Abstract
The International Atomic Energy Agency (IAEA) is committed to strengthening and streamlining the overall effectiveness of the IAEA safeguards system within the context of the Non-Proliferation Treaty (NPT). The IAEA has investigated the use of environmental monitoring techniques and a variety of techniques were studied as part of extensive field trials. The efficacy of long-range monitoring depends on the availability of mobile signature isotopes or compounds and on the ability to distinguish the nuclear signatures from background signals and attribute them to a source. The Comprehensive Nuclear Test Ban Treaty (CTBT) also requires a variety of environmental sampling and analysis techniques. This paper serves as a scientific basis to start discussions of environmental sampling techniques that could be considered for wide-area monitoring for the detection of undeclared nuclear activities within the NPT or for the possible future use within the CTBT.
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Rosenberg R, Brachet G, Lauppe W-D, Vintersved I, Nicholson K, Krey P, Swindle D, Wogman NA, Hanlen RC, others (1999) IAEA use of wide-area environmental sampling in the detection of undeclared nuclear activities. Member State Support Programmes to the IAEA STR-321
Schoengold CR, DeMarre ME, Kirkwood EM (1961) Radiological effluents released from US continental tests 1961 through 1992. Bechtel Nevada, Las Vegas
IAEA (2001) Generic modes for use in assessing the impact of discharges of radioactive substances to the environment, safety series no. 19. International Atomic Energy Agency (IAEA), Vienna
Hetherington JA (1976) The behavior of plutonium nuclides in the Irish Sea. In: Miller MW, Stannard JN (eds) Environmental toxicity of aquatic radionuclides: models and mechanisms. Anna Arbor Science Publishers, Ann Arbor, pp 81–106
Jinks SM, Wrenn ME (1975) Chapter 11, radiocesium transport in the Hudson River Estuary. In: Miller MW, Stannard JN (eds) Environmental toxicity of aquatic radionuclides: models and mechanisms. Anna Arbor Science Publishers, Ann Arbor
Margvelashvily N, Maderich V, Zheleznyak M (1997) THREETOX_A computer code to simulate three-dimensional dispersion of radionuclides in stratified water bodies. Radiat Protect Dosim 73(1–4):177–180
Okubo A (1971) Deep Sea Res 18:789–802
Onishi Y (1981) Sediment and contaminant transport model. J Hydraul Div 107(HY9):1089–1107
Onishi Y (1994) Chapter 11, contaminant transport models in surface waters. In: Chaudrey MH, Mays LW (eds) Computer modeling of free surface and pressurized flows, vol NATO ASI Series E applied sciences, vol 274. Kluwer Academic Publisher, Dordrecht, pp 313–341
Onishi Y (2008) Surface water transport of radionuclides. In: Till JE, Grogan HA (eds) Radiological risk assessment and environmental analysis. Oxford University Press, New York, pp 147–207
Onishi Y, Kivva SL, Zheleznyak MJ, Voitsehkovitch OV (2007) Aquatic assessment of the Chernobyl nuclear accident and its remediation. J Environ Eng 133(11):1015–1023
Onishi Y, Schreiber DL, Codell RB (1979) Chapter 18, mathematical simulation of sediment and radionuclide transport in the Clinch River, Tennessee. In: Baker RA (ed) Processes involving contaminants and sediments. Ann Arbor Scientific Publisher, Ann Arbor
Onishi Y, Trent DS (1985) Three-dimensional simulation of flow, salinity, sediment, radionuclide movements in the Hudson River Estuary. Paper presented at the Proceedings of the 1985 Specialty Conference of the Hydraulics Division, Lake Buena Vista, August 12–17, 1985
Onishi Y, Trent DS (1992) Turbulence modeling for deep ocean radionuclide. Int J Numer Methods Fluid 15(9):1059–1071
Onishi Y, Voitsehkovitch OV, Zheleznyak MJ (eds) (2007) Chernobyl–What have we learned? the successes and failures to mitigate water contamination over 20 years. Springer, Dordrecht
Shepeleva T, Sizonenko V, Mezhneva I (1997) Simulation of countermeasure to diminish radionuclide fluxes from Chernobyl zone via aquatic pathways. Radiat Protect Dosim 73:177–180
Voitsehkovitch OV, Zheleznyak MJ, Onishi Y (1994) Chernobyl nuclear accident hydrologic analysis and emergency evaluation of radionuclide distributions in the Dnieper River, Ukraine during the 1993 summer flood. Pacific Northwest Laboratory, Richland
Zheleznyak M, Donchytz G, Hygynyak V, Marinetz A, Lyahenko G, Tkalitz P (2003) RIVTOX–One dimensional model for the simulation of the transport of radionuclides in a network of river channels. Institute of Mathematical Machines and System Problems, Kiev
Bowyer TW, Abel KH, Hensley WK, Hubbard CW, Panisko ME, Perkins RW, Reeder PL, Thompson RC, Warner RA (1996) Automatic radioxenon analyzer for CTBT monitoring. Pacific Northwest National Laboratory, Richland
Bowyer TW, Abel KH, Hensley WK, Panisko ME, Perkins RW (1997) Ambient 133Xe levels in the Northeast US. J Environ Radioact 37:143–153
Bowyer TW, Abel KH, Hubbard CW, Panisko ME, Reeder PL, Thompson RC, Warner RA (1998) Automated separation and measurement of radioxenon for the comprehensive test ban treaty. J Radioanal Nucl Chem 235:77–81
Bowyer TW, Abel KH, Hubbard CW, Panisko ME, Reeder PL, Thompson RC, Warner RA (1998) Field testing of collection and measurement of radioxenons for the comprehensive test ban treaty. J Radioanal Nucl Chem 240:109–122
Bowyer TW, Hayes JC, McIntyre JI (2007) Environmental measurements of radioxenon. In: Warwick P (ed) Environmental radiochemical analysis III. RSC Publishing, Cambridge, pp 44–51
Bowyer TW, Perkins RW, Abel KH, Hensley WK, Hubbard CW, McKinnon AD, Panisko ME, Reeder PL, Thompson RC, Warner RA (1998) Xenon radionuclides: atmospheric monitoring. In: Meyers RA (ed) Encyclopedia of environmental analysis and remediation, vol 8. Wiley-Interscience, New York, pp 5295–5314
Bowyer TW, Schlosser C, Abel KH, Auer M, Hayes JC, Heimbigner TR, McIntyre JI, Panisko ME, Reeder PL, Satorius H, Schulze J, Weiss W (2002) Detection and analysis of Xenon isotopes for the comprehensive Nuclear-Test-Ban Treaty International Monitoring System. J Environ Radioact 59(2):139–151
Carman AJ, Bowyer TW, Hayes JC, Heimbigner TR, McIntyre JI, Panisko ME (2002) Discrimination between anthropogenic sources of atmospheric radioxenon. Paper presented at the Transactions of the 2002 ANS Winter Meeting, Washington, November 17–21, 2002
Cooper MW, Bowyer TW, Hayes JC, Heimbigner TR, Hubbard CW, McIntyre JI, Schrom BT (2008) Spectral analysis of radioxenon. Paper presented at the Proceedings of the 30th Monitoring Research Review: Ground-Based Nuclear Explosion Monitoring Technologies, Portsmouth, September 23–25, 2008
Le Petit G, Armand P, Brachet G, Taffary T, Fontaine J, Achim P, Blanchard X, Piwowarczyk J, Pointurier F (2008) Contribution to the development of atmospheric radioxenon monitoring. J Radioanal Nucl Chem 276(2):391–398
Prelovskii VV, Kazarinov NM, Donets AY, Popov VY, Popov IY, Skirda NV (2007) The ARIX-03F mobile semiautomatic facility for measuring low concentrations of radioactive xenon isotopes in air and subsoil gas. Prib Tekh Eksp 3:117–121
Ringbom A, Larson T, Axelsson A, Elmgren K, Johansson C (2003) SAUNA-A system for automatic sampling, processing, and analysis of radioactive xenon. Nucl Instrum Meth Phys Res A 508(3):542–553
NCRP (1975) Krypton-85 in the atmosphere-accumulation, biological, significance, and control technology. Task group on 85Kr of the Council’s Scientific Committee 38 on waste disposal, National Council on Radiation Protection and Measurements (NCRP), Bethesda
Jenkins CE, Wogman NA, Rieck HG (1972) Radionuclide distribution in Olympic National Park Washington. Water Air Soil Pollut 1(2):181–204
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Wogman, N.A. Prospects for the introduction of wide area monitoring using environmental sampling for proliferation detection. J Radioanal Nucl Chem 296, 1071–1077 (2013). https://doi.org/10.1007/s10967-012-2076-4
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DOI: https://doi.org/10.1007/s10967-012-2076-4