Abstract
FeNi/glass composites with 0 wt%,1 wt%, and 2 wt% glass content are produced, and their soft magnetic properties are systematically studied. The scanning electron microscope (SEM) results indicate that the FeNi particles are surrounded by glass powder. With the addition of glass powder, the saturation magnetization of the FeNi/glass composites decreases from 170 to 158 emu/g, and the effective permeability decreases from 56.1 to 39.1. With the increase of glass content, the imaginary part μ″ is reduced, indicating that the eddy current loss or excess loss is reduced at high frequency. The magnetic loss measurement results show that the addition of glass powder greatly reduces the eddy current loss. Furthermore, the FeNi/glass composite core with 2 wt% glass content has moderate permeability, higher quality factor Q, and better DC bias characteristics than other cores. The results show that the ideal glass powder content can improve the magnetic properties of FeNi composite materials, and glass powder can be used as an insulator in soft magnetic composites (SCMs).
Similar content being viewed by others
References
Perigo, E., Weidenfeller, B., Kollar, P., Fuzer, J.: Past, present, and future of soft magnetic composites. Appl. Phys. Rev. 5, 031301 (2018)
Shokrollahi, H., Janghorban, K.: Soft magnetic composite materials(SMCs). J. Mater. Process. Technol. 189, 1–12 (2007)
Silveyra, J., Ferrara, E., Huber, D., Monson, T.: Soft magnetic materials for a sustainable and electrified world. Science 362, eaao0195 (2018)
Hu, F., Ni, J., Feng, S., Kan, X., Yang, Y., Lv, Q., Liu, X.: Soft magnetic properties of Fe-6.5wt%Si/SrFe12O19 composites. J. Supercond. Nov. Magn. 33, 2779–2785 (2020)
Hu, F., Ni, J., Feng, S., Kan, X., Zhu, R., Yang, W., Yang, Y., Lv, Q., Liu, X.: Low melting glass as adhesive and insulating agent for soft magnetic composites: case in FeSi powder core. J. Magn. Magn. Mater. 501, 1–6 (2020)
Hou, Z., Yan, P., Sun, B., Elshekh, H., Yan, B.: An excellent soft magnetic Fe/Fe3O4-FeSiAl composite with high permeability and low core loss. Results Phys. 14, 102498 (2019)
Chen, Z., Liu, X., Kan, X., Wang, Z., Zhu, R., Yang, W., Wu, Q., Shezad, M.: Phosphate coatings evolution study and effects of ultrasonic on soft magnetic properties of FeSiAl by aqueous phosphoric acid solution passivation. J. Alloy. Compd. 783, 434–440 (2019)
Suna, H., Lin, Z., Chen, Y., Chen, F., Qu, X., Xie, C., Zhang, L.: Magnetic properties of iron-based soft magnetic composites prepared by utilizing polyimide insulating layer. J. Magn. Magn. Mater. 486, 165287 (2019)
Strečková, M., Medvecký, Ľ, Füzer, J., Kollár, P., Bureš, R., Fáberová, M.: Design of novel soft magnetic composites based on Fe/resin modified with silica. Mater. Lett. 101, 37–40 (2013)
Chen, Z., Liu, X., Kan, X., Wang, Z., Zhu, R., Yang, W., Wang, Y., Hu, X., Wu, Q., Rehman, K., Shezad, M.: Study on the properties of novel soft magnetic composites of FeSiAl. J. Supercond. Nov. Magn. 32, 1805–1809 (2019)
Peng, Y., Yi, Y., Li, L., Yi, J., Nie, J., Bao, C.: Iron-based soft magnetic composites with Al2O3 insulation coating produced using sol–gel method. Mater. Design. 109, 390–395 (2016)
Luo, F., Fan, X., Luo, Z., Hu, W., Wang, J., Wu, Z., Li, G., Li, Y., Liu, X.: Microstructure, formation mechanism and magnetic properties of Fe1.82Si0.18@Al2O3 soft magnetic composites. J. Magn. Magn. Mater. 493, 165744 (2020)
Zhong, X., Chen, J., Wang, L., Li, B., Li, L.: Properties of FeSiAl-based soft magnetic composites with AlN/Al2O3 and hybrid phosphateesilane insulation coatings. J. Alloy. Compd. 735, 1603–1610 (2018)
Luo, F., Fan, X., Luo, Z., Hu, W., Wang, J., Wu, Z., Li, G., Li, Y., Liu, X.: Preparation and magnetic properties of FeSiAl-based soft magnetic composites with MnO/Al2O3 insulation layer. J. Magn. Magn. Mater. 498, 166084 (2020)
Wu, Z., Fan, X., Li, G., Wang, J., Gan, Z.: Inter granular insulated Fe-6.5 wt% Si/SiO2 composite compacts with tunable insulating layer thickness for low core loss applications. RSC Adv. 5, 67031 (2015)
Fan, X., Wang, J., Wu, Z., Li, G.: Core–shell structured FeSiAl/SiO2 particles and Fe3Si/Al2O3 soft magnetic composite cores with tunable insulating layer thicknesses. Mat. Sci. Eng. R. 201, 79–86 (2015)
Li, L., Gao, Z., Li, A., Yi, J.: Ge, Y: Fabrication of carbonyl iron powder/SiO2–reduced iron powder/SiO2 soft magnetic composites with a high resistivity and low core loss. J. Magn. Magn. Mater. 464, 161–167 (2018)
Geng, K., Xie, Y., Xu, L., Yan, B.: Structure and magnetic properties of ZrO2-coated Fe powders and Fe/ZrO2 soft magnetic composites. Adv. Powder. Technol. 28, 2015–2022 (2017)
Geng, K., Xie, Y., Yan, L., Yan, B.: Fe-Si/ZrO2 composites with core-shell structure and excellent magnetic properties prepared by mechanical milling and spark plasma sintering. J. Alloy. Compd. 718, 53–62 (2017)
Peng, Y., Yi, Y., Li, L., Ai, H., Wang, X., Chen, L.: Fe-based soft magnetic composites coated with NiZn ferrite prepared by a co-precipitation method. J. Magn. Magn. Mater. 428, 148–153 (2017)
Lauda, M., Füzer, J., Kollár, P., Strečková, M., Bureš, R., Kováč, J., Baťková, M., Baťko, I.: Magnetic properties and loss separation in FeSi/MnZnFe2O4 soft magnetic composites. J. Magn. Magn. Mater. 411, 12–17 (2016)
Li, J., Peng, X., Yang, Y., Ge, H.: Preparation and characterization of MnZn/FeSiAl soft magnetic composites. J. Magn. Magn. Mater. 426, 132–136 (2017)
Chicinasa, I., Geoffroy, O., Isnard, O., Pop, V.: Soft magnetic composite based on mechanically alloyed nanocrystalline Ni3Fe phase. J. Magn. Magn. Mater. 290–291, 1531–1534 (2005)
Stoppels, D.: Developments in soft magnetic power ferrites. J. Magn. Magn. Mater. 160, 323–328 (1996)
Zhu, S., Ni, J., Feng, S.: Investigation on magnetic power loss in strontium doped Ba1-xSrxTi1.2Co1.2Fe9.6O19 hexaferrites. Mater. Res. Express. 6, 116–122 (2019)
Zhou, Y., Kou, X., Mu, M., Brandon, M., Chen, X.: Loss characterization of Mo-doped FeNi flake for DC-to-DC converter and MHz frequency applications. J. Appl. Phys. 111, 07E329 (2012)
Funding
This work was supported by the National Natural Science Foundation of China (No. 51872004), by the Education Department of Anhui Province (Nos. KJ2019ZD03, KJ2013B293, KJ2018A0039) and by the Key Research and Development Plan of Anhui Province(No. 201904a05020038).
Author information
Authors and Affiliations
Corresponding authors
Ethics declarations
Competing Interests
The authors declare no competing interests.
Additional information
Publisher's Note
Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.
Rights and permissions
About this article
Cite this article
Zhu, S., Wang, Z., Kan, X. et al. FeNi/Glass Soft Magnetic Composites with High Magnetic Properties. J Supercond Nov Magn 35, 1165–1172 (2022). https://doi.org/10.1007/s10948-022-06166-z
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s10948-022-06166-z