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A Significant Role of Tb2O3 on the Optical Properties and Radiation Shielding Performance of Ga2O3–B2O3–Al2O3–GeO2 Glasses

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Abstract

This research article focuses on the significant role of Tb2O3 content on the optical properties and radiation shielding performance of Ga2O3–B2O3–Al2O3–GeO2 glasses named as GBAGT1, GBAGT2, GBAGT3, and GBAGT4 for Tb2O3 of 14, 18, 22 and 25 mol%, respectively. The findings of the optical study indicate that the optical dielectric constant of the present samples increased from 1.85 to 2.06 as the Tb2O3 content increased from 14 to 25 mol%. The results of the radiation shielding confirm that increasing Tb3+-dopant content in GBAGT4 increased its specific gamma ray constant (Γ) values over all other glass samples in the whole energy region. With increasing electron energy, the mass stopping power decreased for all samples and reached the minimum 1.372 and 1.327 (MeV cm2/g) for BGAGT1, BGAGT4, respectively, at 1 MeV electron energy. For a beam of neutrons of 0.1 meV, the total cross section in GBAGT1, GBAGT2, GBAGT3, and GBAGT4 was 294.54, 312.88, 317.24 and 311.69 (cm−1), respectively. The smallest MFP values of GBAGT4 glass sample in all energy regions confirm the superior shielding performance of the studied glass sample among other shielding materials namely traditional concrete and commercial polymers/glasses.

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References

  1. W.C. Wang, B. Zhou, S.H. Xu, Z.M. Yang, Q.Y. Zhang, Recent advances in soft optical glass fiber and fiber lasers. Prog. Mater. Sci. 101, 90–171 (2019)

    Article  CAS  Google Scholar 

  2. N.P. Bansal, R.H. Doremus, Handbook of Glass Properties (Elsevier, Amsterdam, 2013).

    Google Scholar 

  3. P.H. Gaskell, Structure, glass formation and properties. J. Non-Cryst. Solids 192, 9–22 (1995)

    Article  Google Scholar 

  4. I. Boukhris, M.S. Al-Buriahi, H. Akyildirim, A. Alalawi, I. Kebaili, M.I. Sayyed, Chalcogenide glass-ceramics for radiation shielding applications. Ceram. Int. 46(11), 19385–19392 (2020)

    Article  CAS  Google Scholar 

  5. A. Alalawi, M.S. Al-Buriahi, M.I. Sayyed, H. Akyildirim, H. Arslan, M.H.M. Zaid, B.T. Tonguc, Influence of lead and zinc oxides on the radiation shielding properties of tellurite glass systems. Ceram. Int. 46(11), 17300–17306 (2020)

    Article  CAS  Google Scholar 

  6. M.S. Al-Buriahi, Y.S.M. Alajerami, A.S. Abouhaswa, A. Alalawi, T. Nutaro, B. Tonguc, Effect of chromium oxide on the physical, optical, and radiation shielding properties of lead sodium borate glasses. J. Non-Cryst. Solids 544, 120171 (2020)

    Article  CAS  Google Scholar 

  7. I. Boukhris, I. Kebaili, M.S. Al-Buriahi, C. Sriwunkum, M.I. Sayyed, Effect of lead oxide on the optical properties and radiation shielding efficiency of antimony-sodium-tungsten glasses. Appl. Phys. A 126(10), 1–10 (2020)

    Article  Google Scholar 

  8. H. Cheng, Hu. Yuanan, Lead (Pb) isotopic fingerprinting and its applications in lead pollution studies in China: a review. Environ. Pollut. 158(5), 1134–1146 (2010)

    Article  CAS  PubMed  Google Scholar 

  9. M.S. Al-Buriahi, D.K. Gaikwad, H.H. Hegazy, C. Sriwunkum, H. Algarni, Newly developed glasses containing Si/Cd/Li/Gd and their high performance for radiation applications: role of Er2O3. J. Mater. Sci. 32(7), 9440–9451 (2021)

    CAS  Google Scholar 

  10. O. Holmberg, R. Czarwinski, F. Mettler, The importance and unique aspects of radiation protection in medicine. Eur. J. Radiol. 76(1), 6–10 (2010)

    Article  PubMed  Google Scholar 

  11. G.V. Koz'min, N.I. Sanzharova, Radiation technologies in agriculture and food industry. in The 10th Anniversary Russian Scientific Conference Radiation Protection and Radiation Safety in Nuclear Technologies. Book of abstracts (2015)

  12. A.E. Khater, H.A. Al-Sewaidasn, Radiation exposure due to agricultural uses of phosphate fertilizers. Radiat. Meas. 43(8), 1402–1407 (2008)

    Article  CAS  Google Scholar 

  13. J. Wang, J. Wang, Application of radiation technology to sewage sludge processing: a review. J. Hazard. Mater. 143(1–2), 2–7 (2007)

    Article  CAS  PubMed  Google Scholar 

  14. J.P. McCaffrey, H. Shen, B. Downton, E. Mainegra-Hing, Radiation attenuation by lead and nonlead materials used in radiation shielding garments. Med. Phys. 34(2), 530–537 (2007)

    Article  CAS  PubMed  Google Scholar 

  15. I. Boukhris, A. Alalawi, M.S. Al-Buriahi, I. Kebaili, M.I. Sayyed, Radiation attenuation properties of bioactive glasses doped with NiO. Ceram. Int. 46(12), 19880–19889 (2020)

    Article  CAS  Google Scholar 

  16. I. Kebaili, I. Boukhris, M.S. Al-Buriahi, A. Alalawi, M.I. Sayyed, Ge-Se-Sb-Ag chalcogenide glasses for nuclear radiation shielding applications. Ceram. Int. 47(1), 1303–1309 (2021)

    Article  CAS  Google Scholar 

  17. G. Sathiyapriya, K.A. Naseer, K. Marimuthu, E. Kavaz, A. Alalawi, M.S. Al-Buriahi, Structural, optical and nuclear radiation shielding properties of strontium barium borate glasses doped with dysprosium and niobium. J. Mater. Sci. 32(7), 8570–8592 (2021)

    CAS  Google Scholar 

  18. M.S. Al-Buriahi, S. Alomairy, D.K. Gaikwad, H.H. Hegazy, C. Mutuwong, Y.S. Rammah, Effects of AgO addition on the mechanical, optical, and radiation attenuation properties of V2O5/P2O5/B2O3 glass system. Appl. Phys. A 127(3), 1–14 (2021)

    Article  Google Scholar 

  19. M.S. Al-Buriahi, H.H. Somaily, A. Alalawi, S. Alraddadi, Polarizability, optical basicity, and photon attenuation properties of Ag2O–MoO3–V2O5–TeO2 glasses: the role of silver oxide. J. Inorg. Organometall. Polym. Mater. 31(3), 1047–1056 (2021)

    Article  CAS  Google Scholar 

  20. M.S. Al-Buriahi, C. Eke, S. Alomairy, A. Yildirim, H.I. Alsaeedy, C. Sriwunkum, Radiation attenuation properties of some commercial polymers for advanced shielding applications at low energies. Adv. Technol. Polym. (2021). https://doi.org/10.1002/pat.5267

    Article  Google Scholar 

  21. B. Alshahrani, I.O. Olarinoye, C. Mutuwong, C. Sriwunkum, H.A. Yakout, H.O. Tekin, M.S. Al-Buriahi, Amorphous alloys with high Fe content for radiation shielding applications. Radiat. Phys. Chem. 183, 109386 (2021)

    Article  CAS  Google Scholar 

  22. M.S. Al-Buriahi, D.K. Gaikwad, H.H. Hegazy, C. Sriwunkum, R. Neffati, Fe-based alloys and their shielding properties against directly and indirectly ionizing radiation by using FLUKA simulations. Phys. Scr. 96(4), 045303 (2021)

    Article  CAS  Google Scholar 

  23. M.S. Al-Buriahi, V.P. Singh, H. Arslan, V.V. Awasarmol, B.T. Tonguc, Gamma-ray attenuation properties of some NLO materials: potential use in dosimetry. Radiat. Environ. Biophys. 59(1), 145–150 (2020)

    Article  CAS  PubMed  Google Scholar 

  24. M.S. Al-Buriahi, V.P. Singh, Comparison of shielding properties of various marble concretes using GEANT4 simulation and experimental data. J. Aust. Ceram. Soc. 56(3), 1127–1133 (2020)

    Article  CAS  Google Scholar 

  25. G. Gao, A. Winterstein-Beckmann, O. Surzhenko, C. Dubs, J. Dellith, M.A. Schmidt, L. Wondraczek, Faraday rotation and photoluminescence in heavily Tb 3+-doped GeO2-B2O3-Al2O3-Ga2O3 glasses for fiber-integrated magneto-optics. Sci. Rep. 5(1), 1–6 (2015)

    Google Scholar 

  26. G. Battistoni, F. Cerutti, A. Fasso, A. Ferrari, S. Muraro, J. Ranft, S. Roesler, P.R. Sala, The FLUKA code: description and benchmarking. In AIP Conf. Proc., vol. 896, No. 1. (American Institute of Physics, 2007), pp. 31–49

  27. M.I. Sayyed, H. Akyildirim, M.S. Al-Buriahi, E. Lacomme, R. Ayad, G. Bonvicini, Oxyfluoro-tellurite-zinc glasses and the nuclear-shielding ability under the substitution of AlF 3 by ZnO. Appl. Phys. A 126(2), 1–12 (2020)

    Article  Google Scholar 

  28. M.S. Al-Buriahi, B.T. Tonguc, Mass attenuation coefficients, effective atomic numbers and electron densities of some contrast agents for computed tomography. Radiat. Phys. Chem. 166, 108507 (2020)

    Article  CAS  Google Scholar 

  29. M.S. Al-Buriahi, K.S. Mann, Radiation shielding investigations for selected tellurite-based glasses belonging to the TNW system. Mater. Res. Express 6(10), 105206 (2019)

    Article  CAS  Google Scholar 

  30. B.T. Tonguc, H. Arslan, M.S. Al-Buriahi, Studies on mass attenuation coefficients, effective atomic numbers and electron densities for some biomolecules. Radiat. Phys. Chem. 153, 86–91 (2018)

    Article  CAS  Google Scholar 

  31. M.J. Berger, J.H. Hubbell, XCOM: Photon cross sections on a personal computer. No. NBSIR-87-3597. National Bureau of Standards, Washington, DC (USA). Center for Radiation Research, (1987)

  32. F.C. Hila, A. Asuncion-Astronomo, C.A. Dingle, J.F. Jecong, A.M. Javier-Hila, M.B. Gili, C.V. Balderas, G.E. Lopez, N.R. Guillermo, A.V. Amorsolo Jr., EpiXS: a Windows-based program for photon attenuation, dosimetry and shielding based on EPICS2017 (ENDF/B-VIII) and EPDL97 (ENDF/B-VI 8). Radiat. Phys. Chem. 182, 109331 (2021)

    Article  CAS  Google Scholar 

  33. M.S. Al-Buriahi, H. Arslan, B.T. Tonguc, Investigation of photon energy absorption properties for some biomolecules. Nucl. Sci. Techn. 30(7), 1–9 (2019)

    Article  Google Scholar 

  34. H.H. Hegazy, M.S. Al-Buriahi, F. Alresheedi, F.I. El-Agawany, C. Sriwunkum, R. Neffati, Y.S. Rammah, Nuclear shielding properties of B2O3–Bi2O3–SrO glasses modified with Nd2O3: theoretical and simulation studies. Ceram. Int. 47(2), 2772–2780 (2020)

    Article  Google Scholar 

  35. S. Stalin, D.K. Gaikwad, M.S. Al-Buriahi, C. Srinivasu, S.A. Ahmed, H.O. Tekin, S. Rahman, Influence of Bi2O3/WO3 substitution on the optical, mechanical, chemical durability and gamma ray shielding properties of lithium-borate glasses. Ceram. Int. 47(4), 5286–5299 (2020)

    Article  Google Scholar 

  36. H.H. Somaily, H. Algarni, S. Alraddadi, Y.S. Rammah, T. Nutaro, M.S. Al-Buriahi, Mechanical, optical, and beta/gamma shielding properties of alkali tellurite glasses: role of ZnO. Ceram. Int. 46(18), 28594–28602 (2020)

    Article  CAS  Google Scholar 

  37. I. Boukhris, I. Kebaili, M.S. Al-Buriahi, A. Alalawi, A.S. Abouhaswa, B. Tonguc, Photon and electron attenuation parameters of phosphate and borate bioactive glasses by using Geant4 simulations. Ceram. Int. 46(15), 24435–24442 (2020)

    Article  CAS  Google Scholar 

  38. I.I. Bashter, Calculation of radiation attenuation coefficients for shielding concretes. Ann. Nucl. Energy. 24(17), 1389–1401 (1997). https://doi.org/10.1016/S0306-4549(97)00003-0

    Article  CAS  Google Scholar 

  39. M.S. Al-Buriahi et al., Radiation attenuation properties of some commercial polymers for advanced shielding applications. Polym. Adv. Technol. (2021). https://doi.org/10.1002/pat.5267

    Article  Google Scholar 

  40. M.S. Al-Buriahi, E.M. Bakhsh, B. Tonguc, S.B. Khan, Mechanical and radiation shielding properties of tellurite glasses doped with ZnO and NiO. Ceram. Int. 46(11), 19078–19083 (2020)

    Article  CAS  Google Scholar 

  41. Y.S. Rammah et al., Investigations on borate glasses within SBC-Bx system for gamma-ray shielding applications. Nucl. Eng. Technol. 53(1), 282–293 (2021). https://doi.org/10.1016/j.net.2020.06.034

    Article  CAS  Google Scholar 

  42. I.O. Olarinoye et al., The effects of La2O3 addition on mechanical and nuclear shielding properties for zinc borate glasses using Monte Carlo simulation. Ceram. Int. 46(18), 29191–29198 (2020). https://doi.org/10.1016/j.ceramint.2020.08.092

    Article  CAS  Google Scholar 

  43. M.S. Al-Buriahi, B. Tonguç, U. Perişanoğlu, E. Kavaz, The impact of Gd2O3 on nuclear safety proficiencies of TeO2–ZnO–Nb2O5 glasses: a GEANT4 Monte Carlo study. Ceram. Int. 46(15), 23347–23356 (2020)

    Article  CAS  Google Scholar 

  44. M.J. Berger, ESTAR, PSTAR, and ASTAR: Computer programs for calculating stopping-power and range tables for electrons, protons, and helium ions. Unknow (1992)

  45. J.F. Ziegler, M.D. Ziegler, J.P. Biersack, SRIM–The stopping and range of ions in matter. Nucl. Instrum. Methods Phys. Res. Sect. B 268(11–12), 1818–1823 (2010)

    Article  CAS  Google Scholar 

  46. J.S. Alzahrani, M.A. Alothman, C. Eke, H. Al-Ghamdi, D.A. Aloraini, M.S. Al-Buriahi, Simulating the radiation shielding properties of TeO2–Na2O–TiO glass system using PHITS Monte Carlo code. Comput. Mater. Sci. 196, 110566 (2021)

    Article  CAS  Google Scholar 

  47. I. Kebaili, S. Znaidia, J.S. Alzahrani, M.A. Alothman, I. Boukhris, I.O. Olarinoye, C. Mutuwong, M.S. Al-Buriahi, Ge 20 Se 80-x Bi x (x≤ 12) chalcogenide glasses for infrared and gamma sensing applications: structural, optical and gamma attenuation aspects. J. Mater. Sci. 1–14 (2021)

  48. M.S. Al-Buriahi, J.S. Alzahrani, I.O. Olarinoye, H. Akyildirim, S. Alomairy, I. Kebaili, H.O. Tekin, C. Mutuwong, Role of heavy metal oxides on the radiation attenuation properties of newly developed TBBE-X glasses by computational methods. Phys. Scr. 96(7), 075302 (2021)

    Article  Google Scholar 

  49. J. Singh, V. Kumar, Y.K. Vermani, M.S. Al-Buriahi, J.S. Alzahrani, T. Singh, Fabrication and characterization of barium based bioactive glasses in terms of physical, structural, mechanical and radiation shielding properties. Ceram. Int. (2021). https://doi.org/10.1016/j.ceramint.2021.04.188

    Article  Google Scholar 

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Acknowledgements

This research was funded by the Deanship of Scientific Research at Princess Nourah bint Abdulrahman University through the Fast-track Research Funding Program to support publication in the top journal (Grant no. 44-FTTJ-66).

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Correspondence to H. H. Saleh or M. S. Al-Buriahi.

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Alzahrani, J.S., Alrowaili, Z.A., Saleh, H.H. et al. A Significant Role of Tb2O3 on the Optical Properties and Radiation Shielding Performance of Ga2O3–B2O3–Al2O3–GeO2 Glasses. J Inorg Organomet Polym 31, 4300–4312 (2021). https://doi.org/10.1007/s10904-021-02040-y

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