Abstract
Path-integral Monte Carlo calculations have been performed to study superfluid behavior of small para-H2 clusters doped by a single impurity molecule of ortho-D2 at a low temperature of 1.6 K. It is found that the D2 molecule is located near the center of mass of the cluster and H2 molecules are distributed around the D2 molecule to form a shell structure. All the clusters considered here show significant superfluid fractions at this temperature but superfluidity is found to be noticeably quenched at specific sizes of the clusters. The different superfluid propensity depending on the cluster size is understood to be related to the magic number behavior of the para-H2 clusters.
Similar content being viewed by others
References
P. Sindzingre et al., Phys. Rev. Lett. 67, 1871 (1991)
D.F. Brewer et al., J. Low Temp. Phys. 101, 317 (1995)
M. Schindler et al., Phys. Rev. B 53, 11451 (1996)
S. Grebenev et al., Science 289, 1532 (2000)
Y. Kwon, K.B. Whaley, Phys. Rev. Lett. 89, 273401 (2002)
S.A. Khairallah et al., Phys. Rev. Lett. 98, 183401 (2007)
U. Buck et al., J. Chem. Phys. 78, 4439 (1983)
D.M. Ceperley, Rev. Mod. Phys. 67, 279 (1995)
P. Sindzingre et al., Phys. Rev. Lett. 63, 1601 (1989)
R. Guardiola, J. Navarro, Phys. Rev. A 74, 025201 (2006)
J.E. Cuervo, P.-N. Roy, J. Chem. Phys. 125, 124314 (2006)
S. Baroni, S. Moroni, Chem. Phys. Chem. 6, 1884 (2005)
Y. Kwon et al., Phys. Rev. B 74, 174522 (2006)
E.W. Draeger, D.M. Ceperley, Phys. Rev. Lett. 90, 065301 (2003)
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Choo, J., Kwon, Y. Magic Number Stabilities of Small para-H2 Clusters Doped by a Single ortho-D2 . J Low Temp Phys 150, 358–363 (2008). https://doi.org/10.1007/s10909-007-9557-9
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s10909-007-9557-9