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Temperature and Frequency Dependence of Negative Capacitance, Dielectric and Electric Properties in La0.57Nd0.1Sr0.13Ag0.2MnO3 Ceramic

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Abstract

A detailed study of electrical and dielectric properties of the La0.57Nd0.1Sr0.13Ag0.2MnO3 ceramic prepared by conventional solid-state reaction has been presented in this work. The frequency and temperature dependencies of capacitance (C–f–T) and conductance (G–f–T) of the sample were investigated in the frequency and temperature ranges of 40 Hz-110 MHz and 80 to 400 K, respectively. The C–f–T plot shows a phenomenon of negative capacitance (NC) which has been attributed to the blocking of charge carriers at the electrodes and the injection of minority carriers. Frequency and temperature dependencies of C and G show that these parameters are responsible for understanding conduction mechanism and charge transfer in materials. The frequency and temperature dependencies of dielectric properties such as the real and imaginary parts of permittivity (ε’, ε”), electrical modulus (M’, M”) and the real part of impedance (Z’) were obtained from the measurement of capacitance (C) and conductance (G) data. Negative dielectric constant is calculated from NC measurement, and it was attributed to the polarization effect. The ac conductivity versus frequency curve obeys to the Drude model. The ε’, ε”, tan δ and σac show a dispersion at lower frequencies. From the electrical and dielectric measurements, the metal–semiconductor behavior was observed for the sample at a transition temperature of the order of 280 K.

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Funding

This project was supported by the Deanship of Scientific Research at Prince Sattam Bin Abdulaziz University,Project No. 2020/01/16565,Mohamed Lamjed Bouazizi.

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Authors and Affiliations

  1. Research Unit of Valuation and Optimization of Resource, Faculty of Science and Technology of Sidi Bouzid, University of Kairouan, University Campus Agricultural City, 9100, Sidi Bouzid, Tunisia

    M. Nasri, Omar Rejaiba & J. Khelifi

  2. Higher Institute of Applied Sciences and Technology of Gabes (ISSATG), University of Gabes, 6072, Riadh City Zrig, Tunisia

    Omar Rejaiba & J. Khelifi

  3. Department of Physics, College of Sciences, Qassim University, Buraydah, Saudi Arabia

    Raihane Charguia

  4. Condensed Matter Physics Laboratory, Department of Physics, Faculty of Sciences of Tunis, University of Tunis El Manar, Tunis, Tunisia

    Raihane Charguia

  5. Laboratoire de Physique Des Matériaux Et Des Nanomatériaux Appliquée À L’Environnement, Faculté Des Sciences de Gabès Cité Erriadh, Université de Gabès, 6079, Gabès, Tunisia

    M. A. Wederni & K. Khirouni

  6. Department of Mechanical Engineering, College of Engineering, Prince Sattam Bin Abdulaziz University, Alkharj, 11942, Saudi Arabia

    H. Al Robei & M. L. Bouazizi

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  1. M. Nasri
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  2. Omar Rejaiba
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  3. Raihane Charguia
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  8. J. Khelifi
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Correspondence to Omar Rejaiba.

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Nasri, M., Rejaiba, O., Charguia, R. et al. Temperature and Frequency Dependence of Negative Capacitance, Dielectric and Electric Properties in La0.57Nd0.1Sr0.13Ag0.2MnO3 Ceramic. J Low Temp Phys 206, 250–268 (2022). https://doi.org/10.1007/s10909-021-02656-x

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  • DOI: https://doi.org/10.1007/s10909-021-02656-x

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