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Comparative study of different types of granular activated carbon in removing medium level radon from water

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Abstract

Granular activated carbon (GAC) has proven its effectiveness in removing radon from water supplies. Laboratory and pilot plant studies were carried out using three different types of activated carbons (F-300, F-400, and HD-4000) to remove radon from water supply. From the experimental kinetic study, the data indicated that at least 6 h are needed to attain equilibrium between radon activity adsorbed onto carbon and its concentration in the aqueous phase. Also, it showed that HD-4000 has higher capacity for removing radon than the other two investigated carbons F-300 and F-400. The adsorption isotherms were satisfactorily explained by Freundlich equation. In the pilot plant study, the performance of the three activated carbons in removing radon at medium concentration (~111 Bq dm−3) was evaluated over 60 days of continuous water flow. Four empty-bed contact times (EBCTs) corresponding to four bed depths were continuously monitored and the corresponding steady state adsorption-decay constant values were calculated and the efficiency of each carbon was used to provide a facet for comparison. The γ-radiation exposure rate distribution throughout each GAC bed was measured and compared. This study, despite paucity of literature in this field, is useful for designing a GAC adsorption system for the removal of medium level radon concentration from water supplies.

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References

  1. Hess CT, Wiffenbach CV, Norton SA (1983) Environmental radon and cancer correlations in Maine. J Health Phys 45(2):339–348

    Article  CAS  Google Scholar 

  2. Cross FT, Harley NH, Hofmann W (1985) Health effects and risks from Rn-222 in drinking water. J Health Phys 48(5):649–670

    Article  CAS  Google Scholar 

  3. Mills WA (1990) Risk assessment and control management of radon in drinking water. In: Cothern CR, Rebers PA (eds) Radon, Radium and Uranium in drinking water. Lewis Publishers, Chelsea, pp 27–37

    Google Scholar 

  4. Crawford-Brown DJ (1990) Analysis of the health risk from ingested radon. In: Cothern CR, Rebers PA (eds) Radon, Radium and Uranium in drinking water. Lewis Publishers, Chelsea, pp 17–26

    Google Scholar 

  5. Crawford-Brown DJ (1992) Cancer risk from radon. J AWWA 84(3):77–81

    CAS  Google Scholar 

  6. Lowry JD, Moreau E (1986) Removal of extreme radon and uranium from a water supply. In: Proceedings of the ASCE national conference on environmental engineering, Cincinnati

  7. Lowry JD, Brandow JE (1985) Removal of radon from water supplies. J Environ Eng 111(4):511–527

    Article  CAS  Google Scholar 

  8. US Environmental Protection Agency (USEPA) (1991) National primary drinking water regulations; radionuclides; proposed rule. Fed Reg, vol 56, no 138, USA.

  9. Pontius FW (2002) Regulatory compliance planning to ensure water supply safety. J AWWA 94(3):52–64

    CAS  Google Scholar 

  10. US Environmental Protection Agency (USEPA) (1990) Waste by-products document in support of drinking water treatment BAT cost analyses. Prepared by Malcolm Pirnie Inc. for Office of Drinking Water, USA

  11. Alabdula’aly AI, Maghrawy HB (1999) Radon removal from water supplies by diffused bubble aeration system. J Radioanal Nucl Chem 241(1):3–9

    Article  Google Scholar 

  12. Lowry JD, Brandow JE (1981) Removal of radon from groundwater supplies using granular activated carbon or diffused aeration. Research Technical Report, University of Maine, USA

  13. Kinner NE, Jr Malley JP, Clement JA, Fox KR (1993) Using POE techniques to remove radon. J AWWA 85(6):75–86

    CAS  Google Scholar 

  14. Lowry JD, Lowry SB, Cline JK (1991) Radon removal by POE GAC systems: design, performance, and cost. EPA/600/52-90/049, Springfield, VA. National Technical Information Service, PB 91-125-633, AS, USA

  15. STUK-A 169 (2000) Treatment techniques for removing natural radionuclides from drinking water. Helsinki, Finland, 101 pp

  16. Lykins BW Jr, Clark RM, Goodrich JA (1992) Point-of-use/point-of-entry for drinking water treatment. Lewis Publishers, Chelsea

    Google Scholar 

  17. Markkanen M (2005) Technical guidance on safe installation of a GAC filter used for removing radon from water. Radioact Environ 7:665–669

    Article  CAS  Google Scholar 

  18. Raucher RS, Drago J (1992) Estimating the cost of compliance with the drinking water standard for radon. J AWWA 84(3):51–65

    CAS  Google Scholar 

  19. Prichard HM, Gesell TF (1977) Rapid measurements of radon-222 concentration in water with a commercial liquid scintillation counter. J Health Phys 33(12):577–581

    Article  CAS  Google Scholar 

  20. Snoeyink VL (1990) Adsorption of organic compounds. In: Pontius FW (ed) Water quality and treatment: a handbook of community water supplies, chap 13, 4th edn. American Water Works Association, McGraw-Hill, London, pp 781–875

    Google Scholar 

  21. Lowry JD, Brutsaert WF, Mcenerney T, Make C (1987) Point-of-entry removal of radon from drinking water. J AWWA 79(4):162–169

    CAS  Google Scholar 

  22. Reed DF (1989) Radon treatment for a Maine public water supply. SEA Consultants, Cambridge

    Google Scholar 

  23. Turtiainen T, Salonen L, Myllymaki P (2000) Radon removal from different types of groundwater applying granular activated carbon filtration. J Radioanal Nucl Chem 243(2):423–432

    Article  CAS  Google Scholar 

  24. Salonen L (1994) Future groundwater resources at risk. In: Proceedings of the Helsinki conference. IAHS Publ. no. 222, p 71

  25. Finnish Radiation and Nuclear Safety (1993) The radioactivity of household water. ST-Guide 12.3. Finnish Centre for Radiation and Nuclear Safety, Helsinki

  26. Valentine RL, Stearns S, Kurt A, Walsh D, Mielke W (1992) Radon and radium from distribution system and filter media deposits. WQTC, Toronto, pp 15–19

    Google Scholar 

  27. Lowry JD, Lowry SB (1987) Modeling point-of-entry radon removal by GAG. J AWWA 79(10):85–88

    CAS  Google Scholar 

  28. Weber WJ Jr (1972) Physiochemical processes for water quality control. Wiley, New York

    Google Scholar 

  29. Snoeyink VL (1983) Control strategy—adsorption techniques; occurrence and removal of volatile organic chemical from drinking water. AWWA Cooperative Research Report, Denver, USA

  30. Evans RD (1969) Engineer’s guide to the elementary behavior of radon daughters. J Health Phys 17(2):229–252

    Article  CAS  Google Scholar 

  31. Rydell S, Keene B, Lowry J (1989) Granular activated carbon water treatment and potential radiation hazards. J NEWWA 103(4):234–248

    CAS  Google Scholar 

Download references

Acknowledgments

The work reported has been funded by King Abdulaziz City for Science and Technology (KACST), Riyadh, Saudi Arabia whom the authors appreciate.

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  1. King Abdulaziz City for Science and Technology, P.O. Box 6086, Riyadh, 11442, Saudi Arabia

    Abdulrahman I. Alabdula’aly & Hamed B. Maghrawy

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  1. Abdulrahman I. Alabdula’aly
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  2. Hamed B. Maghrawy
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Correspondence to Abdulrahman I. Alabdula’aly.

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Alabdula’aly, A.I., Maghrawy, H.B. Comparative study of different types of granular activated carbon in removing medium level radon from water. J Radioanal Nucl Chem 287, 77–85 (2011). https://doi.org/10.1007/s10967-010-0804-1

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