Skip to main content
Log in

Neutron resonance transmission analysis of cylindrical samples used for reactivity worth measurements

  • Published:
Journal of Radioanalytical and Nuclear Chemistry Aims and scope Submit manuscript

Abstract

A characterization of cylindrical samples by neutron resonance transmission analysis (NRTA) at the GELINA facility of JRC Geel (Belgium) is presented. The samples were designed and produced for reactivity worth measurements in the MINERVE reactor of CEA Cadarache (France). NRTA was applied to determine the nuclide composition of UO2, Al2O3 and liquid samples that were doped with silver. The volume number densities of 238U, 107Ag and 109Ag obtained by NRTA are within 2% fully consistent with the values that are quoted by the manufacturer. In addition, the NRTA data reveal a tungsten contamination which is not reported by the provider. It is shown that such a contamination contributes by up to 5.7% to the reactivity worth.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6
Fig. 7
Fig. 8
Fig. 9

Similar content being viewed by others

References

  1. Bernard D, Leconte P (2010) Validation of actinides nuclear cross-section using pile-oscillation experiments performed at MINERVE facility. Proc J Korean Phys Soc. https://doi.org/10.3938/jkps.59.1119

    Article  Google Scholar 

  2. Sanchez R et al (2010) Apollo2 year 2010. Nucl Eng Technol 42(5):474–499

    Article  Google Scholar 

  3. Gruel A et al (2011) Interpretation of fission product oscillations in the MINERVE reactor, from thermal to epithermal spectra. Nucl Sci Eng 169:229–244

    Article  CAS  Google Scholar 

  4. Ingle JDJ, Crouch SR (1988) Spectrochemical analysis. Prentice Hall, Englewood Cliffs

    Google Scholar 

  5. Schillebeeckx P, Becker B, Harada H, Kopecky S (2014) Neutron resonance spectroscopy for the characterization of materials and objects. JRC Sci Policy Reports, Report EUR 26848

  6. Šalamon L et al (2019) 107Ag and 109Ag resonance parameters for neutron induced reactions below 1 keV. Nucl Instrum Methods Phys Res B 446:19–28

    Article  CAS  Google Scholar 

  7. Thiollay N et al (1999) Burn-up credit for fission products nuclides in PWR(UOX) spent fuels. In: International conference on nuclear criticality safety (ICNC’99), Versailles, France

  8. Leconte P et al (2013) MAESTRO: An Ambitious Experimental Programme for the Improvement of Nuclear Data of Structural, Detection, Moderating and Absorbing Materials - First results for natV, 55Mn, 59Co and 103Rh. In: 3rd international conference on advancements in nuclear instrumentation, measurement methods and their applications (ANIMMA), Marseille, France. https://doi.org/10.1109/animma.2013.6728101

  9. Mondelaers W, Schillebeeckx P (2006) GELINA, a neutron time-of-flight facility for high-resolution neutron data measurements. Notiziario Neutroni e Luce di Sincrotrone 2(2):19–25

    Google Scholar 

  10. Salome JM, Cools R (1981) Neutron producing targets at GELINA. Nucl Instrum Methods 179(1):13–19

    Article  CAS  Google Scholar 

  11. de Jonge (1987) Fast time digitizer type 8514 A. Intern Report GE/DE/R/24/87, IRMM, Geel

  12. Gonzalez J, Bastian C, Hofmans K (1997) Modular multi-parameter multiplexer MMPM. Hardware description and user guide. Intern Report GE/R/INF/06/97, IRMM, Geel

  13. Mihailescu LC et al (2009) Investigations for the use of the fast digitizers with C6D6 detectors for radiative capture measurements at GELINA. Nucl Instrum Methods A 600(2):453–459

    Article  CAS  Google Scholar 

  14. Schillebeeckx P et al (2012) Determination of resonance parameters and their covariances from neutron induced reaction cross section data. Nucl Data Sheets 113:3054–3100

    Article  CAS  Google Scholar 

  15. Becker B et al (2012) Data reduction and uncertainty propagation of time-of-flight spectra with AGS. J Instrum 7:P11002

    Article  Google Scholar 

  16. Harada H et al (2014) Generalized analysis method for neutron resonance transmission analysis. J Nucl Sci Technol 52(6):837–843

    Article  CAS  Google Scholar 

  17. Moxon MC, Brisland JB (1991) GEEL REFIT, a least squares fitting program for resonance analysis of neutron transmission and capture data computer code. Technical report AEA-InTec-0630

  18. Jackson HE, Lynn JE (1962) Resonant absorption of neutrons by crystals. Phys Rev 127(2):461–468

    Article  CAS  Google Scholar 

  19. Phillips NE (1971) Low-temperature heat capacity of metals. Crit Rev Solid State Phys Sci 2(4):467–553

    Article  CAS  Google Scholar 

  20. Ho CY et al (1974) Thermal conductivity of the elements: a comprehensive review. J Phys Chem Ref Data 3(1):1–796

    Article  Google Scholar 

  21. Ashcroft NW, Mermin ND (1976) Solid state physics. Holt-Saunder, Eastbourne

    Google Scholar 

  22. Gao HX, Peng LM (1999) Parameterization of the temperature dependence of the Debye–Waller factors. Acta Cryst A 55(5):926–932

    Article  CAS  Google Scholar 

  23. Feranchuk ID et al (2002) Estimation of the Debye temperature for crystals with polyatomic unit cell. Eur Phys J Appl Phys 19(2):95–101

    Article  CAS  Google Scholar 

  24. Kittel C (2005) Introduction to solid state physics, 8th edn. Wiley, Hoboken

    Google Scholar 

  25. X-5 Monte Carlo Team (2005) MCNP-A general Monte Carlo N-particle transport code, Version 5, vol I: Overview and Theory LA-UR-03-1987

  26. Derrien H, Courcelle A, Leal LC, Larson NM (2009) R-Matrix analysis of 238U high-resolution neutron transmissions and capture cross sections in the energy range 0 to 20 keV. Nucl Sci Eng 161(2):131–159

    Article  CAS  Google Scholar 

Download references

Acknowledgements

This work was supported by the EUFRAT open access programme of the Joint Research Centre. The authors would like to thank technical staff for the dedicated and skillful operation of GELINA. We are also grateful to scientists of EC-JRC-Geel for their valuable comments and suggestions. L. Šalamon acknowledges the GENTLE project (Grant No. 323304) for the support during his stay at the JRC Geel.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Lino Šalamon.

Additional information

Publisher's Note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Šalamon, L., Geslot, B., Heyse, J. et al. Neutron resonance transmission analysis of cylindrical samples used for reactivity worth measurements. J Radioanal Nucl Chem 321, 519–530 (2019). https://doi.org/10.1007/s10967-019-06611-9

Download citation

  • Received:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s10967-019-06611-9

Keywords

Navigation