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A Non-interpenetrated Microporous Bi-pillared-Layer Framework: Synthesis, Structure and Photoluminescence Properties

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Abstract

A non-interpenetrated microporous bi-pillared-layer framework of Zn(II), {[Zn(hip)(4,4′-bipy)](DMA)·(4H2O)}n (1) (H2hip = 5-hydroxyisophthalic acid; 4,4′-bipy = 4,4′-bipyridine; DMA = N,N′-diethylformamide) composed of mixed ligand system has been synthesized and structurally characterized. The hip linkers form a 2D corrugated sheet of {Zn(hip)}n by linking the secondary building unit of Zn2(CO2)2 in the bc plane, which are further connected by double 4,4′-bipy pillars resulting in a bi-pillared-layer type 3D framework. The 3D framework is non-interpenetrated and exhibits a 3D channel structure occupied by the guest DMA molecules. The thermal stability and luminescent properties were also investigated.

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Acknowledgments

We gratefully thank the financial support of the NSF of China (Grant No. 21301129), Shandong Provincial Natural Science Foundation (ZR2010BL011), and Shandong Province Higher Educational Science and Technology Program (J06A55), Science and Technology Program of Weifang (2014GX025).

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  1. College of Chemical Engineering and Environmental Chemistry, Weifang University, Weifang, 261061, China

    Jitao Lu, Haiyan Sui, Dandan Meng & Qingguo Meng

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  1. Jitao Lu
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  2. Haiyan Sui
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Correspondence to Jitao Lu or Qingguo Meng.

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Lu, J., Sui, H., Meng, D. et al. A Non-interpenetrated Microporous Bi-pillared-Layer Framework: Synthesis, Structure and Photoluminescence Properties. J Inorg Organomet Polym 25, 936–941 (2015). https://doi.org/10.1007/s10904-015-0194-5

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