Abstract
Lutetium has been used as a radiochemistry detector to measure neutron fluence in NTS tests. A measure of the neutron capture cross sections on 173Lu is needed to improve the interpretation value of the Lu radiochemistry isotopic ratios. A natural hafnium target was irradiated with protons to produce neutron poor lutetium radioisotopes. The short lived species were allowed to decay prior to chemical processing resulting in predominantly 173Lu with a small amount of 174Lu. This material was deposited on a titanium foil for use in the neutron capture cross section measurement.
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Acknowledgments
The authors would like to thank Los National Laboratory groups C-IIAC, C-NR, LANSCE-NS, IPF, Lujan Center, LANSCE accelerator facility, LDRD support, and the LANS LLC. This measurement is supported out the stockpile stewardship program by DOE/NNSA under the auspices of the US Department of Energy at Los Alamos National Laboratory by the Los Alamos National Security LLC, Contract No. DE-AC52-06NA25396.
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Taylor, W.A., Rundberg, R.S., Bond, E.M. et al. Production of a 173Lu target for neutron capture cross section measurements. J Radioanal Nucl Chem 282, 391–394 (2009). https://doi.org/10.1007/s10967-009-0278-1
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DOI: https://doi.org/10.1007/s10967-009-0278-1