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Effect of gamma window setting on activity measurement of 134Cs by 4πβ(LS)-γ coincidence method

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Abstract

The complex decay scheme of 134Cs allows the activity measurement of the nuclide by the 4πβ(LS)-γ coincidence method to be performed at different γ-window settings. This paper describes the activity measurement of 134Cs by 4πβ (LS)-γ coincidence method based on five γ-window settings. The use of different γ-window settings affects the efficiency curve used to determine the activity value. The possible sources that are affecting the efficiency function are discussed. Despite the different efficiency functions obtained from the five γ-windows, a linear extrapolation can be performed by limiting the fitting range within the highest efficiency range. The results show that the specific activity value of each setting is differed by less than 0.3%, with the mean activity value of (1145.6 ± 4.4) kBq/g at the reference time. The quoted uncertainty is evaluated at k = 1.

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References

  1. Sochorová J, Auerbach P (2014) Activity standardization of 134Cs and 137Cs. Appl Radiat Isot 87:207–210. https://doi.org/10.1016/j.apradiso.2013.11.127

    Article  CAS  PubMed  Google Scholar 

  2. Kossert K, Marganiec-Gałązka J, Nähle OJ (2017) Primary activity standardization of134Cs. J Radioanal Nucl Chem 314:545–553. https://doi.org/10.1007/s10967-017-5338-3

    Article  CAS  Google Scholar 

  3. Nedjadi Y, Bailat CJ, Bochud FO (2012) Primary activity measurements with a 4πΒ-4πγ coincidence counting system. Appl Radiat Isot 70:249–256. https://doi.org/10.1016/j.apradiso.2011.07.017

    Article  CAS  PubMed  Google Scholar 

  4. da Silva CJ, da Cruz PAL, Iwahara A et al (2018) 134Cs activity standardization by 4πβ(LS)-γ(NaI-Tl) anticoincidence counting and submission to international reference system. Appl Radiat Isot 134:316–320. https://doi.org/10.1016/j.apradiso.2017.10.025

    Article  CAS  PubMed  Google Scholar 

  5. García-Torao E, Barquero LR, Roteta M (2002) Standardization of 134Cs by three methods. Appl Radiat Isot 56:211–214. https://doi.org/10.1016/S0969-8043(01)00190-7

    Article  Google Scholar 

  6. van Rooy MW, van Staden MJ, Lubbe J, Simpson BRS (2016) Activity determination of59Fe by 4π beta-gamma counting using liquid scintillation in the beta channel. Appl Radiat Isot 109:276–280. https://doi.org/10.1016/j.apradiso.2015.11.054

    Article  CAS  PubMed  Google Scholar 

  7. Yunoki A, Sato Y, Joseph L et al (2020) Report of APMP comparison of the activity measurements of Fe-59 (APMP.RI(II)-K2.Fe-59). Metrologia 57:1–17. https://doi.org/10.1088/0026-1394/57/1A/06002

    Article  Google Scholar 

  8. Marganiec-Gałązka J, Nähle OJ, Kossert K (2017) Activity determination of 88Y by means of 4πβ(LS)-γ coincidence counting. J Radioanal Nucl Chem 314:599–604. https://doi.org/10.1007/s10967-017-5411-y

    Article  CAS  Google Scholar 

  9. Cessna JT, Fitzgerald R, Zimmerman BE et al (2018) Results of an international comparison of activity measurements of 68 Ge. Appl Radiat Isot 134:385–390. https://doi.org/10.1016/j.apradiso.2017.10.052

    Article  CAS  PubMed  Google Scholar 

  10. International Commission on Radiation Units and Measurements, ICRU (1994) Particle counting in radioactivity measurements. 52:44–46. https://doi.org/10.1093/jicru/os27.1.Report52

  11. Lee KB, Lee JM, Park TS, Lee SH (2010) Development of a high-efficiency 4πβ(LS)-γ coincidence system for direct measurements of activity in radioactive decay. IEEE Trans Nucl Sci 57:2613–2616. https://doi.org/10.1109/TNS.2010.2040753

    Article  CAS  Google Scholar 

  12. Lee KB, Lee JM, Park TS et al (2011) Application of digital sampling techniques for 4πβ (LS) γ coincidence counting. Nucl Instruments Methods Phys Res Sect A Accel Spectrometers, Detect Assoc Equip 626–627:72–76. https://doi.org/10.1016/j.nima.2010.10.091

    Article  CAS  Google Scholar 

  13. Baerg AP (1973) The efficiency extrapolation method in coincidence counting. Nucl Instrum Methods 112:143–150. https://doi.org/10.1016/0029-554X(73)90788-X

    Article  CAS  Google Scholar 

  14. Yunoki A, Kawada Y, Hino Y (2016) Improvements of the standardization of 134Cs by the critical window setting for 605 keV photopeak. Appl Radiat Isot 109:374–377. https://doi.org/10.1016/j.apradiso.2015.12.011

    Article  CAS  PubMed  Google Scholar 

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Acknowledgements

The authors would like to thank the Korea Research Institute of Standards and Science (KRISS) for supporting this research activity.

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Correspondence to Kyoung Beom Lee.

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Agusbudiman, A., Lee, K.B., Lee, J.M. et al. Effect of gamma window setting on activity measurement of 134Cs by 4πβ(LS)-γ coincidence method. J Radioanal Nucl Chem 330, 539–545 (2021). https://doi.org/10.1007/s10967-021-07803-y

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  • DOI: https://doi.org/10.1007/s10967-021-07803-y

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