Abstract
Measurements of the cross-section for the 122Te(n,2n)121mTe and 122Te(n,2n)121gTe reactions and their ratio within the energy range of 13 –5 MeV have been carried out using the method of activation and off-line γ-ray spectrometry. The fast-moving neutrons were produced via the 3H(d,n)4He reaction on a K-400 neutron generator. Natural high-purity Te powder was used as the target material. The value of pure ground-state cross-section σg was obtained. Theoretical excitation functions were also calculated by means of the nuclear-reaction codes TALYS-1.95 with six level densities, at neutron energies varying from the reaction threshold to 20 MeV. The results were also discussed and compared with some of the corresponding values found in the literature.
Similar content being viewed by others
References
Bormann M, Bissen HH, Magiera E, Warnemunde R (1970) Total cross sections and isomeric cross section rations for (n,2n) reactions in the energy region 12–18 MeV. Nucl Phys A 157:481
Brzosko J, Decowski P, Siwek-diament K, Wilhelmi Z (1965) Isomeric cross section for the 130Te(n,2n)129Te reaction. Nucl Phys 74:438
Majumdar NK, Chatterjee A (1963) 14.8 MeV neutron activation cross-section measurements of a few tellurium isotopes. Nucl Phys 41:192
Bonazzola GC, Brovetto P, Chiavassa E, Spinoglio R, Pasquarelli A (1964) The measurement by activation of cross sections for 14.7 MeV neutrons. Nucl Phys 51:337
Hasan SS, Prasad R, Seghal ML (1972) The 14.8MeV neutron cross sections for enriched isotopes of Se-82, Mo-92, Sn-117, Te-128 and Te-130. Nucl Phys A 181:101
Levkovskiy VN, Artem’ev OI (1971) Cross-sections of reactions (n, p) and (n, α) at the neutron energy 14.8 MeV. Yad Fiz 13:923
Struwe W, Winkler G (1974) Measurement of (n, p) cross sections on isotopes of Cd, Sn and Te for 14 MeV neutrons. Nucl Phys A 222:605
Brzosko J, Decowski P, Siwek-diament K, Wilhelmi Z (1963) Isomeric cross section for (n, p) reactions in Sn and Te isotopes. Nucl Phys 45:579
Gopych PM, Demchenko MN, Zalyubovskiy II, Kizim PS, Sotnikov VV, Shchus AF (1987) Neutron cross-sections for tin, tellurium, silicon and phosphorus nuclei at the neutron energy 14.6 MeV. In: First international conference on neutron physics vol 3
Zhou F, Zhang Y, Tuo F, Yi Y, Kong X (2006) Cross-section measurements for the 128Te(n,2n)127mTe reaction induced by neutrons around 14 MeV. Appl Radia Isoto 64:815
Lu WD, Ranakumar N, Fink RW (1970) Activtion cross sections for (n,2n) reactions at 14.4 MeV in the region Z=40–60 precision measurements and systematics. Phys Rev C 1:350
Husain L, Kuroda PK (1968) Isomeric cross section ratios for some reactions induced by 14.8 MeV neutrons in Te isotopes. Nucl Phys A 114:663
Kayashima K, Nagao A, Kumabe I (1979) Activation cross section on Ti, Mn, Cu, Zn, Sr, Y, Cd, In and Te for 14.6 neutrons. Progress Report, Japanese report to NEANDC; No.61U, 94
Schnabel C, Leya I, Michel R, Csikai J, Dezso Z, Lopez-Gutierrez JM, Synal HA (2000) Non-destructive and radiochemical determination of the neutron-induced production cross section of I-129 from Te and other neutron-induced cross sections on Te at 14.7 MeV. Radiochim Acta 88:439
Zhou F, Tuo F, Yi Y, Kong X (2007) Cross-section measurements for (n, 2n) and (n, p) reactions on tellurium isotopes in the neutron energy range of 13.5–14.6 MeV. Radiochim Acta 95:553
Filatenkov AA (2016) Neutron activation cross sections measured at KRI in neutron energy region 13.4–14.9 MeV. Report, USSR report to the I.N.D.C.; No.0460
Evaluated Nuclear Structure Data File (ENSDF), https://www.nndc.bnl.gov/ensdf/.
Luo J, Jiang L, Wang X (2018) Activation cross section and isomeric cross-section ratio for the 76Ge(n,2n)75m, gGe process. Eur Phys J A 54:67
Luo J, Tuo F, Kong X, Liu R, Jiang L (2008) Measurements of activation cross-sections for the 96Ru(n, d*)95gTc reaction for neutrons with energies between 13.3 and 15.0 MeV. Appl Radiat Isot 66:1920
Wagner M, Vonach H, Pavlik A, Strohmaier B, Tagesen S, Martinez-Rico J (1990) Physik Daten-physics data, evaluation of cross sections for 14 important Neutron-dosimetry Reactions, Fachinformationszentrum Karlsruhe, Gesellschaft für wissenschaftlich-technische Information mbH, in the Federal Republic of Germany. No.13–5, Karlsruhe.
Luo J, Du L, Zhao J (2013) A method to determine fast neutron energies in large sample. Nucl Instrum Meth B 298:61
Nethaway DR (1978) The 93Nb (n,2n) 92mNb cross section. J Inorg Nucl Chem 40:1285
Luo J, Liu J, Han J, Liu R, Jiang L, Ge S, Liu Z (2013) Measurement of 167Er(n,p)167Ho reaction at 13.5 and 14.8 MeV. Radiat Phys Chem 92:28
Luo J, Tuo F, Zhou F, Kong X (2008) Semi-empirical systematics for the cross-sections of the reactions (n, α), (n, p) and (n,2n) at 14.5 MeV neutrons on the basis of experimental data measured by Lanzhou University. Nucl Instru Meth B 266:4862
Luo J, Wang X, Liu Z, Tuo F, Kong X (2009) Activation cross-sections for 158Dy(n,p)158Tb, 156Dy(n,α)153Gd and 160Dy(n,p)160Tb reactions induced by neutrons at 14.7 MeV. Appl Radiat Isot 67:1892
Hubbell JH, Seltzer SM (2013) Tables of X-ray mass attenuation coefficients and mass energy-absorption coefficients from 1 keV to 20 MeV for elements Z = 1 to 92 and 48 additional substances of dosimetric Interest. https://physics.nist.gov/PhysRefData/XrayMassCoef/tab3.html.
Taylor JR (1982) An introduction to uncertainty analysis. University Science Books, Mill Valley, California
Koning A, Hilaire S, Goriely S (2019) “TALYS-1.95, A nuclear reaction program,” NL-1755 ZG Petten, The Netherlands. https://www.talys.eu
Koning J, Delaroche JP (2003) Local and global nucleon optical models from 1 keV to 200 MeV. Nucl Phys A 713:231
Hauser W, Feshbach H (1952) The inelastic scattering of neutrons. Phys Rev 87:366
Watanabe S (1958) High energy scattering of deuterons by complex nuclei. Nucl Phys 8:484
Kalbach C (1986) Two-component exciton model: Basic formalism away from shell closures. Phys Rev C 33:818
Capote R, Herman M, Oblozinsky P, Young PG, Goriely S, Belgya T, Ignatyuk AV, Koning AJ, Hilaire S, Plujko VA, Avrigeanu M, Bersillon O, Chadwick MB, Fukahori T, Ge Z, Han Y, Kailas S, Kopecky J, Maslov VM, Reffo G, Sin M, Soukhovitskii ESh, Talou P (2009) RIPL—reference input parameter library for calculation of nuclear reactions and nuclear data evaluations. Nucl Data Sheets 110:3107
Filatenkov AA, Chuvaev SV, Aksenov VN, Yakovlev VA, Malyshenkov AV, Vasil’ev Sk, Avrigeanu M, Avrigeanu V, Smith DL, Ikeda Y, Wallner A, Kutschera W, Priller A, Steier P, Vonach H, Mertens G, Rochow W (1999) Systematic measurement of activation cross sections at neutron energies from 13.4 to 14.9 MeV. Report: INDC(CCP)-252, IAEA, Vienna
Acknowledgements
We would like to thank the Intense Neutron Generator group at Chinese Academy of Engineering Physics for performing the irradiations. This work was supported by the National Natural Science Foundation of China (Grant No. 11565012).
Author information
Authors and Affiliations
Corresponding author
Additional information
Publisher's Note
Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.
Rights and permissions
About this article
Cite this article
Luo, J., Jiang, L., Shan, L. et al. Activation cross-section and isomeric cross-section ratio for the 122Te(n,2n)121m,gTe process. J Radioanal Nucl Chem 324, 913–920 (2020). https://doi.org/10.1007/s10967-020-07119-3
Received:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s10967-020-07119-3