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Construction of a 2D Polymer by Rigid Dicarboxylate and Methylimidazol Derivatives: Structure and Photocatalytic Feature

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Abstract

A new 2D coordination polymer, namely{[Cd2(BDC)2(bmb)2]·H2O}n (1) (H2BDC = 1,4-benzenedicarboxylic acid and bmb = 1,4-bis(2-methyl-1H-imidazol-1-yl)butane), has been prepared and full characterized. Coordination polymer 1 has 2D layer, which was further extended into 3D supramolecular motif through the π–π packing interactions. Coordination polymer 1 illustrated effectively photocatalytic performance to the disintegration of dyes Rhodamine B (Rh B), methyl orange (MO) and methylene blue (MB). Coordination polymer 1 can remove the dye MB with 90.37% after 100 min under simulated UV light and its catalytic feature conforms to the first order kinetics model. In addition, the possible mechanism of the catalytic degradation toward MB was suggested through the trapping experiments and LC–MS methods.

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Acknowledgements

Dr. Mohd. Muddassir is grateful to Researchers Supporting Project number (RSP-2021/141), King Saud University, Riyadh, Saudi Arabia, for financial assistance. The authors acknowledge financial assistance from Sichuan University of Science and Engineering (No. 2019RC21), the Open Project of Chemical Synthesis and Pollution Control Key Laboratory of Sichuan Province (No. CSCP202108), the Opening Project of Key Laboratory of Green Chemistry of Sichuan Institutes of Higher Education (No. LYJ2101), Featured Innovation Project of Guangdong Province (2019KTSCX052 and 2019KTSCX053).

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Authors and Affiliations

  1. School of Chemistry and Environmental Engineering, Sichuan University of Science & Engineering, Zigong, People’s Republic of China

    Weiping Wu, Lu Lu & Jun Wang

  2. Guangdong Provincial Key Laboratory of Research and Development of Natural Drugs, and School of Pharmacy, Guangdong Medical University, Guangdong Medical University Key Laboratory of Research and Development of New Medical Materials, Dongguan, 523808, China

    Donghui Liao, Baohong Li & Xuezhang Liu

  3. Department of Chemistry, College of Sciences, King Saud University, Riyadh, 11451, Saudi Arabia

    Mohd. Muddassir

  4. Department of Science, Faculty of Science, Yamagata University, 1-4-12 Kojirakawa, Yamagata, 990-8560, Japan

    Hiroshi Sakiyama

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CCDC < 2097246 > contains the supplementary crystallographic data for 1. These data can be obtained free of charge via http://www.ccdc.cam.ac.uk/conts/retrieving.html, or from the Cambridge Crystallographic Data Centre, 12 Union Road, Cambridge CB2 1EZ, UK; fax: (+44) 1223-336-033; or e-mail: deposit@ccdc.cam.ac.uk.

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Wu, W., Lu, L., Liao, D. et al. Construction of a 2D Polymer by Rigid Dicarboxylate and Methylimidazol Derivatives: Structure and Photocatalytic Feature. J Inorg Organomet Polym 32, 875–882 (2022). https://doi.org/10.1007/s10904-021-02150-7

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