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A program to generate simulated radioxenon beta–gamma data for concentration verification and validation and training exercises

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Abstract

PNNL developed a beta–gamma simulator (BGSim) that incorporated GEANT-modeled data sets from radioxenon decay chains, as well as functionality to use nuclear detector-acquired data sets to create new beta–gamma spectra with varying amounts of background, 133Xe, 131mXe, 133mXe, 135Xe, and 222Rn and its decay products. After BGSim was developed, additional uses began to be identified for the program output: training sets of two-dimensional spectra for data analysts at the IDC and other NDC, and spectra for exercises such as the Integrated Field Exercise 2014 held in Jordan at the Dead Sea.

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Notes

  1. In consultation with Dr. Chushiro Yonezawa, Center for Promotion of Disarmament and Non-Proliferation Japan Institute of International Affairs.

References

  1. Bowyer TW, Abel KH, Hubbard CW, McKinnon AD, Panisko ME, Perkins RW, Reeder PL, Thompson RC, Warner RA (1998) Automated separation and measurement of radioxenon for the Comprehensive Test Ban Treaty. J Radioanal Nucl Chem 235:77–81

    Article  CAS  Google Scholar 

  2. Ringbom A, Larson T, Axelsson A, Elmgren K, Johansson C (2003) SAUNA—a system for automatic sampling, processing, and analysis of radioactive xenon. Nucl Instrum Methods Phys Res Sect A 508(3):542–553

    Article  CAS  Google Scholar 

  3. Auer M, Axelsson A, Blanchard X, Bowyer TW, Brachet G, Bulowski I, Dubasov Y, Elmgren K, Fontaine JP, Harms W, Hayes JC, Heimbeigner TR, McIntyre JI, Panisko ME, Popov Y, Ringbom A, Sartorius H, Schmid S, Schulze J, Sclosser C, Taffary T, Weiss W, Wernsperger B (2004) Intercomparison experiments of systems for the measurement of xenon radionuclides in the atmosphere. Appl Radiat Isot 60(6):863–877

    Article  CAS  Google Scholar 

  4. Cagniant A, Le Petit G, Gross P, Douysset G, Richard-Bressand H, Fontaine J-P (2014) Improvements of low-level radioxenon detection sensitivity by a state-of-the art coincidence setup. Appl Radiat Isot 87:48–52

    Article  CAS  Google Scholar 

  5. Xie F, He X, Jiang W, Zhang X, Shi Q, Wu S, Liu L, Zhang C, Chen L (2014) Development of a radioxenon measurement system and its application in monitoring Fukushima nuclear accident. Radiat Phys Chem 97:85–89

    Article  CAS  Google Scholar 

  6. Xie F, Jiang W, Li X, He X, Zhang J, Yu G (2013) Single channel beta–gamma coincidence system for radioxenon measurement using well-type HPGe and plastic scintillator detectors. Nucl Instrum Methods Phys Res Sect A 729:900–904

    Article  CAS  Google Scholar 

  7. Cooper MW, McIntyre JI, Bowyer TW, Carman AJ, Hayes JC, Heimbigner TR, Hubbard CW, Lidey L, Litke KE, Morris SJ, Ripplinger MD, Suarez R, Thompson R (2007) Redesigned β–γ radioxenon detector. Nucl Instrum Methods Phys Res Sect A 579:426–430

    Article  CAS  Google Scholar 

  8. Agostinelliae S, Allisonas J, Amakoe K, Apostolakisa J, Araujoaj H, Arcel P, Asaig M, Axeni D, Banerjeeb S, Barrandan G, Behner F, Bellagambac L, Boudreaubd J, Brogliaar L, Brunengoc A, Burkhardt H, Chauvie S, Chuma J, Chytracek R, Cooperman G, Cosmo G, Degtyarenko P, Dell’Acqua A, Depaolay G, Dietrich D, Enami R, Feliciello A, Ferguson C, Fesefeldt H, Folger G, Foppiano F, Forti A, Garelli S, Giani S, Giannitrapani R, Gibin D, Gómez Cadenas JJ (2003) GEANT4-a simulation toolkit. Nucl Instrum Methods Phys Res Sect A 506(3):250–303

    Article  Google Scholar 

  9. Allison J, Amako K, Apostolakis J, Araujo H, Dubois PA, Asai M, Barrand G, Capra R, Chauvie S, Chytracek R, Cirrone GAP, Cooperman G, Cosmo G, Cuttone G, Daquino GG, Donszelmann M, Dressel M, Folger G, Foppiano F, Generowicz J, Grichine V, Guatelli S, Gumplinger P, Heikkinen A, Hrivnacova I, Howard A, Incerti S, Ivanchenko V, Johnson T, Jones F, Koi T, Kokoulin R, Kossov M, Kurashige H, Lara V, Larsson S, Lei F, Link O, Longo F, Maire M, Mantero A, Mascialino B, McLaren I, Lorenzo PM, Minamimoto K, Murakami K, Nieminen P, Pandola L, Parlati S, Peralta L, Perl J, Pfeiffer A, Pia MG, Ribon A, Rodrigues P, Russo G, Sadilov S, Santin G, Sasaki T, Smith D, Starkov N, Tanaka S, Tcherniaev E, Tome B, Trindade A, Truscott P, Urban L, Verderi M, Walkden A, Wellisch JP, Williams DC, Wright D, Yoshida H (2006) Geant4 developments and applications. IEEE Trans Nucl Sci 53(1):270–278

    Article  Google Scholar 

  10. Penn D, Biegalski S (2002) Monte Carlo simulations of prototype radioxenon beta–gamma counting systems. In: Trombka JI, Spears DP, Solomon PH (eds) Unattended radiation sensor systems for remote applications. American Institute of Physics, College Park, pp 17–27

    Google Scholar 

  11. Haas DA, Biegalski SR, Folz Biegalski KM (2008) Modeling β-γ coincidence spectra of 131mXe, 133Xe, 133mXe, and 135Xe. J Radioanal Nucl Chem 277(3):561–565

    Article  CAS  Google Scholar 

  12. Farsoni AT, Alemayehu B, Alhawsawi A, Becker EM (2013) A phoswich detector with compton suppression capability for radioxenon measurements. IEEE Trans Nucl Sci 60(1):456–464

    Article  CAS  Google Scholar 

  13. Alemayehu B, Farsoni AT, Ranjbar L (2014) A well-type phoswich detector for nuclear explosion monitoring. J Radioanal Nucl Chem 301:323–332

    Article  CAS  Google Scholar 

  14. Heimbigner TR, Bowyer TW, McIntyre JI, Abel KH, Hayes JC, Panisko ME, Pitts WK (2000) The DOE automated radioxenon sampler-analyzer (ARSA) beta–gamma coincidence spectrometer data analyzer. In: Proceedings of the 22nd annual DoD/DOE seismic research symposium, planning for verification of and compliance with the comprehensive nuclear-test-ban treaty (CTBT) held in New Orleans, Louisiana on September, pp 13–15

  15. McIntyre JI, Abel KH, Bowyer TW, Hayes JC, Heimbigner TR, Panisko ME, Reeder PL, Thompson RC (2001) Measurements of ambient radioxenon levels using the automated radioxenon sampler/analyzer (ARSA). J Radioanal Nucl Chem 248(3):629–635

    Article  CAS  Google Scholar 

  16. Axelsson A, Ringbom A (2014) On the calculation of activity concentrations and nuclide ratios from measurements of atmospheric radioactivity. Appl Radiat Isot 92:12–17

    Article  CAS  Google Scholar 

  17. Peräjärvi K, Eronen T, Elomaa V-V, Hakala J, Jokinen A, Kettunen H, Kolhinen VS, Laitinen M, Moore ID, Penttilä H, Rissanen J, Saastamoinen A, Toivonen H, Turunen J, Äystö J (2010) Ultra-high resolution mass separator—application to detection of nuclear weapons tests. Appl Radiat Isot 68(3):450–453

    Article  Google Scholar 

  18. Peräjärvi K, Turunen J, Hakala J, Jokinen A, Moore ID, Penttilä H, Saastamoinen A, Siiskonen T, Toivonen H, Äystö J (2008) The decay of 133mXe. Appl Radiat Isot 66(4):530–534

    Article  Google Scholar 

  19. Keillor ME, Cooper MW, Hayes JC, McIntyre JI (2009) Degradation of 81 keV 133 Xe gamma-rays into the 31 keV X-ray peak in CsI scintillators. J Radioanal Nucl Chem 282(3):699–702

    Article  CAS  Google Scholar 

  20. Reeder PL, Bowyer TW, McIntyre JI, Pitts WK, Ringbom A, Johansson C (2004) Gain calibration of a β/γ coincidence spectrometer for automated radioxenon analysis. Nucl Instrum Methods Phys Res Sect A 521(2–3):586–599

    Article  CAS  Google Scholar 

  21. Haas DA, Biegalski SR, Foltz Biegalski KM (2009) Radioxenon production through neutron irradiation of stable xenon gas. J Radioanal Nucl Chem 282(3):677–680

    Article  CAS  Google Scholar 

  22. Peräjärvi K, Eronen T, Cagniant A, Gorelov D, Hakala J, Jokinen A, Kankainen A, Kettunen H, Kolhinen VS, Laitinen M, Moore ID, Penttilä H, Rissanen J, Saastamoinen A, Toivonen H, Turunen J, Äystö J (2013) Production of pure samples of 131mXe and 135Xe. Appl Radiat Isot 71(1):34–36

    Article  Google Scholar 

  23. Ely JH, Schrom BT, Cooper MW, McIntyre JI, Haas DA, Hayes, JC (2011) Software for calculations of xenon radioisotope concentrations. PNNL-20530 Pacific Northwest National Laboratory, Richland, Washington

  24. Browne E, Firestone RB (1986) Table of radioactive isotopes. John Wiley & Sons, New York

    Google Scholar 

  25. McIntyre JI, Bowyer TW, PL Reeder (2006) Calculation of minimum-detectable-concentration levels of radioxenon isotopes using the PNNL ARSA system. PNNL-13102 Pacific Northwest National Laboratory, Richland, Washington

  26. Kalinowski MB, Axelsson A, Bean M, Blanchard X, Bowyer TW, Brachet G, Hebel S, McIntyre JI, Peters J, Pistner C, Raith M, Ringbom A, Saey PRJ, Schlosser C, Stocki TJ, Taffary T, Kurt Ungar R (2010) Discrimination of nuclear explosions against civilian sources based on atmospheric xenon isotopic activity ratios. Pure Appl Geophys 167(4–5):517–539

    Article  Google Scholar 

  27. Schoengold CR, DeMarre ME, Kirkwood EM (1996) Radiological effluents released from U.S. continental tests 1961 through 1992. DOE/NV-317 (Rev. 1) UC-702 Bechtel Nevada, Las Vegas

  28. Ely JH, Cooper MW, Haas DA, Hayes JC, Heimbigner TR, Schrom BT (2011) Interference terms for xenon. In: 2011 Monitoring research review, Los Alamos National Laboratory, Los Alamos, vol 1, pp 664–670

  29. On-site Inspection IFE14 Jordan. https://www.ctbto.org/specials/integrated-field-exercise-2014/. Accessed Oct 14 2015

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Acknowledgments

The authors wish to acknowledge the funding support of the Office of Nuclear Detonation Detection (NA-222), Office of Defense Nuclear Nonproliferation R&D (NA-22), Office of Defense Nuclear Nonproliferation (NA-20), and the National Nuclear Security Administration.

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McIntyre, J.I., Schrom, B.T., Cooper, M.W. et al. A program to generate simulated radioxenon beta–gamma data for concentration verification and validation and training exercises. J Radioanal Nucl Chem 307, 2381–2387 (2016). https://doi.org/10.1007/s10967-015-4620-5

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