Development of a 212Pb and 212Bi generator for homolog studies of flerovium and moscovium

  • John D. Despotopulos
  • Kelly N. Kmak
  • Kenton J. Moody
  • Dawn A. Shaughnessy
Article
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Abstract

A simple generator using AG 50Wx8 cation exchange resin has been developed for continual elution of 212Pb and 212Bi from the parent radionuclide 228Th, derived from 232U. Using 0.4 M HCl as an eluent will elute 212Bi while 212Pb is eluted with 2 M HCl. The generator has shown good reproducibility of elution bands. A generator set-up in 2013 has been in continual use over 4 years demonstrating that this generator system has a long and stable lifetime. The generator system presented here has served as a long-term method for attaining no-carrier-added 212Pb and 212Bi radionuclides for homolog studies of flerovium and moscovium.

Keywords

Cation exchange Radioisotope generator Flerovium Moscovium Homologs Heavy element 

Notes

Acknowledgements

This study was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. This work was funded by the Laboratory Directed Research and Development Program at LLNL under project tracking code 11-ERD-011 and 17-LW-035.

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Copyright information

© Akadémiai Kiadó, Budapest, Hungary 2018

Authors and Affiliations

  • John D. Despotopulos
    • 1
  • Kelly N. Kmak
    • 2
  • Kenton J. Moody
    • 1
  • Dawn A. Shaughnessy
    • 1
  1. 1.Nuclear and Chemical Sciences DivisionLawrence Livermore National LaboratoryLivermoreUSA
  2. 2.University of California BerkeleyBerkeleyUSA

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