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FeNi/Glass Soft Magnetic Composites with High Magnetic Properties

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Abstract

FeNi/glass composites with 0 wt%,1 wt%, and 2 wt% glass content are produced, and their soft magnetic properties are systematically studied. The scanning electron microscope (SEM) results indicate that the FeNi particles are surrounded by glass powder. With the addition of glass powder, the saturation magnetization of the FeNi/glass composites decreases from 170 to 158 emu/g, and the effective permeability decreases from 56.1 to 39.1. With the increase of glass content, the imaginary part μ″ is reduced, indicating that the eddy current loss or excess loss is reduced at high frequency. The magnetic loss measurement results show that the addition of glass powder greatly reduces the eddy current loss. Furthermore, the FeNi/glass composite core with 2 wt% glass content has moderate permeability, higher quality factor Q, and better DC bias characteristics than other cores. The results show that the ideal glass powder content can improve the magnetic properties of FeNi composite materials, and glass powder can be used as an insulator in soft magnetic composites (SCMs).

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References

  1. Perigo, E., Weidenfeller, B., Kollar, P., Fuzer, J.: Past, present, and future of soft magnetic composites. Appl. Phys. Rev. 5, 031301 (2018)

    Article  ADS  Google Scholar 

  2. Shokrollahi, H., Janghorban, K.: Soft magnetic composite materials(SMCs). J. Mater. Process. Technol. 189, 1–12 (2007)

    Article  Google Scholar 

  3. Silveyra, J., Ferrara, E., Huber, D., Monson, T.: Soft magnetic materials for a sustainable and electrified world. Science 362, eaao0195 (2018)

    Article  Google Scholar 

  4. Hu, F., Ni, J., Feng, S., Kan, X., Yang, Y., Lv, Q., Liu, X.: Soft magnetic properties of Fe-6.5wt%Si/SrFe12O19 composites. J. Supercond. Nov. Magn. 33, 2779–2785 (2020)

    Article  Google Scholar 

  5. Hu, F., Ni, J., Feng, S., Kan, X., Zhu, R., Yang, W., Yang, Y., Lv, Q., Liu, X.: Low melting glass as adhesive and insulating agent for soft magnetic composites: case in FeSi powder core. J. Magn. Magn. Mater. 501, 1–6 (2020)

    Article  Google Scholar 

  6. Hou, Z., Yan, P., Sun, B., Elshekh, H., Yan, B.: An excellent soft magnetic Fe/Fe3O4-FeSiAl composite with high permeability and low core loss. Results Phys. 14, 102498 (2019)

    Article  Google Scholar 

  7. Chen, Z., Liu, X., Kan, X., Wang, Z., Zhu, R., Yang, W., Wu, Q., Shezad, M.: Phosphate coatings evolution study and effects of ultrasonic on soft magnetic properties of FeSiAl by aqueous phosphoric acid solution passivation. J. Alloy. Compd. 783, 434–440 (2019)

    Article  Google Scholar 

  8. Suna, H., Lin, Z., Chen, Y., Chen, F., Qu, X., Xie, C., Zhang, L.: Magnetic properties of iron-based soft magnetic composites prepared by utilizing polyimide insulating layer. J. Magn. Magn. Mater. 486, 165287 (2019)

    Article  Google Scholar 

  9. Strečková, M., Medvecký, Ľ, Füzer, J., Kollár, P., Bureš, R., Fáberová, M.: Design of novel soft magnetic composites based on Fe/resin modified with silica. Mater. Lett. 101, 37–40 (2013)

    Article  Google Scholar 

  10. Chen, Z., Liu, X., Kan, X., Wang, Z., Zhu, R., Yang, W., Wang, Y., Hu, X., Wu, Q., Rehman, K., Shezad, M.: Study on the properties of novel soft magnetic composites of FeSiAl. J. Supercond. Nov. Magn. 32, 1805–1809 (2019)

    Article  Google Scholar 

  11. Peng, Y., Yi, Y., Li, L., Yi, J., Nie, J., Bao, C.: Iron-based soft magnetic composites with Al2O3 insulation coating produced using sol–gel method. Mater. Design. 109, 390–395 (2016)

    Article  Google Scholar 

  12. Luo, F., Fan, X., Luo, Z., Hu, W., Wang, J., Wu, Z., Li, G., Li, Y., Liu, X.: Microstructure, formation mechanism and magnetic properties of Fe1.82Si0.18@Al2O3 soft magnetic composites. J. Magn. Magn. Mater. 493, 165744 (2020)

    Article  Google Scholar 

  13. Zhong, X., Chen, J., Wang, L., Li, B., Li, L.: Properties of FeSiAl-based soft magnetic composites with AlN/Al2O3 and hybrid phosphateesilane insulation coatings. J. Alloy. Compd. 735, 1603–1610 (2018)

    Article  Google Scholar 

  14. Luo, F., Fan, X., Luo, Z., Hu, W., Wang, J., Wu, Z., Li, G., Li, Y., Liu, X.: Preparation and magnetic properties of FeSiAl-based soft magnetic composites with MnO/Al2O3 insulation layer. J. Magn. Magn. Mater. 498, 166084 (2020)

    Article  Google Scholar 

  15. Wu, Z., Fan, X., Li, G., Wang, J., Gan, Z.: Inter granular insulated Fe-6.5 wt% Si/SiO2 composite compacts with tunable insulating layer thickness for low core loss applications. RSC Adv. 5, 67031 (2015)

    Article  ADS  Google Scholar 

  16. Fan, X., Wang, J., Wu, Z., Li, G.: Core–shell structured FeSiAl/SiO2 particles and Fe3Si/Al2O3 soft magnetic composite cores with tunable insulating layer thicknesses. Mat. Sci. Eng. R. 201, 79–86 (2015)

    Article  Google Scholar 

  17. Li, L., Gao, Z., Li, A., Yi, J.: Ge, Y: Fabrication of carbonyl iron powder/SiO2–reduced iron powder/SiO2 soft magnetic composites with a high resistivity and low core loss. J. Magn. Magn. Mater. 464, 161–167 (2018)

    Article  ADS  Google Scholar 

  18. Geng, K., Xie, Y., Xu, L., Yan, B.: Structure and magnetic properties of ZrO2-coated Fe powders and Fe/ZrO2 soft magnetic composites. Adv. Powder. Technol. 28, 2015–2022 (2017)

    Article  Google Scholar 

  19. Geng, K., Xie, Y., Yan, L., Yan, B.: Fe-Si/ZrO2 composites with core-shell structure and excellent magnetic properties prepared by mechanical milling and spark plasma sintering. J. Alloy. Compd. 718, 53–62 (2017)

    Article  Google Scholar 

  20. Peng, Y., Yi, Y., Li, L., Ai, H., Wang, X., Chen, L.: Fe-based soft magnetic composites coated with NiZn ferrite prepared by a co-precipitation method. J. Magn. Magn. Mater. 428, 148–153 (2017)

    Article  ADS  Google Scholar 

  21. Lauda, M., Füzer, J., Kollár, P., Strečková, M., Bureš, R., Kováč, J., Baťková, M., Baťko, I.: Magnetic properties and loss separation in FeSi/MnZnFe2O4 soft magnetic composites. J. Magn. Magn. Mater. 411, 12–17 (2016)

    Article  ADS  Google Scholar 

  22. Li, J., Peng, X., Yang, Y., Ge, H.: Preparation and characterization of MnZn/FeSiAl soft magnetic composites. J. Magn. Magn. Mater. 426, 132–136 (2017)

    Article  ADS  Google Scholar 

  23. Chicinasa, I., Geoffroy, O., Isnard, O., Pop, V.: Soft magnetic composite based on mechanically alloyed nanocrystalline Ni3Fe phase. J. Magn. Magn. Mater. 290–291, 1531–1534 (2005)

    Article  ADS  Google Scholar 

  24. Stoppels, D.: Developments in soft magnetic power ferrites. J. Magn. Magn. Mater. 160, 323–328 (1996)

    Article  ADS  Google Scholar 

  25. Zhu, S., Ni, J., Feng, S.: Investigation on magnetic power loss in strontium doped Ba1-xSrxTi1.2Co1.2Fe9.6O19 hexaferrites. Mater. Res. Express. 6, 116–122 (2019)

    Google Scholar 

  26. Zhou, Y., Kou, X., Mu, M., Brandon, M., Chen, X.: Loss characterization of Mo-doped FeNi flake for DC-to-DC converter and MHz frequency applications. J. Appl. Phys. 111, 07E329 (2012)

    Article  Google Scholar 

Download references

Funding

This work was supported by the National Natural Science Foundation of China (No. 51872004), by the Education Department of Anhui Province (Nos. KJ2019ZD03, KJ2013B293, KJ2018A0039) and by the Key Research and Development Plan of Anhui Province(No. 201904a05020038).

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Correspondence to Shuangjiu Feng or Xiansong Liu.

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Zhu, S., Wang, Z., Kan, X. et al. FeNi/Glass Soft Magnetic Composites with High Magnetic Properties. J Supercond Nov Magn 35, 1165–1172 (2022). https://doi.org/10.1007/s10948-022-06166-z

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