Skip to main content
SpringerLink
Log in

Measurement of cross sections for the formation of 100gRh in natPd(p,x)100m,gRh reactions up to 42.61 MeV

  • Published:
Journal of Radioanalytical and Nuclear Chemistry Aims and scope Submit manuscript

Abstract

We measured the cross sections for the formation of the ground state nucleus 100gRh through natPd(p,x)100m,gRh reactions. The experiment was carried out using the stacked-foil activation technique in the energy range from threshold to 42.61 MeV. The cross section was determined on the basis of the measured activity of the corresponding residual nucleus using a high energy resolution HPGe γ-ray detector. The energy dependent flux of the proton beam was determined using the natCu(p,x)62Zn and natCu(p,x)65Zn monitoring reactions. In order to enhance the accuracy of the experimental results, the activity contributions from the decay of the 100mAg, 100gAg and 100Pd to 100gRh, which were also produced in the same palladium foil were corrected. The present experimental results are compared with the previously published data and with the theoretical predictions from the TENDL-2017 library.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Log in via an institution

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Institutional subscriptions

Fig. 1
Fig. 2
Fig. 3
Fig. 4

Similar content being viewed by others

References

  1. Sudár S, Qaim SM (1996) Isomeric cross-section ratio for the formation of 58m,gCo in neutron, proton, deuteron, and alpha-particle induced reactions in the energy region up to 25 MeV. Phys Rev 53:2885–2892

    Article  Google Scholar 

  2. Qaim SM (2001) Nuclear data relevant to the production and application of diagnostic radionuclides. Radiochim Acta 89:223–232

    CAS  Google Scholar 

  3. Qaim SM, Tárkányi F, Obložinský P, Gul K, Hermanne A, Mustafa MG, Nortier FM, Scholten B, Shubin Yu, Takács S, Zhuang Y (2001) Charged particle cross-section database for medical radioisotope production: diagnostic radioisotopes and monitor reactions. IAEA-TECDOC-1211, Vienna http://www-nds.iaea.org/medical/

  4. Birattari C, Gadioli E, Strini MG, Strini G, Tagliaferri G, Zetta L (1971) (p, xn) reactions induced in 169Tm, 181Ta and 209Bi with 20 to 45 MeV protons. Nuclear Phys A 166:605–623

    Article  CAS  Google Scholar 

  5. Ditrói F, Tárkányi F, Takács S, Hermanne A (2016) Activation cross-sections of proton induced reactions on vanadium in the 37–65 MeV energy range. Nucl Instr Methods B 381:16–28

    Article  CAS  Google Scholar 

  6. Rangacharyulu C, Fukuda M, Kanda H, Nishizaki S, Takahashi N (2017) Assessment of 43,44Sc isotope production in proton- and alpha-induced reactions. J Radioanal Nucl Chem 314:1967–1971

    Article  CAS  Google Scholar 

  7. Tárkányi F, Ditrói F, Takács S (2016) Activation cross sections of proton induced nuclear reactions on palladium up to 80 MeV. Appl Radiat Isot 114:128–144

    Article  CAS  PubMed  Google Scholar 

  8. Khandaker MU, Kim KS, Kim GN, Otuka N (2010) Cyclotron production of the 105,106mAg, 100,101Pd, 100,101 m,105Rh radionuclides by natPd(p,x) nuclear processes. Nucl Instr Methods B 268:2303–2311

    Article  CAS  Google Scholar 

  9. Dogra R, Brett DA, Byrne AP, Mestnik-Filho J, Li Y, Ridgway MC (2006) Do palladium–dopant pairs exist in silicon. Phys B 376–377:245–248

    Article  CAS  Google Scholar 

  10. Potzger K, Bertschat HH, Burchard A, Forkel-Wirth D, Granzer H, Niehus H, Seeger S, Zeitz WD (1998) ISOLDE collaboration: correlation between local magnetic and structural properties at the Ni/Pd interface. Nucl Instr Methods B 146:618–623

    Article  CAS  Google Scholar 

  11. Johnston K, Schell J, Correia JG, Deicher M, Gunnlaugsson HP, Fenta AS, Bosne ED, Costa ARG, Lupascu DC (2017) The solidstate physics programme at ISOLDE: recent developments and perspectives. J Phys G: Nucl Part Phys 44:104001

    Article  CAS  Google Scholar 

  12. Khandaker MU, Meaze AKMMH, Kim KS, Son DC, Kim GN (2006) Measurements of the proton-induced reaction cross-sections of natMo by using the MC50 cyclotron at the Korean Institute of Radiological and Medical Sciences. J Korean Phys Soc 48:821–826

    CAS  Google Scholar 

  13. National Nuclear Data Center, Brookhaven National Laboratory, Nuclear structure and decay data (NuDat 2.7) (2017) http://www.nndc.bnl.gov/nudat2/

  14. Singh B (2008) Nuclear data sheets for A = 100. Nucl Data Sheets 109:297–516

    Article  CAS  Google Scholar 

  15. Do NV, Khue PD, Thanh KT, Nam TH, Rahman MS, Kim KS, Lee MW, Kim GN, Lee HS, Cho MH, Ko IS, Namkung W (2011) Measurement of isomeric yield ratios for the 44 m, gSc isomeric pairs produced from 45Sc and natTi targets at 50-, 60-, and 70-MeV bremsstrahlung. J Radioanal Nucl Chem 287:813–820

    Article  CAS  Google Scholar 

  16. Dillmann I, Coquard L, Domingo-Pardo C, Käppeler F, Marganiec J, Uberseder E, Giesen U, Heiske A, Feinberg G, Hentschel D, Hilpp S (2011) Cross sections for proton-induced reactions on Pd isotopes at energies relevant for the γ process. Phys Rev C 84:015802

    Article  CAS  Google Scholar 

  17. Cervenák J, Lebeda O (2016) Experimental cross-sections for proton-induced nuclear reactions on natMo. Nucl Instr Methods B 380:32–49

    Article  CAS  Google Scholar 

  18. Hubbell JH, Seltzer SM (2004) National Institute of Standards and Technology, NIST Standard Reference Database 126 https://physics.nist.gov/PhysRefData/XrayMassCoef/tab3.html

  19. Montgomery DM, Montgomery GA (1995) A method for assessing and correcting coincidence summing effects for germanium detector efficiency calibrations. J Radioanal Nucl Chem 193:71–79

    Article  CAS  Google Scholar 

  20. Piton F, Lépy MCh, Bé MM, Plagnard J (2000) Efficiency transfer and coincidence summing corrections for γ-ray spectrometry. Appl Radiat Isot 52:791–795

    Article  CAS  PubMed  Google Scholar 

  21. Ziegler JF (2004) SRIM-2003. Nucl Inst Methods B 219–220:1027–1036

    Article  CAS  Google Scholar 

  22. Ziegler JF, Biersack JP, Littmark U (2003) SRIM 2003 code, Version 96.xx. The stopping and range of ions in solids. Pergamon, New York http://www.srim.org/

  23. Calculation of reaction Q-values and thresholds, Los Alamos National Laboratory, T-2 Nuclear Information Service http://t2.lanl.gov/data/qtool.html/

  24. Koning AJ, Rochman D (2012) Modern nuclear data evaluation with the TALYS code system. Nucl Data Sheets 113:2841–2934

    Article  CAS  Google Scholar 

  25. Hayakawa HI, Hyman I, Lee JKP (1980) Decay of 100Ag. Phys Rev C 22:247–251

    Article  CAS  Google Scholar 

  26. Koning AJ, Rochman D, van der Marck SC, Kopecky J, Sublet JCh, Pomp S, Sjostrand H, Forrest R, Bauge E, Henriksson H, Cabellos O, Goriely S, Leppanen J, Leeb H, Plompen A, Mills R (2017) TENDL-2017, TALYS-based evaluated nuclear data library. Nucler Research and Consultancy Group (NRG), Petten https://tendl.web.psi.ch/tendl_2017/tendl2017.html

  27. Koning AJ, Rochman D, Ch Sublet J, Dzysiuk N, Fleming M, van der Marck S (2019) TENDL: complete nuclear data library for innovative nuclear science and technology. Nucl Data Sheets 155:1–55

    Article  CAS  Google Scholar 

  28. Ditrói F, Tárkányi F, Takács S, Mahunka I, Csikai J, Hermanne A, Uddin MS, Hagiwara M, Baba M, Ido T, Shubin Yu, Dityuk AI (2007) Measurement of activation cross sections of the proton induced nuclear reactions on palladium. J Radioanal Nucl Chem 272:231–235

    Article  CAS  Google Scholar 

Download references

Acknowledgements

The authors express their sincere thanks to the staff of the MC-50 Cyclotron Laboratory in the Korea Institute of Radiological and Medical Sciences (KIRAMS), Korea for the excellent operation and their support during the experiment. This research was partly supported by the National Research Foundation of Korea through a grant provided by the Ministry of Science, ICT and Future Planning (NRF-2017R1D1A1B03030484, NRF-2018M7A1A1072274, and NRF-2018R1A6A1A06024970) and by the Vietnam National Foundation for Science and Technology Development (NAFOSTED) under Grant No. 103.04-2018.314.

Author information

Authors and Affiliations

  1. Institute of Theoretical and Applied Research, Duy Tan University, Hanoi, 100000, Vietnam

    Van Do Nguyen

  2. Institute of Physics, Vietnam Academy of Science and Technology, 10 Dao Tan, Hanoi, Vietnam

    Van Do Nguyen & Thanh Luan Nguyen

  3. Graduate School of Science and Technology, VAST, 18 Hoang Quoc Viet, Hanoi, Vietnam

    Thi Xuan Nguyen

  4. Department of Physics, Kyungpook National University, Daegu, 41566, Republic of Korea

    Thi Hien Nguyen, Guinyun Kim & Kwangsoo Kim

Authors
  1. Van Do Nguyen
    View author publications

    You can also search for this author in PubMed Google Scholar

  2. Thanh Luan Nguyen
    View author publications

    You can also search for this author in PubMed Google Scholar

  3. Thi Xuan Nguyen
    View author publications

    You can also search for this author in PubMed Google Scholar

  4. Thi Hien Nguyen
    View author publications

    You can also search for this author in PubMed Google Scholar

  5. Guinyun Kim
    View author publications

    You can also search for this author in PubMed Google Scholar

  6. Kwangsoo Kim
    View author publications

    You can also search for this author in PubMed Google Scholar

Corresponding author

Correspondence to Guinyun Kim.

Additional information

Publisher's Note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Do Nguyen, V., Nguyen, T.L., Nguyen, T.X. et al. Measurement of cross sections for the formation of 100gRh in natPd(p,x)100m,gRh reactions up to 42.61 MeV. J Radioanal Nucl Chem 321, 117–123 (2019). https://doi.org/10.1007/s10967-019-06554-1

Download citation

  • Received:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s10967-019-06554-1

Keywords

Search

Navigation