Abstract
The results of the gamma spectrometry analysis of the 40 samples of highly radioactive granites used in the construction industry in Serbia are presented. Based on the measured activity concentrations of 226Ra, 232Th and 40K, radiological hazard indices, annual effective doses, as well as indoor radon concentration were determined. Calculated indoor radon concentration caused by investigated granite samples in 25% of cases exceeds the upper limit of 300 Bq m−3 recommended by the World Health Organization.
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Khan AR, Rafique M, Jabbar A, Rahman SU, Shahzad MI, Khan ME, Yasin M (2018) Radionuclide concentrations in sand samples from riverbanks of Muzaffarabad, Azad Kashmir. Nucl Sci Technol 29:93. https://doi.org/10.1007/s41365-018-0442-9
Abdullahi S, Ismail AF, Samat S (2018) Determination of indoor doses and excess lifetime cancer risks caused by building materials containing natural radionuclides in Malaysia. Nucl Eng Technol 51:325–336. https://doi.org/10.1016/j.net.2018.09.017
Cazula CD, Campos MP, Mazzilli BP (2015) Gamma exposure due to building materials in a residential building at Peruibe, Sao Paulo, Brazil. J Radioanal Nucl Chem 306:637–640
Medhat ME (2009) Assessment of radiation hazards due to natural radioactivity in some building materials used in Egyptian dwellings. Radiat Prot Dosim 133:177–185. https://doi.org/10.1093/rpd/ncp032
Stoulos S, Mamolopoulou M, Papastefanou C (2003) Assessment of natural radiation exposure and radon exhalation from building materials in Greece. J Environ Radioact 69:225–240. https://doi.org/10.1016/S0265-931X(03)00081-X
UNSCEAR (2000) Sources and effects of ionizing radiation. United Nations Scientific Committee on the Effects of Atomic Radiation. United Nations Publication, New York
Alali E, Al-Shboul KF, Albdour SA (2018) Radioactivity measurement and radiological hazard assessment of the commonly used granite and marble in Jordan. Radiat Prot Dosim 182:386–393. https://doi.org/10.1093/rpd/ncy077
Gupta M, Chauhan RP (2011) Estimating radiation dose from building materials. Iran J Radiat Res. 9:187–194
Abbasi A, Hassanzadeh M (2017) Measurement and Monte Carlo simulation of gamma-ray dose rate in high-exposure building materials. Nucl Sci Technol 28:1–5. https://doi.org/10.1007/s41365-016-0171-x
Anjos RM, JuriAyub J, Cid AS, Cardoso R, Lacerda T (2011) External gamma-ray dose rate and radon concentration in indoor environments covered with Brazilian granites. J Environ Radioact 102:1055–1061. https://doi.org/10.1016/j.jenvrad.2011.06.001
Llope WJ (2011) Activity concentrations and dose rates from decorative granite countertops. J Environ Radioact 102:620–629. https://doi.org/10.1016/j.jenvrad.2011.03.012
Markkanen M (1995) Radiation dose assessments for materials with elevated natural radioactivity. Finnish Centre for Radiation and Nuclear Safety STUK-B-STO 32, Helsinki
UNSCEAR (1993) Sources, effects and risks of ionizing radiation. United Nations Scientific Committee on the Effects of Atomic Radiation, United Nations New York, USA
Official Gazette RS 36/18 (2018) Regulation on limits of radionuclide content in drinking water, foodstuffs, feeding stuffs, drugs, items of general use, building materials and other goods to be placed on the market (in Serbian). Serbian Radiation and Nuclear Safety and Security Directorate, Belgrade
Council Directive 2013/59/Euratom of 5 Dec. 2013 (2014) Laying down basic safety standards for protection against the dangers arising from exposure to ionising radiation, and repealing directives 89/618/Euratom, 90/641/Euratom, 96/29/Euratom, 97/43/Euratom and 2003/122/Euratom. L13, vol 57. ISSN 1977-0677. https://ec.europa.eu/energy/sites/ener/files/documents/CELEX-32013L0059-EN-TXT.pdf
Sola P, Srinuttrakul W, Laoharojanaphand S, Suwankot N (2014) Estimation of indoor radon and the annual effective dose from building materials by ionization chamber measurement. J Radioanal Nucl Chem 302:1531–1535. https://doi.org/10.1007/s10967-014-3716-7
Vimercati L, Fucilli F, Cavone D, De Maria L, Birtolo F, Ferri G, Soleo L, Lovreglio P (2018) Radon levels in indoor environments of the University Hospital in Bari-Apulia Region Southern Italy. Int J Environ Res Public Health 15:694. https://doi.org/10.3390/ijerph15040694
World Health Organization (2009) In: Zeeb H, Shannoun F (eds) Handbook on indoor radon: a public health perspective. WHO Library Cataloguing-in-Publication Data. World Health Organization, Geneva
Commission European (1999) Radiation Protection 112—radiological protection principles concerning the natural radioactivity of building materials. EC, Luxembourg
Chen J, Rahman NM, Atiya IA (2010) Radon exhalation from building materials for decorative use. J Environ Radioact 101:317–322. https://doi.org/10.1016/j.jenvrad.2010.01.005
International Atomic Energy Agency (1989) Measurement of radionuclides in food and the environment. Technical Reports Series No. 295., Vienna, Austria
Todorovic N, Forkapic S, Bikit I, Mrdja D, Veskovic M, Todorovic S (2011) Monitoring for exposures to TENORM Sources in Vojvodina region. Radiat Prot Dosim 144:655–658. https://doi.org/10.1093/rpd/ncq414
Moens L, Donder JD, Xi-lei L, Corte FD, Wispelaere AD, Simonits A, Hoste J (1981) Calculation of the absolute peak efficiency of gamma-ray detectors for different counting geometries. Nucl Instr Methods 187:451–472. https://doi.org/10.1016/0029-554X(81)90374-8
Aykamis AS, Turhan S, AysunUgur F, Baykan UN, Kilic AM (2013) Natural radioactivity, radon exhalation rates and indoor radon concentration of some granite samples used as construction material in Turkey. Radiat Prot Dosim 157:105–111. https://doi.org/10.1093/rpd/nct110
Beretka J, Mathew PJ (1985) Natural radioactivity of Australian building materials, industrial wastes and byproducts. Health Phys 48:87–95
NEA-OECD (1979) Nuclear Energy Agency. Exposure to Radiation from Natural Radioactivity in Building Materials. Reported by NEA Group of Experts, OECD, Paris
Kobeissi MA, El-Samad O, Rachidi I (2013) Health assessment of natural radioactivity and radon exhalation rate in granites used as building materials in Lebanon. Radiat Prot Dosim 153:342–351. https://doi.org/10.1093/rpd/ncs110
Al-Zahrani JH (2017) Estimation of natural radioactivity in local and imported polished granite used as building materials in Saudi Arabia. J Radiat Res Appl Sci 10:241–245. https://doi.org/10.1016/j.jrras.2017.05.001
Thabayneh KM (2013) Measurement of natural radioactivity and radon exhalation rate in granite samples used in Palestinian buildings. Arab J Sci Eng 38:201–207. https://doi.org/10.1007/s13369-012-0391-2
Pantelic GK, Todorovic DJ, Nikolic JD, Rajacic MM, Jankovic MM, Sarap NB (2014) Measurement of radioactivity in building materials in Serbia. J Radioanal Nucl Chem 303:2517–2522. https://doi.org/10.1007/s10967-014-3745-2
Righi S, Bruzzi L (2006) Natural radioactivity and radon exhalation in building materials used in Italian dwellings. J Environ Radioact 88:158–170. https://doi.org/10.1016/j.jenvrad.2006.01.009
International Commission on Radiological Protection (1994) Protection against Radon-222 at home and at work (ICRP Publication No. 65). Annals of the ICRP 23(2). Pergamon Press, Oxford
Qureshi AA, Jadoon IAK, Wajid AA, Attique A, Masood A, Anees M, Manzoor S, Waheed A, Tubassam A (2013) Study of natural radioactivity in mansehra granite, Pakistan: environmental concerns. Radiat Prot Dosim 158:466–478. https://doi.org/10.1093/rpd/nct271
Hassan MN, Mansour NA, Fayez-Hassan M (2013) Evaluation of radionuclide concentration and associated radiological hazard indexes in building materials used in Egypt. Radiat Prot Dosim 157:214–220. https://doi.org/10.1093/rpd/nct129
UNSCEAR (2008) Sources and effects of ionizing radiation. United Nations Scientific Committee on the Effects of Atomic Radiation. United Nations Publication, New York
International Commission on Radiological Protection (2006) Assessing dose of the representative person for the purpose of the radiation protection of the public. (ICRP Publication No. 101a) Annals of the ICRP 36(3)
Leal ALC, Lauria DC (2016) Assessment of doses to members of the public arising from the use of ornamental rocks in residences. J Radiol Prot 36:680–694. https://doi.org/10.1088/0952-4746/36/3/680
Poncela LSQ, Fernández PL, Gómez Arozamena J, Sainz C, Fernández JA, Mahou ES, Matarranz M, Cascón MC (2004) Natural gamma radiation map (MARNA) and indoor radon levels in Spain. Environ Int 29:1091–1096. https://doi.org/10.1016/S0160-4120(03)00102-8
Sharaf JM, Hamideen MS (2013) Measurement of natural radioactivity in Jordanian building materials and their contribution to the public indoor gamma dose rate. Appl Radiat Isot 80:61–66. https://doi.org/10.1016/j.apradiso.2013.06.016
Al-Jarallah M (2001) Radon exhalation from granites used in Saudi Arabia. J Environ Radioact 53:91–98. https://doi.org/10.1016/s0265-931x(00)00110-7
Rafique M, Rathore MH (2013) Determination of radon exhalation from granite, dolerite and marbles decorative stones of the Azad Kashmir area, Pakistan. Int J Environ Sci Technol 10:1083–1090. https://doi.org/10.1007/s13762-013-0288-y
Bala P, Kumar V, Mehra R (2017) Measurement of radon exhalation rate in various building materials and soil samples. J Earth Syst Sci 126:31. https://doi.org/10.1007/s12040-017-0797-z
Acknowledgements
The authors thanks the financial support of the Ministry of Education, Science and Technological Development of the Government of the Republic of Serbia, within the projects Nuclear Methods Investigations of Rare Processes and Cosmic No. 171002, Biosensing Technologies and Global System for Continues Research and Integrated Management No. 43002 and Development and Application of Multifunctional Materials Using Domestic Raw Materials in Upgraded Processing Lines No. III45008.
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Kuzmanović, P., Todorović, N., Nikolov, J. et al. Assessment of radiation risk and radon exhalation rate for granite used in the construction industry. J Radioanal Nucl Chem 321, 565–577 (2019). https://doi.org/10.1007/s10967-019-06592-9
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DOI: https://doi.org/10.1007/s10967-019-06592-9