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Design Strategies of Metal Complexes Based on Chelating Polymer Ligands and Their Application in Nanomaterials Science

  • Gulzhian I. Dzhardimalieva
  • Igor E. Uflyand
Topical Review
  • 304 Downloads

Abstract

The advances and problems associated with the synthesis, properties and structure of metal complexes based on chelating polymer ligands are presented and assessed. The polymeric metal chelates (PMCs) are divided into molecular, intracomplex, macrocyclic and polynuclear types, which in turn are grouped according to the nature of the donor atoms (N,N-, N,О-, N,S-, О,О-, O,S-, S,S-, Р,Р-chelates, etc.). The main attention is focused on the similarities and differences between low and high molecular weight metal chelates, as well as the spatial organization of PMCs. The most important areas of research in the field of such compounds are highlighted. Thermal transformations of metal complexes based on chelating polymer ligands leading to the formation of nanostructured materials are considered. The bibliography includes the articles published after 2010.

Keywords

Polymeric metal chelates Molecular metal chelates Intracomplex compounds Macrocyclic complexes Polynuclear metal chelates 

Abbreviations

AAm

Acrylamide

Acac

Acetylacetonate anion

ATRP

Atom transfer radical polymerization

BINAM

2,2′-Binaphthyldiamine

BINOL

1,1′-Bi-2-naphtol

BPP

2,6-Bis(pyrazolyl)pyridine

bpy

2,2′-Bipyridine

CIE

International Commission on Illumination

CMC

Critical concentration of micelle formation

CN

Coordinative number

COD

1,5-Cyclooctadiene

CPL

Chelating polymer ligand

dien

Diethylene triamine

DIPY

Dipyromethene

DP

Polymerization degree

DOTA

1,4,7,10-Tetraazacyclododecane-1,4,7,10-tetraacetic acid

DTPA

Diethylenetriamine pentacetic acid

DVB

Divinylbenzene

EDAX

Energy dispersive X-ray analysis

EDTA

Ethylenediaminetetraacetic acid

EL

Electroluminescence

en

Ethylenediamine

GMA

Glycidyl methacrylate

HQ

8-Hydroxyquinoline

8HQ5S

8-Hydroxyquinoline-5-sulfonic acid

IDA

Iminodiacetic acid

Ksv

Stern–Volmer constant

LCST

Lower critical solution temperature

LMC

Low molecular weight metal chelate

MC

Merocyanine

MLCT

Metal-to-ligand charge transfer

MMA

Methyl methacrylate

Mn

Number-average molecular weight

MRI

Magnetic resonance imaging

MXn

Metal compound

Mw

Weight-average molecular weight

NCF

Nitrogen-doped carbon microfiber

NIPAM

N-Isopropylacrylamide

NIR

Near-infrared

NVK

N-Vinylcarbazole

PAA

Polyacrylic acid

PAAm

Polyacrylamide

PAMAM

Polyamidoamines

PAN

Polyacrylonitrile

Pc

Phthalocyanine

PCD

Poly(chloromethylstyrene-co-divinylbenzene)

PCN

Porphyrinic conjugated network

PCS

Polychloromethylstyrene

PDI

Polydispersity index

PEG

Polyethylene glycol

PEI

Polyethylene imine

PEO

Poly(ethylene oxide)

PET

Photoinduced electron transfer

phen

1,10-Phenanthroline

PIB

Polyisobutylene

PL

Photoluminescence

PLL

Poly-l-lysine

PLQY

Photoluminescence quantum yield

PMA

Poly(methacrylate)

PMC

Polymeric metal chelate

Pp

Porphyrin

ppy

2-Phenylpyridine

PS

Polystyrene

PVC

Poly(vinyl chloride)

pybox

Pyridine-bis(oxazoline)

ROMP

Ring-open metathesis polymerization

ROP

Ring-opening polymerization

salen

N,N′-Bis(salicylidene)ethylenediamine

salphen

N,N′-Phenylenebis(salicylideneimine)

SEM

Scanning electron microscopy

SP

Spiropyran

St

Styrene

TEM

Transmission electron microscopy

tpy

2,2′,6′,2′′-Terpyridine

trien

Triethylenetetramine

TTA

1-(2-Thenoyl)-3,3,3-trifluoroacetonate

XPS

X-ray photoelectron spectrometry

XRD

X-ray diffraction

Notes

Compliance with Ethical Standards

Conflict of interest

The authors declare no competing financial interest.

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© Springer Science+Business Media, LLC, part of Springer Nature 2018

Authors and Affiliations

  1. 1.Laboratory of MetallopolymersThe Institute of Problems of Chemical Physics RASChernogolovkaRussian Federation
  2. 2.Department of ChemistrySouthern Federal UniversityRostov-on-DonRussian Federation

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