Abstract
The determination of the radionuclides of U- and Th-series as well as of 40K and 137Cs in soils and waters in a lignite mining area was performed. The measurements in the soils were undertaken by γ-ray spectrometry while the concentrations of 234U and 238U in waters and the isotopic ratio 234U/238U were determined by α-ray spectrometry. Slight seasonal variation of the radioactivity was observed with high values in summer and low in winter. The estimated annual radiation dose from soil was lower than the worldwide average whereas in the case of water only one location showed increment in the internal radiation about 18 % of the worldwide average.
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References
Papastefanou C, Charalambous S (1984) On the escaping radioactivity from lignite coal power plants (CPP). Health Phys 46(2):293–302
Krylov DA, Sidorova GP (2013) Radioactivity of coal and ash-slag TPP wastes. At Energy 114(1):56–60
Dimotakis PN, Papaefthymiou H, Springer A, Goetz L (1988) Trace metals in lignite and ashes of Greek power plants. J Radioanal Nucl Chem Lett 127:133–141
Mijac L, Krizman M (1996) Radioactive contamination of surface waters from a fly-ash depository at Velenje (Slovenia). Environ Int 22:339–345
Georgakopoulos A, Filippidis A, Kassoli-Fournaraki A, Iordanidis A, Fernández-Turiel JL, Ilorens JF, Gimeno D (2002) Environmentally important elements in fly ashes and their leachates of the power stations of Greece. Energy Sources 24:83–91
Karamanis D, Ioannides K, Stamoulis K (2009) Environmental assessment of natural radionuclides and heavy metals in waters discharged from a lignite-fired power plant. Fuel 88:2046–2052
Charro E, Pardo R, Pena V (2013) Chemometric interpretation of vertical profiles of radionuclides in soils near a Spanish coal-fired power plant. Chemosphere 90:488–496
Asokan P, Saxena M, Asolekar SR (2005) Coal combustion residues environmental implications and recycling potentials. Res Conserv Recycl 43:239–262
Public power corporation of Greece (2003) http://www.dei.gr Accessed 28 Jan 2016
Megalovasilis P, Papastergios G, Filippidis A (2013) Behavior study of trace elements in pulverized lignite, bottom ash, and fly ash of Amyntaio power station, Greece. Environ Monit Assess 185:6071–6076
Papaefthymiou H, Symeopoulos BD, Soupioni M (2007) Neutron activation analysis and natural radioactivity measurements of lignite and ashes from Megalopolis basin, Greece. J Radioanal Nucl Chem 274:123–130
Manolopoulou M, Stoulos S, Mironaki D, Papastefanou C (2003) A new technique for the accurate measurement of 226Ra by gamma spectroscopy in voluminous samples. Nucl Instrum Methods A 508:362–366
Kiliari T, Pashalidis (2010) Simplified alpha-spectroscopic analysis of uranium in natural waters its separation by cation-exchange. J Radioanal Nucl Chem 284:547–551
Tsiaili A, Kiliari T, Pashalidis I (2011) Seasonal variation of the alpha-radioactivity concentration in natural water systems in Cyprus. Radiat Meas 46:145–148
Tsikritzis LI, Ganatsios SS, Duliu OG (2001) Natural Ra-228, K-40 and artificial Cs-137 radionuclides distribution in soil in area of lignite power plants of western Macedonia. J Trace Microprobe Tech 19(2):256–266
Anagnostakis MJ, Hinis EP, Simopoulos SE, Angelopoulos MG (1996) Natural radioactivity mapping of Greek surface soil. Environ Int 22:S3–S8
Papadopoulos NK, Efstathopoulos AV, Karangelos DJ, Petropoulos NP (2011) Determination of uranium isotope concentrations in precipitation in the vicinity of lignite-fired power plants. Nucl Technol Radiat 26:1–10
Tsertos H, Tzortzis M (2004) Determination of thorium, uranium and potassium elemental concentration in surface soils in Cyprus. J Environ Radioact 77:325–338
Santawamaitre T, Malain D, Al-Sulaiti HA, Bradley DA, Matthews MC, Regan PH (2014) Determination of 238U, 232Th and 40K activity concentrations in riverbank soil along the Chao Phraya river basin in Thailand. J Environ Radioact 138:80–86
Coles DG, Meadows JWT, Lindeken CU (1977) The direct measurement of ppm levels of uranium in soils using high-resolution gamma-ray spectroscopy. Sci Total Environ 5:171–179
Kohler M, Niese S, Gleisberg B, Jenk U, Nindel K (2000) Simultaneous determination of Ra and Th nuclides, 238U and 227Am in uranium mining waters by g-ray spectrometry. Appl Radiat Isot 52:717–723
Papastefanou C, Manolopoulou M, Charalambous S (1988) Cesium-137 in soils from Chernobyl fallout. Health Phys 55:985–987
Lawrence DG (2016) Uranium toxicity literature with commentaries, Department of chemistry and biochemistry, Long Island University, Brooklyn (2004). http://myweb.brooklyn.liu.edu/lawrence/duproject/litsum3.pdf. Accessed 19 Jan 2016
Karpas Z (2015) Analytical chemistry of uranium. CRC Press, Boca Raton
Pendias-Kabata A (2011) Trace elements in soils and plants, 4th edn. CRC Press, Boca Raton
Triantafyllou AG, Zoras S, Evagelopoulos V (2006) Particulate matter over a seven year period in urban and rural areas within, proximal and far from mining and power station operations in Greece. Environ Monitor Asses 122:41–60
WHO 2015 (2011) Guidelines for drinking-water quality, 4th Edn. World Health Organization, Geneva. (http://whqlibdoc.whoint/publications/2011/9789241548151_eng.pdf. Accessed 29 Jan 2016
Kehagia K, Koukouliou V, Bratakos S, Seferlis S, Tzoumerkas F, Potiriadis C (2007) Radioactivity monitoring in drinking water of Atttika, Greece. Desalination 213:98–103
Savidou Α, Sideris G, Zoyridakis N, Ochsenkuhn K, Sotiropoulos P (2002) Uranium in public water supplies in Migdonia Basin, Central Macedonia Northen Greece. J Balk Geophys Soc 5(4):131–134
Ioannidou A, Samaropoulos I, Efstathiou M, Pashalidis I (2011) Uranium in ground water samples in Northen Greece. J Radioanal Nucl Chem 289:551–555
Noli F, Kazakis N, Vargemezis G, Ioannidou A (2016) The Uranium isotopes in the characterization of groundwater in Thermi-Vasilika Region, Northern Greece. Isot Environ Healt Stud 16:1–9
Noli F, Tamos P (2016) Concentrations of heavy metals and trace elements in soils, waters and vegetables and health risk in the vicinity of a lignite-fired power plant. Sci Total Environ 563–564:377–385
Skwarzec B, Struminska-Parulska DI, Borylo A, Kabat K (2012) Polonium, uranium and plutonium radionuclides in aquatic and land ecosystem of Poland. J Environ Sci Health A 47:479–496
Abdul-Hadi A, Alhassanieh O, Ghafar M (2001) Disequilibrium of uranium isotopes in some Syrian groundwater. Appl Radiat Isot 55:109–113
Bampaiti A, Misaelides P, Noli F (2015) Uranium removal from aqueous solutions using a raw and HDTMA-modified phillipsite-bearing tuff. J Radioanal Nucl Chem 303:2233–2241
Shaheen SM, Hooda PS, Tsadilas CD (2014) Opportunities and challenges in the use of coal fly ash for soil improvements—a review. J Environ Manag 145:249–267
UNSCEAR (2000) Sources and effects of ionizing radiation. United Nations, New York
Boryło A (2013) Determination of uranium isotopes in environmental samples. J Radioanal Nucl Chem 295:621–663
Al-Masri MS, Byrakdar ME, Mamish S, Al-Haleem MA (2004) Determination of natural radioactivity in Euphrates river. J Radioanal Nucl Chem 216:349–355
Tripathi RM, Sahoo SK, Mohapatra S, Lenka P, Dubey JS, Puranik VD (2013) Study of uranium isotopic composition in groundwater and deviation from secular equilibrium condition. J Radioanal Nucl Chem 295:1195–1200
El-Aassy IE, El-Feky MG, Issa FA, Ibrahim NM, Desouky OA, Khattab MR (2015) Uranium and 234U/238U isotopic ratios in some groundwater wells at Southwestern Sinai Egypt. J Radioanal Nucl Chem 303:357–362
ICRP (2012) Annals of the ICRP. ICRP Publication 119 41:1–130
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Noli, F., Tsamos, P. & Stoulos, S. Spatial and seasonal variation of radionuclides in soils and waters near a coal-fired power plant of Northern Greece: environmental dose assessment. J Radioanal Nucl Chem 311, 331–338 (2017). https://doi.org/10.1007/s10967-016-5082-0
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DOI: https://doi.org/10.1007/s10967-016-5082-0