First measurements of 238Pu and 238Pu/137Cs activity ratio in Montenegro soil

  • Nevenka M. Antovic
  • Perko Vukotic
  • Nikola Svrkota
  • Sergey K. Andrukhovich
Article

Abstract

Plutonium-238 (238Pu) activity concentrations in soil samples from Montenegro (six samples from three localities) have been measured for the first time. The 238Pu/137Cs activity ratio was determined on the basis of alpha and gamma-spectrometric measurements, and found to be with an average of 0.0006 and standard deviation of 0.0003. By using the activity ratios determined in the present study, 238Pu activity concentrations were estimated for three localities in the central: one in the northern, and two in the eastern part of Montenegro.

Keywords

238Pu activity 238Pu/137Cs ratio Soil Montenegro 

References

  1. 1.
    Sarcevic L, Mihalj A, Kljajic R, Hasanbasic D, Horsic E, Milosevic Z (1983) Migration of Sr-90 and Cs-137 in soils depending on type of soil and altitude. In: Proceedings of the XII Yugoslav symposium on radiation protection, Ohrid, 31 May–3 June 1983, pp 124–127 (in Serbian)Google Scholar
  2. 2.
    Vukotic P, Antovic N, Dapchevic S, Borisov GI, Kuzmich VV, Kulakov VM, Mirkovic M, Pajovic M, Svrkota R, Fustic B, Djuretic G, Dlabach A (1997) Background gamma-radiation in Montenegro. In: IRPA regional symposium—radiation protection in neighboring countries of central Europe, Prague, pp 477–479Google Scholar
  3. 3.
    Andreev VV, Bykov VT, Vodin AN, Maksimenko NV, Olejnik SN, Rudak EA, Tulubtsov AJ (2005) The evaluation of plutonium emission in the aerosol form after the accident in the Chernobyl NNP. Preprint of Institute of Physics NAN B, 742, Minsk (in Russian)Google Scholar
  4. 4.
    Kulakov VM, Kulazhko VG, Lisin SK (1990) Experimental determination of the correlation coefficient between plutonium isotopes and Ce-144 content in soil. Ser Nucl Phys Res 5:149–150 (in Russian)Google Scholar
  5. 5.
    Antovic N, Rudak EA, Tulubtsov AJ, Vukotic P (2005) Correlations significant for estimation of transuranium isotopes activities. In: Proceedings of XXIII symposium of the Serbia and Montenegro radiation protection society, Donji Milanovac, Serbia, pp 157–160 (in Serbian)Google Scholar
  6. 6.
    HASL-300 (1997) EML Procedures manual. Environmental measurements laboratory, US. Department of Energy, 28th ednGoogle Scholar
  7. 7.
    Antovic NM, Vukotic P, Svrkota N, Andrukhovich SK (2012) Pu-239+240 and Cs-137 in Montenegro soil—their correlation and origin. J Environ Radioact (Submitted)Google Scholar
  8. 8.
    Vesterbacka P, Vartti VP, Heikkinen T, Ikaheimonen TK (2010) High-grade radiochemical analyses act a basis for good assessment in radiation protection. In: Proceedings of the third European IRPA Congress, Helsinki, Finland. http://www.irpa2010europe.com/proceedings/P12/P12-10.pdf
  9. 9.
    Hölgye Z, Schlesingerová E, Tecl J, Filgas R (2004) 238Pu, 239,240Pu, 241Am, 90Sr and 137Cs in soils around nuclear research centre Rez, near Prague. J Environ Radioact 71(2):115–125CrossRefGoogle Scholar
  10. 10.
    Baggoura B, Noureddine A, Benkrid M (1998) Level of natural and artificial radioactivity in Algeria. Appl Radiat Isot 49(7):867–873CrossRefGoogle Scholar
  11. 11.
    Al Hamarneh I, Wreikat A, Toukan K (2003) Radioactivity concentrations of 40K, 134Cs, 137Cs, 90Sr, 241Am, 238Pu and 239+240Pu radionuclides in Jordanian soil samples. J Environ Radioact 67(1):53–67CrossRefGoogle Scholar
  12. 12.
    Suplińska M, Adamczyk A (2009) Distribution of Cs-137, Pu-239,240, Pu-238, Sr-90, and Ra-226 in bottom sediments of southern Baltic Sea in 2008. Helsinki Commission HELCOM MORS-PRO 14/2009. Project group for monitoring of radioactive substances in the Baltic Sea (MORS), 14th meeting Stockholm, Sweden, 5–7 MayGoogle Scholar
  13. 13.
    Jia G, Testa C, Desideri D, Guerra F, Meli MA, Roselli C, Belli ME (1999) Soil concentration, vertical distribution and inventory of plutonium, 241Am, 90Sr and 137Cs in the Marche region of central Italy. Health Phys 77(1):52–61CrossRefGoogle Scholar
  14. 14.
    Popov L, Mihailova G, Naidenov I (2010) Determination of activity ratios of 238, 239+240,241Pu, 241Am, 134,137Cs and 90Sr in Bulgarian soils. J Radioanal Nucl Chem 285:223–237CrossRefGoogle Scholar
  15. 15.
    Eikenberg J, Bajo S, Hitz J, Wyer L (2001) Environmental radionuclide analyses around nuclear installations in northern Switzerland. http://www.lanl.gov/BAER-onference/BAERCon-47p-Eikenberg.pdf
  16. 16.
    Danesi PR, Bleise A, Burkart W, Cabianca T, Campbell MJ, Makarewicz M, Moreno J, Tuniz C, Hotchkis M (2003) Isotopic composition and origin of uranium and plutonium in selected soil samples collected in Kosovo. J Environ Radioact 64(2–3):121–131CrossRefGoogle Scholar
  17. 17.
    Hardy EP, Krey PW, Volchok HL (1973) Global inventory and distribution of fallout plutonium. Nature 241:444–445CrossRefGoogle Scholar
  18. 18.
    Yamamoto M, Tsumura A, Katayama Y, Tsukatami T (1996) Plutonium isotopic composition in soil from the former semipalatinsk nuclear test site. Radiochim Acta 72:209–215Google Scholar
  19. 19.
    Pavlotskaya FI, Myasoedov BF (1991) Plutonium in soils. Priroda 5:57–61 (in Russian)Google Scholar
  20. 20.
    Carbol P, Solatie D, Erdmann N, Nylen T, Betti M (2003) Deposition and distribution of Chernobyl fallout fission products and actinides in a Russian soil profile. J Environ Radioact 68(1):27–46CrossRefGoogle Scholar
  21. 21.
    Irweck K, Wickie J (1998) Isotopic composition of plutonium emissions in Austria after the Chernobyl accident. J Radioanal Nucl Chem 227(1–2):133–136CrossRefGoogle Scholar

Copyright information

© Akadémiai Kiadó, Budapest, Hungary 2012

Authors and Affiliations

  • Nevenka M. Antovic
    • 1
  • Perko Vukotic
    • 2
  • Nikola Svrkota
    • 3
  • Sergey K. Andrukhovich
    • 4
  1. 1.Faculty of Natural Sciences and MathematicsUniversity of MontenegroPodgoricaMontenegro
  2. 2.Montenegrin Academy of Sciences and ArtsPodgoricaMontenegro
  3. 3.Center for Ecotoxicological ResearchPodgoricaMontenegro
  4. 4.B. I. Stepanov Institute of Physics, National Academy of Sciences of BelarusMinskBelarus

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