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Matching Charge Towards Synthesis of Tetrazole Frameworks for Iodine Uptake

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Abstract

Up to now, the experience that matching the total and local charge in advance will effect on the success of synthesis for metal–organic frameworks has been confirmed. In this work, we report two tetrazole-frameworks based on binuclear and trinuclear cluster Zn, respectively, namely [Zn2(btz)2(bdc)]·(solvents) (1) and [Zn3(atz)(bdc)3]·(cation)·(solvents) (2) (bdc = 1,4-benzenedicarboxylate acid, btz = 5-benzyl-1H-tetrazole, atz = 5-amino-1H-tetrazole). The result showed that pre-computing the charge can determine whether ionic template agent should present in the synthetic process, which could perfect the intentionality of design and synthesis of crystalline materials. Meanwhile compound 1 also exhibited the characteristic of reversible adsorption of iodine.

Graphic Abstract

Presented here is that pre-computing the total and local charge can determine whether ionic template agent should be added during the synthetic process, which could perfect the intentionality of design and synthesis of metal-organic frameworks.

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Acknowledgements

We gratefully acknowledge the Science and Technology Planning Project in Sichuan Province (2019YJ0686), the Science and Technology Planning Project in Panzhihua City (2019ZD-G-11) for supporting this work.

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Authors and Affiliations

  1. School of Materials Science and Engineering, Xihua University, Chengdu, 610039, Sichuan, People’s Republic of China

    Yu Du & Zhi-Qiang Jiang

  2. Deep-Processing of Fine Flake Graphite Sichuan Province Key Laboratory of Colleges and Universities, Panzhihua University, Panzhihua, 617000, Sichuan, People’s Republic of China

    Yu Du, Jin Lu, Hui Chang, Yu-Feng Li, Bi Foua claude Alain Gohi & Zhi-Qiang Jiang

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  1. Yu Du
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  2. Jin Lu
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  3. Hui Chang
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  4. Yu-Feng Li
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  5. Bi Foua claude Alain Gohi
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  6. Zhi-Qiang Jiang
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Correspondence to Jin Lu, Yu-Feng Li or Zhi-Qiang Jiang.

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Du, Y., Lu, J., Chang, H. et al. Matching Charge Towards Synthesis of Tetrazole Frameworks for Iodine Uptake. J Inorg Organomet Polym 30, 4764–4770 (2020). https://doi.org/10.1007/s10904-020-01592-9

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  • DOI: https://doi.org/10.1007/s10904-020-01592-9

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