–173. https://doi.org/10.1016/j.jenvrad.2014.05.022

    Article  CAS  PubMed  Google Scholar 

  7. Uda T (2010) Detection efficiency of plastic scintillator for gaseous tritium sampling and measurement system. Fusion Eng Des 85:1474–1478. https://doi.org/10.1016/j.fusengdes.2010.04.019

    Article  CAS  Google Scholar 

  8. Röllig M, Ebenhöch S, Niemes S, Priester F, Sturm M (2015) Development of a compact tritium activity monitor and first tritium measurements. Fusion Eng Des 100:177–180. https://doi.org/10.1016/j.fusengdes.2015.05.056

    Article  CAS  Google Scholar 

  9. Jang KW (2011) Fiber-optic radiation sensor for detection of tritium. Nucl Instrum Methods Phys Res Sect A Accel Spectrom Detect Assoc Equip 652:928–931. https://doi.org/10.1016/j.nima.2010.09.060

    Article  CAS  Google Scholar 

  10. Li G (2020) RO film-based pretreatment method for tritium determination by LSC. Appl Radiat Isot 166:109343. https://doi.org/10.1016/j.apradiso.2020.109343

    Article  CAS  PubMed  Google Scholar 

  11. Dove A (2021) Tritium in Laurentian Great Lakes surface waters. J Great Lakes Res 47:1458–1463. https://doi.org/10.1016/j.jglr.2021.06.007

    Article  Google Scholar 

  12. Iraola E (2021) SMART_TC: an R&D Programme on uses of artificial intelligence techniques for tritium monitoring in complex ITER-like tritium plant systems. Fusion Eng Des 166:112409. https://doi.org/10.1016/j.fusengdes.2021.112409

  13. Aoyama T (1989) A new type of tritium-in-air monitor for fusion reactors. Fusion Eng Des 10:423–427. https://doi.org/10.1016/0920-3796(89)90087-2

    Article  Google Scholar 

  14. Röllig M (2013) Activity monitoring of a gaseous tritium source by beta induced X-ray spectrometry. Fusion Eng Des 88:1263–1266. https://doi.org/10.1016/j.fusengdes.2012.11.001

    Article  CAS  Google Scholar 

  15. Tanaka M (2017) Development of an active tritium sampler for discriminating chemical forms without the use of combustion gases in a fusion test facility. Appl Radiat Isot 125:53–59. https://doi.org/10.1016/j.apradiso.2017.03.028

    Article  CAS  PubMed  Google Scholar 

  16. Tanaka M (2021) Estimation of tritium inventory in exhaust detritiation system for fusion test device in the initial tritium recovery operation. Fusion Eng Des 172:112808. https://doi.org/10.1016/j.fusengdes.2021.112808

  17. Higgy RH (1998) Natural and man-made radioactivity in soils and plants around the research reactor of Inshass. Appl Radiat Isot 49:1709–1712. https://doi.org/10.1016/S0969-8043(98)00009-8

    Article  CAS  PubMed  Google Scholar 

  18. Singh AN (1995) A fast responding tritium in air monitor for use in operational areas of heavy water power reactors. Nucl Instrum Methods Phys Res Sect A Accel Spectrom Detect Assoc Equip 357:601–604. https://doi.org/10.1016/0168-9002(94)01738-7

    Article  CAS  Google Scholar 

  19. Shu WM (2004) Characteristics of a promising tritium process monitor detecting bremsstrahlung X-rays. Nucl Instrum Methods Phys Res Sect A Accel Spectrom Detect Assoc Equip 521:423–429. https://doi.org/10.1016/j.nima.2003.10.110

    Article  CAS  Google Scholar 

  20. Wampler WR (1994) Low-energy beta spectroscopy using pin diodes to monitor tritium surface contamination. Nucl Instrum Methods Phys Res Sect A Accel Spectrom Detect Assoc Equip 349:473–480. https://doi.org/10.1016/0168-9002(94)91213-0

    Article  CAS  Google Scholar 

  21. Anh HL (2018) Monitoring of tritium concentration in Hanoi’s precipitation from 2011 to 2016. J Environ Radioact 192:143–149. https://doi.org/10.1016/j.jenvrad.2018.06.009

    Article  CAS  PubMed  Google Scholar 

  22. Shu WM (2006) Monitoring of tritium in diluted gases by detecting bremsstrahlung X-rays. Fusion Eng Des 81:803–808. https://doi.org/10.1016/j.fusengdes.2005.05.006

    Article  CAS  Google Scholar 

  23. Dolan K (2021) Tritium generation, release, and retention from in-core fluoride salt irradiations. Prog Nucl Energy 131:103576. https://doi.org/10.1016/j.pnucene.2020.103576

  24. Tanaka M (2008) Performance of the electrochemical hydrogen pump of a proton-conducting oxide for the tritium monitor. Fusion Eng Des 83:1414–1418. https://doi.org/10.1016/j.fusengdes.2008.06.038

    Article  CAS  Google Scholar 

  25. Loughlin MJ (2007) Tritium monitoring in the ITER neutral beam test facility. Fusion Eng Des 82:646–651. https://doi.org/10.1016/j.fusengdes.2007.07.008

    Article  CAS  Google Scholar 

  26. Li S (2021) Assessment of supervision monitoring for radiation environment around the typical research reactors in China. Nucl Eng Technol 53:4150–4157. https://doi.org/10.1016/j.net.2021.06.032

    Article  CAS  Google Scholar 

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Acknowledgements

This work was supported by the logistics open research project (Grant Number BY221C014220719016).

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Correspondence to Xianyun Ai.

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Li, S., Ai, X., Yu, Z. et al. Assessment of tritium monitoring for radiation environment around the typical nuclear power plants in China. J Radioanal Nucl Chem 332, 2581–2588 (2023). https://doi.org/10.1007/s10967-023-08939-9

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