Abstract
U–Zr–RE heel residue was manufactured after fabricating U–Zr–RE fuel slugs by an injection casting method. In order to increase the fabrication yield rate, the uranium scrap waste should be reused as raw materials through surface treatment. Various impurity elements existed on the surface of the heel residue. Scanning electron microscopy and Energy-dispersive X-ray spectroscopy results showed that rare-earth elements in the dilute nitric acid were removed using air agitation. Impurity elements for the heel residue were removed from the top and bottom layers by pickling. Metallic fuel slugs were soundly fabricated using the pickled heel residue as raw materials.
Similar content being viewed by others
References
Kim JH, Song H, Kim KH, Lee CB (2014) J Radioanal Nucl Chem 301:797–803
Kim JH, Kim HT, Kim KIM, Kim CB (2014) J Radioanal Nucl Chem 300:1245–1251
Kim JH, Song H, Kim KH, Lee CB (2015) Surf Interface Anal 47:301–307
Ha SJ, Kim KH, Park JY, Hong SI (2017) Sci Adv Mater 9:1837–1842
Ogata T, Tsukada T (2007) Global. 2007:557–562
Song H, Kim JH, Ko YM, Woo YM, Kim KH, Lee CB (2014) Sci Adv Mater 6:1–8
Kim KH, Lee CT, Lee CB, Fielding RS, Kennedy JR (2011) Thin Solid Films 519:6969–6973
Pfdender E (1999) Plasma Chem Plasma Process 19:1–30
Kuk SW, Kim KH, Kim JH, Song H, Oh SJ, Park JY, Lee CB, Youn YS, Kim JY (2017) J Nucl Mater 486:53–59
Lee EH, Lim JK, Chung DY, Yang HB, Yoo JH, Kim KW (2009) J Radioanal Nucl Chem 281:330–346
Mooney Ted (2002) Metal Finish 100:731–738
Kim JH, Lee BO, Lee CB, Jee SH, Yoon YS (2012) J Rare Earth 30:599–603
Vera Serna P et al (2016) Mater Res 19(2):389–393
Reddy Benjaram M et al (2009) Catal Lett 131(1):328–336
Acknowledgements
This work was supported by Nuclear Research and Development Program of the National Research Foundation Grant funded by the Ministry of Education, Science and Technology in Korea.
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Ha, SJ., Kim, KH., Park, JY. et al. Characterization of reused U–10Zr heel residue containing rare-earth elements through surface treatment. J Radioanal Nucl Chem 316, 1157–1163 (2018). https://doi.org/10.1007/s10967-018-5869-2
Received:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s10967-018-5869-2